Related papers: Direct frequency comb spectroscopy of trapped ions
We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an…
The coupled motion of ions in a radiofrequency trap has been used to connect the frequency- dependent laser-induced heating of a sympathetically cooled spectroscopy ion with changes in the fluorescence of a laser-cooled control ion. This…
Cavity-enhanced direct frequency comb spectroscopy (CE-DFCS) has demonstrated powerful potential for trace gas detection based on its unique combination of high bandwidth, rapid data acquisition, high sensitivity, and high resolution, which…
We report the laser-cooling and confinement of Cd atoms in a magneto-optical trap, and characterize the loading process from the background Cd vapor. The trapping laser drives the 1S0-1P1 transition at 229 nm in this two-electron atom and…
$^{133}\text{Ba}^+$ has been identified as an attractive ion for quantum information processing due to the unique combination of its spin-1/2 nucleus and visible wavelength electronic transitions. Using a microgram source of radioactive…
Using optical Ramsey interferometry, we precisely measure the laser-induced AC-stark shift on the $S_{1/2}$ -- $D_{5/2}$ "quantum bit" transition near 729 nm in a single trapped $^{40}$Ca$^+$ ion. We cancel this shift using an additional…
The absolute frequency measurement for all of the hyperfine transitions of 6P1/2 -> 7S1/2 using a self-referencing frequency comb is reported. This transition can be used as a bench marker for the accurate atomic wave function, and then…
We demonstrated the observation of Rb two-photon absorption directly excided by an optical frequency comb at fiber communication bands. A chain of comb spectral control is elaborately implemented to increase the power of the second harmonic…
We demonstrate the first cavity-enhanced optical frequency comb spectroscopy in the mid-infrared wavelength region and report the sensitive real-time trace detection of hydrogen peroxide in the presence of a large amount of water. The…
Coherent dual-comb spectroscopy (DCS) enables high-resolution measurements at high speeds without the trade-off between resolution and update rate inherent to mechanical delay scanning approaches. However, high system complexity and limited…
Frequency combs have revolutionized optical frequency metrology, allowing one to determine highly accurate transition frequencies of a wealth of molecular species. Despite a recognized scientific interest, these progresses have only…
We describe a measurement of the frequency of the 2S1/2(F = 0) - 2D3/2(F' = 2) transition of 171Yb+ at the wavelength 436 nm (frequency 688 THz), using a single Yb+ ion confined in a Paul trap and two caesium fountains as references. In one…
Direct comb spectroscopy is a useful tool for obtaining highly accurate spectroscopic information. However, as the number of comb modes is very large and the optical energy is dispersed over them, the optical energy per each comb mode is…
We study the feasibility of nearly-degenerate two-photon rovibrational spectroscopy in ensembles of trapped, sympathetically cooled hydrogen molecular ions using a resonance-enhanced multiphoton dissociation (REMPD) scheme. Taking advantage…
We demonstrate broadband and sensitive cavity ring-down spectroscopy using a near infrared frequency comb and a time-resolved Fourier transform spectrometer. The cavity decays are measured simultaneously and spectrally sorted, leading to…
A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2],…
We report precision measurements of the excited state lifetime of the $5p$ $^2P_{1/2}$ and $5p$ $^2P_{3/2}$ levels of a single trapped Cd$^+$ ion. The ion is excited with picosecond laser pulses from a mode-locked laser and the distribution…
We demonstrate quantum control of $^9$Be$^+$ ions directly implemented by an optical frequency comb. Based on numerical simulations of the relevant processes in $^9$Be$^+$ for different magnetic field regimes, we demonstrate a wide…
Optical frequency comb synthesizers (FCs) [1] are laser sources covering a broad spectral range with a number of discrete, equally spaced and highly coherent frequency components, fully controlled through only two parameters: the frequency…
We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…