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The electronic ground state of Ca3LiOsO6 was recently considered within an intermediate coupling regime that revealed J=3/2 spin-orbit entangled magnetic moments. Through inelastic neutron scattering and density functional theory we…

Strongly Correlated Electrons · Physics 2017-11-29 S. Calder , D. J. Singh , V. O. Garlea , M. D. Lumsden , Y. G. Shi , K. Yamaura , A. D. Christianson

A quantum spin liquid (QSL) is a state of matter characterized by fractionalized quasiparticle excitations, quantum entanglement, and a lack of long-range magnetic order. However, QSLs have evaded definitive experimental observation.…

Strongly Correlated Electrons · Physics 2024-12-31 Sangyun Lee , Andrew J. Woods , Minseong Lee , Shengzhi Zhang , Eun Sang Choi , A. O. Scheie , D. A. Tennant , J. Xing , A. S. Sefat , R. Movshovich

A large part of the interest in magnets with frustrated antiferromagnetic interactions comes from the many new phases found in applied magnetic field. In this Article, we explore some of the new phases which arise in a model with frustrated…

Strongly Correlated Electrons · Physics 2016-02-29 Luis Seabra , Philippe Sindzingre , Tsutomu Momoi , Nic Shannon

Rare-earth triangular-lattice magnets serve as an excellent platform for investigating exotic quantum magnetic phenomena. Recently, the hexaaluminate \cmao\ has been proposed to host a $U(1)$ Dirac quantum spin liquid state with dominant…

Strongly Correlated Electrons · Physics 2025-07-16 Yantao Cao , Huanpeng Bu , Toni Shiroka , Helen C. Walker , Zhendong Fu , Zhaoming Tian , Jinkui Zhao , Hanjie Guo

Using powder neutron diffraction we have discovered an unusual magnetic order-order transition in the Ising spin chain compound Ca3Co2O6. On lowering the temperature an antiferromagnetic phase with propagation vector k=(0.5,-0.5,1) emerges…

Strongly Correlated Electrons · Physics 2011-05-17 S. Agrestini , C. L. Fleck , L. C. Chapon , C. Mazzoli , A. Bombardi , M. R. Lees , O. A. Petrenko

We study a model which could explain some of the unusual magnetic properties observed for the one-dimensional helical spin system Co(hfac)_2 NITPhOMe. One of the properties observed is that the magnetization shows plateaus near zero and…

Statistical Mechanics · Physics 2009-11-10 V. Ravi Chandra , S. Ramasesha , Diptiman Sen

A cluster Monte Carlo method for systems of classical spins with purely dipolar couplings is presented. It is tested and applied for finite arrays of perpendicular Ising dipoles on the triangular lattice. This model is a modification with…

Statistical Mechanics · Physics 2009-11-07 Ulrich K. Roessler

The results of ac and dc magnetization and heat capacity measurements as a function of temperature (T = 1.8 to 300 K) are reported for a quasi-one-dimensional compound, Ca$_3$CuMnO$_6$, crystallizing in a triclinically distorted…

Strongly Correlated Electrons · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , K. K. Iyer , E. V. Sampathkumaran

The dielectric behavior of the single crystals of the spin-chain system Ca3Co2O6, undergoing geometrically frustrated antiferromagnetic ordering below 25 K, has been investigated as a function of temperature and magnetic field (H) and…

Materials Science · Physics 2016-03-17 Tathamay Basu , Kartik K. Iyer , P. L. Paulose , E. V. Sampathkumaran

We present thermodynamic phase diagrams showing magnetic analog of "three states of matter," namely, spin liquid, paramagnetic, and magnetically ordered phases, obtained by unbiased quantum Monte Carlo simulations. Our simulations are…

Strongly Correlated Electrons · Physics 2015-09-30 Yoshitomo Kamiya , Yasuyuki Kato , Joji Nasu , Yukitoshi Motome

We investigate the spin-induced polarization in the multiferroic compound Ba2CuGe2O7 using variarional and finite temperature mean field approaches. The compound is described by a spin-3/2 Heisenberg model extended with easy plane…

Strongly Correlated Electrons · Physics 2012-02-21 Judit Romhanyi , Miklos Lajko , Karlo Penc

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

Fluctuation dynamics in magnetization plateaux are a relatively poorly explored area in frustrated magnetism. Here we use muon spin relaxation to determine the fluctuation timescale and associated field distribution width in the partial…

Strongly Correlated Electrons · Physics 2015-05-28 P. J. Baker , J. S. Lord , D. Prabhakaran

Heat-capacity (C) and ac susceptibility measurements have been performed on the spin-chain compounds, Sr3ZnRhO6 and Ca3NiMnO6, to establish their magnetic behavior and to explore whether there are magnetic frustration effects due to…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran , Y. Matsushita

Low-temperature ($T$) thermodynamic properties in magnetic fields ($B$) of the quasi-Kagome antiferromagnet CePdAl ($T_{\rm N}\sim$ 2.7 K) were studied by means of magnetization and specific-heat $C(T,B)$ measurements. The unusual magnetic…

The subtle interplay between competing degrees of freedom, crystal electric fields, and spin correlations can lead to exotic quantum states in 4f ion-based frustrated triangular lattice antiferromagnets. We present the crystal structure,…

Strongly Correlated Electrons · Physics 2026-03-17 M. Barik , J. Khatua , Suyoung Kim , Eundeok Mun , Suheon Lee , Bassam Hitti , Gerald D. Morris , Kwang-Yong Choi , P. Khuntia

We study magnetic properties of the $S=1/2$ Ising-like XXZ model on the Shastry-Sutherland lattices with long-range interactions, using the quantum Monte Carlo method. This model shows magnetization plateau phases at one-half and one-third…

Strongly Correlated Electrons · Physics 2015-05-14 Takahumi Suzuki , Yusuke Tomita , Naoki Kawashima

Using inelastic neutron scattering, we have observed a quasi-one-dimensional dispersive magnetic excitation in the frustrated triangular-lattice spin-2 chain oxide Ca3Co2O6. At the lowest temperature (T = 1.5 K), this magnon is…

Strongly Correlated Electrons · Physics 2013-12-17 Anil Jain , P. Y. Portnichenko , Hoyoung Jang , G. Jackeli , G. Friemel , A. Ivanov , A. Piovano , S. M. Yusuf , B. Keimer , D. S. Inosov

The low temperature magnetization process of antiferromagnetic spin-S chains doped with mobile spin-(S-1/2) carriers is studied in an exactly solvable model. For sufficiently high magnetic fields the system is in a metallic phase with a…

Strongly Correlated Electrons · Physics 2009-10-31 Holger Frahm , Constantin Sobiella

Ag2CrO2 is an S=3/2 frustrated triangular lattice antiferromagnet without orbital degree of freedom. With decreasing temperature, a 4-sublatice spin state develops. However, a long-range partially disordered state with 5 sublattices…

Strongly Correlated Electrons · Physics 2012-04-13 M. Matsuda , H. Yoshida , M. Isobe , C. de la Cruz , R. S. Fishman