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We numerically analyze the use of intense entangled twin beams for ultra-sensitive spectroscopic measurements in chemical and biological systems. The examined scheme makes use of intense frequency-modulated (chirped) entangled beams to…

Quantum Physics · Physics 2018-05-16 Jiří Svozilík , Jan Peřina , Roberto de J. León-Montiel

Transient X-ray absorption techniques can measure ultrafast dynamics of the elemental edges in a material or multiple layer junction, giving them immense potential for deconvoluting concurrent processes. However, the interpretation of the…

Materials Science · Physics 2021-06-10 Hanzhe Liu , Isabel M. Klein , Jonathan M. Michelsen , Scott K. Cushing

The junction of a scanning tunneling microscope (STM) operating in the tunneling regime was irradiated with femtosecond laser pulses. A photo-excited hot electron in the STM tip resonantly tunnels into an excited state of a single molecule…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Shiwei Wu , Wilson Ho

Sideband transitions are spectroscopically probed in a system consisting of a Cooper pair box strongly but non-resonantly coupled to a superconducting transmission line resonator. When the Cooper pair box is operated at the optimal charge…

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

Interaction of atoms with twisted light is the subject of intense experimental and theoretical investigation. In almost all studies, the atom is viewed as a localized probe of the twisted light field. However, as argued in this paper,…

Quantum Physics · Physics 2021-08-16 Igor P. Ivanov

Recent interest in the role of quantum mechanics in the primary events of photosynthetic energy transfer has led to a convergence of nonlinear optical spectroscopy and quantum optics on the topic of energy-transfer dynamics in…

Quantum Physics · Physics 2014-01-23 Agata M. Branczyk , Daniel B. Turner , Gregory D. Scholes

We demonstrate a dual wavelength optical frequency standard based on the dual optical transition modulation transfer spectroscopy (DOTMTS) between different quantum transitions of the rubidium D1 (795 nm) and D2 (780 nm) lines. In a single…

Optics · Physics 2024-11-05 Jie Miao , Jingming Chen , Deshui Yu , Qiaohui Yang , Duo Pan , Jingbiao Chen

We investigate the mutiphoton process between different Bloch states in an amplitude modulated optical lattice. In the experiment, we perform the modulation with more than one frequency components, which includes a high degree of freedom…

Quantum Gases · Physics 2015-04-14 Linxiao Niu , Dong Hu , Shengjie Jin , Xiangyu Dong , Xuzong Chen , Xiaoji Zhou

The transfer technique of quantum states from light to collective atomic excitations in a double $\Lambda$ type system is extended to matter waves in this paper, as a novel scheme towards making a continuous atom laser. The intensity of the…

Quantum Physics · Physics 2009-11-10 Xiong-Jun Liu , Hui Jing , Xiao-Ting Zhou , Mo-Lin Ge

The electronic structure of atomic quantum systems and their dynamical interaction with light is reflected in transition dipole matrix elements coupling the system's energy eigenstates. In this work, we measure phase shifts of the…

This is the first in a series of two papers investigating the effect of electron-phonon coupling in two-dimensional Fourier transformed electronic spectroscopy. We present a series of one- and two-dimensional nonlinear spectroscopic…

Multi-molecular excited states accompanied by an intra- and inter-molecular geometric relaxation are commonly encountered in optical and electrooptical studies and applications of organic semiconductors as, for example excimers or charge…

Materials Science · Physics 2022-11-14 Sebastian Hammer , Theresa Linderl , Kristofer Tvingstedt , Wolfgang Brütting , Jens Pflaum

We study and experimentally implement a double-slit quantum eraser in the presence of a controlled decoherence mechanism. A two-photon state, produced in a spontaneous parametric down conversion process, is prepared in a maximally entangled…

Quantum Physics · Physics 2015-05-14 F. A. Torres-Ruiz , G. Lima , A. Delgado , S. Pádua , C. Saavedra

In this paper we present a technique for the precise measurement of electric dipole allowed transitions in trapped ions. By applying a probe and a cooling laser in quick succession, the full transition can be probed without causing…

Atomic Physics · Physics 2015-06-19 Amy Gardner , Kevin Sheridan , William Groom , Nicolas Seymour-Smith , Matthias Keller

The measured multi-dimensional spectral response of different light harvesting complexes exhibits oscillatory features which suggest an underlying coherent energy transfer. However, making this inference rigorous is challenging due to the…

Quantum Physics · Physics 2019-12-06 J. Lim , C. M. Bösen , A. D. Somoza , C. P. Koch , M. B. Plenio , S. F. Huelga

In this work we present a simple method to reconstruct the complex spectral wavefunction of a biphoton, and hence gain complete information about the spectral and temporal properties of a photon pair. The technique, which relies on quantum…

Two-dimensional superconductivity has become a major frontier in condensed matter physics. It holds the key to the mechanism of high-temperature superconductors and offers an exceptional arena to stabilize emergent quantum states enabled by…

Superconductivity · Physics 2026-03-16 Qiang-Jun Cheng , Xu-Cun Ma , Qi-Kun Xue , Can-Li Song

We propose a quantum memory for a single-photon wave packet in a superposition of two different colors, i.e., two different frequency components, using the electromagnetically induced transparency technique in a double-{\Lambda} system. We…

Quantum Physics · Physics 2013-01-16 D. Viscor , V. Ahufinger , J. Mompart , A. Zavatta , G. C. La Rocca , M. Artoni

The linear polarization signals produced by scattering processes in strong resonance lines are rich in information on the magnetic and thermal structure of the chromosphere and transition region of the Sun and of other stars. A correct…

Solar and Stellar Astrophysics · Physics 2015-06-19 Luca Belluzzi , Javier Trujillo Bueno