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We employ ultrafast pump-probe spectroscopy to directly monitor electron tunneling between discrete orbital states in a pair of spatially separated quantum dots. Immediately after excitation, several peaks are observed in the pump-probe…

The prospect of coherent dynamics and excitonic delocalization across several light-harvesting structures in photosynthetic membranes is of considerable interest, but challenging to explore experimentally. Here we demonstrate theoretically…

We provide an intuitive platform for engineering exciton transfer dynamics. We show that careful consideration of the spectral density, which describes the system-bath interaction, leads to opportunities to engineer the transfer of an…

Quantum Physics · Physics 2015-05-18 Alejandro Perdomo , Leslie Vogt , Ali Najmaie , Alán Aspuru-Guzik

Periodic driving of quantum dots is analyzed as a basis for developing dynamic switching devices. We study transport through periodically modulated energy levels which are coupled to leads via tunneling coefficients. Utilizing Floquet…

Mesoscale and Nanoscale Physics · Physics 2025-09-10 Jan Mathis Giesen , Daniel Weber , Sebastian Eggert

We investigate the optical response of quantum dot molecules coherently driven by polarized laser light. Our description includes the splitting in excitonic levels caused by isotropic and anisotropic exchange interactions. We consider…

Mesoscale and Nanoscale Physics · Physics 2016-11-25 H. S. Borges , A. M. Alcalde , Sergio E. Ulloa

We provide physically intuitive mechanisms for the effect of noise on excitation energy transfer (EET) in networks. Using these mechanisms of dephasing-assisted transport (DAT) in a hybrid basis of both excitons and sites, we develop a…

Quantum Physics · Physics 2015-05-14 Alex W. Chin , Animesh Datta , Filippo Caruso , Susana F. Huelga , Martin B. Plenio

The high density of evanescent modes in the vicinity of a metal leads to enhancement of the near-field F\"{o}rster resonant energy transfer (FRET) rate. We present a classical approach to calculate the FRET rate based on the dyadic Green's…

Mesoscale and Nanoscale Physics · Physics 2016-03-01 Amrit Poudel , Xin Chen , Mark A. Ratner

Conformational dynamics of biomolecules are of fundamental importance for their function. Single-molecule F\"orster Resonance Energy Transfer (smFRET) is a powerful approach to inform on the structure and the dynamics of labeled molecules.…

Excited-state charge-transfer complexes (exciplexes) have been actively exploited in organic optoelectronic devices to improve performance; however, diffusion of exciplexes has not been actively studied despite its influence on performance…

Materials Science · Physics 2019-06-25 Hwang-Beom Kim , Jang-Joo Kim

We propose a coherent control scheme based on the optical Stark effect in optically generated excitons in quantum dot molecules (QDMs). We show that, by the combined action of voltage bias detuning sweeps and Rosen-Zener pulsed…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 J. E. Rolon , J. E. Drut

We theoretically investigate the Stark shift of the exciton goundstate in two vertically coupled quantum dots as a function of the interdot distance. The coupling is shown to enhance the tuneability of the linear optical properties,…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 F. Troiani , E. Molinari

F\"orster theory describes electronic exciton energy migration in molecular assemblies as an incoherent hopping process between donor and acceptor molecules. The rate is expressed in terms of the overlap integral between donor fluorescence…

Chemical Physics · Physics 2018-10-17 Marco Schröter , Tõnu Pullerits , Oliver Kühn

Interfacial adhesion is caused by intermolecular forces that only occur between surfaces at nano-scale contact (NSC) i.e., 0.1-0.4nm. To evaluate NSC and its influence on adhesion, F\"orster resonance energy transfer (FRET) spectroscopy has…

Materials Science · Physics 2023-01-27 Mónica Gaspar Simões , Robert Schennach , Ulrich Hirn

We explore the coherent transfer of electronic signatures from a strongly correlated, optically gated nanoscale quantum dot to a weakly interacting, electrically backgated microscale channel. In this unique side-coupled `T' geometry for…

Mesoscale and Nanoscale Physics · Physics 2010-08-31 Smitha Vasudevan , Kamil Walczak , Avik W. Ghosh

The signature of coherent coupling between two quantum states is an anticrossing in their energies as one is swept through the other. In single semiconductor quantum dots containing an electron-hole pair the eigenstates form a two-level…

Motivated by the ongoing debate about nanophotonic control of Foerster resonance energy transfer (FRET), notably by the local density of optical states (LDOS), we study an analytic model system wherein a pair of ideal dipole emitters -…

Optics · Physics 2016-05-30 Martijn Wubs , Willem L. Vos

We present magneto-optical studies of a self-assembled semiconductor quantum dot in neutral and positively charged states. The diamagnetic shifts and Zeeman splitting of many well-identified optical transitions are precisely measured.…

Mesoscale and Nanoscale Physics · Physics 2025-03-19 Giora Peniakov , Ayal Beck , Eilon Poem , Zu-En Su , Boaz Taitler , Sven Hoefling , Garnett. W. Bryant , David Gershoni

We optically probe the spectrum of ground and excited state transitions of an individual, electrically tunable self-assembled quantum dot molecule. Photocurrent absorption measurements show that the spatially direct neutral exciton…

Mesoscale and Nanoscale Physics · Physics 2011-11-15 K. Müller , G. Reithmaier , E. C. Clark , V. Jovanov , M. Bichler , H. J. Krenner , M. Betz , G. Abstreiter , J. J. Finley

We study the coherent light-matter interactions of GaAs quantum wells associated with excitons, biexcitons and many-body effects. For most polarization configurations, excitonic features dominate the phase-resolved two-dimensional…

Other Condensed Matter · Physics 2011-12-13 Alan D. Bristow , Denis Karaiskaj , Xingcan Dai , Richard. P. Mirin , Steven T. Cundiff

Experimental evidence of strong coupling between excitons confined in a quantum well and the photonic modes of a two-dimensional dielectric lattice is reported. Both resonant scattering and photoluminescence spectra at low temperature show…