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The search for room-temperature magnetocaloric materials for refrigeration has led to investigations of double perovskites. In particular, a puzzle has appeared in the La$_2$MnNiO$_6$, La$_2$MnCoO$_6$ and La$_2$MnFeO$_6$ family of…

Strongly Correlated Electrons · Physics 2019-03-04 C. Gauvin-Ndiaye , T. E. Baker , P. Karan , É. Massé , M. Balli , N. Brahiti , M. A. Eskandari , P. Fournier , A. -M. S. Tremblay , R. Nourafkan

We have prepared crystallographically ordered and disorder specimens of the double perovskite, Sr$_2$FeMoO$_6$ and investigated their magnetoresistance behaviour. The extent of ordering between the Fe and Mo sites in the two samples is…

Strongly Correlated Electrons · Physics 2009-10-31 D. D. Sarma , E. V. Sampathkumaran , Sugata Ray , R. Nagarajan , Subham Majumdar , Ashwani Kumar , G. Nalini , T. N. GuruRow

The synthesis and physical properties of the double perovskite (DP) compound Ba2CdReO6 with the 5d1 electronic configuration are reported. Three successive phases originating from a spin-orbit-entangled Jeff = 3/2 state, confirmed by the…

Strongly Correlated Electrons · Physics 2021-04-06 Daigorou Hirai , Zenji Hiroi

We present a powder inelastic neutron scattering study of magnetic excitations in Ba$_2$FeReO$_6$, a member of the double perovskite family of materials which exhibit half-metallic behavior and high Curie temperatures. We find clear…

Strongly Correlated Electrons · Physics 2013-06-04 K. W. Plumb , A. M. Cook , J. P. Clancy , A. I. Kolesnikov , B. C. Jeon , T. W. Noh , A. Paramekanti , Young-June Kim

We elucidate a mechanism for obtaining polar behavior in magnetic perovskites based on A-site disorder and demonstrate this mechanism by density functional calculations for the double perovskite (La,Lu)MnNiO$_6$ with Lu concentrations at…

Materials Science · Physics 2007-12-11 D. J. Singh , Chul-Hong Park

Ion-exchange treatment of Na2SnTeO6 in molten salt mixtures resulted in rosiaite (PbSb2O6)-related MnSnTeO6. Its crystal structure was refined by the Rietveld method. Of the three possible models of Sn/Te distribution, the disordered model…

We formulate the double exchange (DE) model for systems with $t_{2g}$ orbital degeneracy, relevant for hole-doped cubic vanadates. In the relevant regime of strong on-site Coulomb repulsion $U$ we solve the model using two distinct…

Strongly Correlated Electrons · Physics 2007-06-13 Krzysztof Wohlfeld

We report on the structural, magnetic, and electronic properties of two new double-perovskites synthesized under high pressure; Pb2CaOsO6 and Pb2ZnOsO6. Upon cooling below 80 K, Pb2CaOsO6 simultaneously undergoes a metal--insulator…

The double exchange model describing interactions of itinerant electrons with localized spins is usually used to explain ferromagnetism in metals. We show that for a variety of crystal lattices of different dimensionalities and for a wide…

Strongly Correlated Electrons · Physics 2017-01-18 Maria Azhar , Maxim Mostovoy

We establish the double perovskite Ba$_2$CeIrO$_6$ as a nearly ideal model system for j=1/2 moments, with resonant inelastic x-ray scattering indicating a deviation of less than 1% from the ideally cubic j=1/2 state. The local j=1/2 moments…

The electronic and magnetic structure, including the Heisenberg model exchange interaction parameters, was explored for the recently proposed novel cuprate Cu$_2$F$_5$. Using the DFT+U calculation, it is shown that the compound is formed by…

Strongly Correlated Electrons · Physics 2021-08-11 Dmitry M. Korotin , Dmitry Y. Novoselov , Vladimir I. Anisimov , Artem R. Oganov

I study the one-dimensional spin-1 Blume-Emery-Griffiths model with bilinear and biquadratic exchange interactions and single-ion crystal field under an applied magnetic field. This model can be exactly mapped into a tight-binding Hubbard…

Statistical Mechanics · Physics 2010-03-30 F. P. Mancini

We report structural, magnetic, and Raman studies of the disordered double perovskite GdSrCoMnO$_{6}$~(GSCM). DC magnetization shows a ferromagnetic transition at $T_{C} \approx 153$~K. The inverse susceptibility exhibits a downturn above…

First principles electronic structure calculations have been carried out on ordered double perovskites Sr_2B'B"O_6 (for B' = Cr or Fe and B" 4d and 5d transition metal elements) with increasing number of valence electrons at the B-sites,…

Materials Science · Physics 2009-11-13 T. K. Mandal , C. Felser , M. Greenblatt , J. Kubler

Ordered double perovskite oxides of the general formula, A2BB'O6, have been known for several decades to have interesting electronic and magnetic properties. However, a recent report of a spectacular negative magnetoresistance effect in a…

Strongly Correlated Electrons · Physics 2015-06-24 D. D. Sarma

In this study, the magnetic ground state of iridium perovskites (Sr$_{n+1}$Ir$_{n}$O$_{3n+1}$, where $n=1$, 2, and $\infty$) was considered using muon spin spectroscopy ($\mu$SR). When probed by muons in Sr$_2$IrO$_4$ and Sr$_3$Ir$_2$O$_7$…

Strongly Correlated Electrons · Physics 2015-04-13 M. Miyazaki , R. Kadono , M. Hiraishi , A. Koda , K. M. Kojima , K. Ohashi , T. Takayama , H. Takagi

We present the discovery and refinement by neutron powder diffraction of a new magnetic phase in the Na1-xCaxMn7O12 quadruple perovskite phase diagram, which is the incommensurate analogue of the well-known pseudo-CE phase of the simple…

Strongly Correlated Electrons · Physics 2018-08-01 R. D. Johnson , F. Mezzadri , P. Manuel , D. D. Khalyavin , E. Gilioli , P. G. Radaelli

Resonant inelastic X-ray scattering measurements reveal robust magnetic excitations in the perovskite iridates SrIr$_{1-x}$Sn$_x$O$_3$. We analyzed the dispersions of the magnetic excitation with spin-dilution ratio $x$ = 0, 0.03, 0.06,…

Strongly Correlated Electrons · Physics 2026-04-14 Xiang Li , Yifan Jiang , Yuan Wan , Xuerong Liu

We propose a scheme for constructing classical spin Hamiltonians from Hunds coupled spin-fermion models in the limit J_H/t \to \infinity. The strong coupling between fermions and the core spins requires self-consistent calculation of the…

Strongly Correlated Electrons · Physics 2009-11-10 Sanjeev Kumar , Pinaki Majumdar

The scaling of magnetic memory into nanometer size calls for a theoretical model to accurately predict the switching current. Previous models show large discrepancy with experiments in studying the spin-orbit torque switching of…

Mesoscale and Nanoscale Physics · Physics 2024-08-27 Xue Zhang , Zhengde Xu , Zhifeng Zhu