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A new approach to observe the radiative decay of the $^{229}$Th nuclear isomer, and to determine its energy and radiative lifetime, is presented. Situated at a uniquely low excitation energy, this nuclear state might be a key ingredient for…

A possibility of amplification of the 7.6 eV $\gamma$-radiation by the stimulated $\gamma$-emission of the ensemble of the $^{229m}$Th isomeric nuclei in a host dielectric crystal is proved theoretically. This amplification is a result of:…

Nuclear Theory · Physics 2011-05-05 E. V. Tkalya

We aim to perform direct optical spectroscopy of the Th-229 nuclear isomer to measure its energy and lifetime, and to demonstrate optical coupling to the nucleus. To this end, we develop Th-doped CaF2 crystals, which are transparent at the…

The first nuclear excited state of $^{229}$Th offers the unique opportunity for laser-based optical control of a nucleus. Its exceptional properties allow for the development of a nuclear optical clock which offers a complementary…

Direct laser excitation of the lowest known nuclear excited state in $^{229}$Th has been a longstanding objective. It is generally assumed that reaching this goal would require a considerably reduced uncertainty of the isomer's excitation…

We have recently described a novel method for the construction of a solid-state optical frequency reference based on doping $^{229}$Th into high energy band-gap crystals. Since nuclear transitions are far less sensitive to environmental…

We report on the development and characterization of a medium resolution monochromator for synchrotron-based hyperfine spectroscopy at the 73 keV nuclear resonance of 193-Ir. The device provides high throughput of 6*10^8 ph/s in an energy…

The process of internal conversion from excited electronic states is investigated theoretically for the case of the vacuum-ultraviolet nuclear transition of $^{229}{\mathrm Th}$. Due to the very low transition energy, the $^{229}{\mathrm…

Atomic Physics · Physics 2017-03-22 Pavlo V. Bilous , Georgy A. Kazakov , Iain D. Moore , Thorsten Schumm , Adriana Pálffy

Thorium-229 has the lowest nuclear-excited state (an isomer state) at approximately 8.356 eV, making it excitable with tabletop vacuum-ultraviolet lasers. Despite the recent success of laser excitation, the isomer quenching inside the…

Peik and Tamm [Europhys. Lett. 61, 181 (2003)] proposed a nuclear clock based on the isomeric transition between the ground state and the first excited state of thorium-229. This transition was recognized as a potentially sensitive probe of…

Atomic Physics · Physics 2021-01-19 Pavel Fadeev , Julian C. Berengut , Victor V. Flambaum

The reduced magnetic dipole and electric quadrupole transition probabilities for the radiative decay of the $^{229}$Th 7.8 eV isomer to the ground state are predicted within a detailed nuclear-structure model approach. We show that the…

Nuclear Theory · Physics 2017-06-13 Nikolay Minkov , Adriana Pálffy

Ro-vibrational spectra of different electronic states of molecules are often used as absolute wavelength or frequency standards. These standards are also used to mitigate any slow drift of laser frequency during an experiment. In precision…

Atomic Physics · Physics 2018-10-17 T. Dutta , M. Mukherjee

A possibility of the two-photon excitation of an isomeric state in a nucleus of thorium-229 has been discussed. The fluorescence intensity of the excitation is demonstrated to be identical for the irradiation of nuclei with either…

Solid-state $^{229}$Th nuclear clocks are set to provide new opportunities for precision metrology and fundamental physics. Taking advantage of a nuclear transition's inherent low sensitivity to its environment, orders of magnitude more…

With the example of the 229Th nucleus, which is the most likely candidate for the creation frequency standard of a future, the dynamics of the interplay and the relationship of various resonance conversion mechanisms is analyzed. As a…

Nuclear Theory · Physics 2021-04-07 F. F. Karpeshin , M. B. Trzhaskovskaya

We describe a frequency stabilized diode laser at 698 nm used for high resolution spectroscopy of the 1S0-3P0 strontium clock transition. For the laser stabilization we use state-of-the-art symmetrically suspended optical cavities optimized…

Atomic Physics · Physics 2011-01-13 Marco. G. Tarallo , Nicola Poli , Marco Schioppo , Guglielmo M. Tino

In the whole landscape of atomic nuclei, $^{229}$Th is currently the only known nucleus which could allow for the development of a nuclear-based frequency standard, as it possesses an isomeric state of just 7.6 eV energy above the ground…

Instrumentation and Detectors · Physics 2017-11-01 Lars von der Wense , Benedict Seiferle , Mustapha Laatiaoui , Peter G. Thirolf

We present and characterize a laser system for the spectroscopy on highly-charged ^209Bi^82+ ions at a wavelength of 243.87 nm. For absolute frequency stabilization, the laser system is locked to a near-infra-red laser stabilized to a…

Atomic Physics · Physics 2012-09-12 S. Albrecht , S. Altenburg , C. Siegel , N. Herschbach , G. Birkl

The results of experimental studies of the low-energy isomeric state in the $^{229}$Th nucleus are presented. The work is consisted of several stages. During the first stage $^{229}$Th nuclei were excited with the inverse internal…

The exceptionally low-energy isomeric transition in $^{229}$Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large…