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The Leibler weak segregation theory in molten diblock copolymers is generalized with due regard for the 2nd shell harmonics contributions defined in the paper and the phase diagrams are built for the linear and miktoarm ternary ABC triblock…

Soft Condensed Matter · Physics 2009-11-11 Igor Ya. Erukhimovich

In this paper we study a new model for patterns in two dimensions, inspired by diblock copolymer melts with a dominant phase. The model is simple enough to be amenable not only to numerics but also to analysis, yet sophisticated enough to…

Analysis of PDEs · Mathematics 2013-12-06 D. P. Bourne , M. A. Peletier , S. M. Roper

A general theory has been developed for a polydisperse semi-flexible multi-block copolymer melt. Using the Bawendi-Freed approach to model semi-flexible chains an expression for the Landau free energy is derived in the weak segregation…

Soft Condensed Matter · Physics 2023-03-22 P. M. Jager , W. J. Briels , J. J. M. Slot

We study morphologies of thin-film diblock copolymers between two flat and parallel walls. The study is restricted to the weak segregation regime below the order-disorder transition temperature. The deviation from perfect lamellar shape is…

Soft Condensed Matter · Physics 2009-11-07 Yoav Tsori , David Andelman

A concentrated suspension of lamellar colloidal particles (e. g. clay) is modelled by considering a single, uniformly charged, finite platelet confined with co- and counterions to a Wigner-Seitz (WS) cell. The system is treated within…

Soft Condensed Matter · Physics 2009-10-30 Emmanuel Trizac , Jean-Pierre Hansen

We analyze the energetics of sphere-like micellar phases in diblock copolymers in terms of well-studied, geometric quantities for their lattices. We argue that the A15 lattice with Pm3n symmetry should be favored as the blocks become more…

Soft Condensed Matter · Physics 2007-05-23 G. M. Grason , B. A. DiDonna , R. D. Kamien

We discuss symmetry breaking in two-dimensional quantum dots resulting from strong interelectron repulsion relative to the zero-point kinetic energy associated with the confining potential. Such symmetry breaking leads to the emergence of…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Constantine Yannouleas , Uzi Landman

In this paper, we analyze the effect of geometrical constraint on the conformational properties of an infinitely long linear semiflexible polymer chain confined in-between two constraints under good solvent condition in two dimensions. The…

Soft Condensed Matter · Physics 2020-12-29 Pramod Kumar Mishra

We compute phase diagrams for $A_nB_m$ starblock copolymers in the strong-segregation regime as a function of volume fraction $\phi$, including bicontinuous phases related to minimal surfaces (G, D, and P surfaces) as candidate structures.…

Soft Condensed Matter · Physics 2009-10-31 Peter D. Olmsted , Scott T. Milner

Surface segregation of the low-molecular weight component in a polymeric mixture leads to degradation of industrial formulations. We report a simultaneous phase separation and surface migration phenomena in oligomer-polymer and oligomer-gel…

Soft Condensed Matter · Physics 2019-07-10 Biswaroop Mukherjee , Buddhapriya Chakrabarti

We present a novel computational implementation of strong segregation theory, developed specifically for calculations of phase separated ABC star terpolymers. The method allows calculation of free energies of common two-dimensional…

Soft Condensed Matter · Physics 2026-05-21 Merin Joseph , Daniel J. Read , Alastair M. Rucklidge

At very low density, the electrons in a uniform electron gas spontaneously break symmetry and form a crystalline lattice called a Wigner crystal. But which type of crystal will the electrons form? We report a numerical study of the density…

We study the phase behavior of diblock copolymers in presence of an external electric field. We employ self-consistent field theory and treat the relevant Maxwell equation as an additional self-consistent equation. Because we do not treat…

Soft Condensed Matter · Physics 2008-06-23 Chin-Yet Lin , Michael Schick , David Andelman

An infinite system of nonlocal, individually confining solitons is considered as a model of high-density nuclear matter. The soliton-lattice problem is discussed in the Wigner-Seitz approximation. The cell size is varied to study the…

Nuclear Theory · Physics 2008-11-26 Charles W. Johnson , George Fai

Twisted bilayers of two-dimensional (2D) materials have emerged as a highly tunable platform to study and engineer properties of excitons. However, the atomistic description of these properties has remained a significant challenge as a…

Materials Science · Physics 2025-03-13 Indrajit Maity , Arash A. Mostofi , Johannes Lischner

We analyze equilibrium properties and adsorption desorption phase transition behaviour of a linear semiflexible copolymer chain under constrained geometrical situation on square lattice in a good solvent. One dimensional stair shaped line…

Statistical Mechanics · Physics 2010-06-04 Pramod Kumar Mishra

We present several ordering mechanisms in diblock copolymers. For temperatures above the order-disorder temperature and in the weak segregation regime, a linear response theory is presented which gives the polymer density in the vicinity of…

Soft Condensed Matter · Physics 2007-05-23 Yoav Tsori , David Andelman

We extensively study the phase diagram of a diblock copolymer melt confined in a cylindrical nanopore using real-space self-consistent mean-field theory. We discover a rich variety of new two-dimensional equilibrium structures that have no…

Soft Condensed Matter · Physics 2009-11-11 Weihua Li , Robert A. Wickham

We study structural properties of a ring polymeric melt confined in a film in comparison to a linear counterpart using molecular dynamics simulations. Local structure orderings of ring and linear polymers in the vicinity of the surface are…

Soft Condensed Matter · Physics 2015-10-21 Eunsang Lee , YounJoon Jung

We have generalized the Edwards' method of collective description of dense polymer systems in terms of effective potentials to polymer blends in the presence of a surface. With this method we have studied conformationally asymmetric…

Soft Condensed Matter · Physics 2009-11-11 Semjon Stepanow , Andrei A. Fedorenko
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