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Many processes in chemistry, physics, and biology involve rare events in which the system escapes from a metastable state by surmounting an activation barrier. Examples range from chemical reactions, protein folding, and nucleation events…

Chemical Physics · Physics 2020-10-07 Niels Zijlstra , Daniel Nettels , Rohit Satija , Dmitrii E. Makarov , Benjamin Schuler

We present experiments in which an ultra-cold sample of ammonia molecules is released from an electrostatic trap and recaptured after a variable time. It is shown that, by performing adiabatic cooling before releasing the molecules and…

Chemical Physics · Physics 2015-06-19 Marina Quintero-Pérez , Thomas E. Wall , Steven Hoekstra , Hendrick L. Bethlem

In the real-time manipulation of quantum states, it is necessary to dynamically control the parameters of the system's Hamiltonian. We have studied the survival probability during the conveyance of a particle by a trapping potential, where…

Quantum Physics · Physics 2026-02-19 Yoshiaki Teranishi , Satoshi Morita , Seiji Miyashita

In a quantum system with a smoothly and slowly varying Hamiltonian, which approaches a constant operator at times $t\to \pm \infty$, the transition probabilities between adiabatic states are exponentially small. They are characterized by an…

Quantum Physics · Physics 2009-10-31 Michael Wilkinson , Michael A. Morgan

We report the measurement of one-body loss rates for magnetically trapped metastable europium atoms and the study of their loss mechanism. The loss of atoms observed in a magneto-optical trap is not fully understood because of the…

Atomic Physics · Physics 2021-09-22 Hiroki Matsui , Yuki Miyazawa , Ryotaro Inoue , Mikio Kozuma

We examine time-resolved X-ray diffraction from molecules in the gas phase which undergo nonadiabatic avoided-crossing dynamics involving strongly coupled electrons and nuclei. Several contributions to the signal are identified,…

Chemical Physics · Physics 2017-05-30 Markus Kowalewski , Kochise Bennett , Shaul Mukamel

We study nonadiabatic electron transfer within the biased spin-boson model. We calculate the incoherent transfer rate in analytic form at all temperatures for a power law form of the spectral density of the solvent coupling. In the Ohmic…

Statistical Mechanics · Physics 2009-10-31 G. Lang , E. Paladino , U. Weiss

We explore nonadiabatic quantum phase transitions in an Ising spin chain with a linearly time-dependent transverse field and two different spins per unit cell. Such a spin system passes through critical points with gapless excitations,…

Statistical Mechanics · Physics 2021-02-23 Bin Yan , Vladimir Y. Chernyak , Wojciech H. Zurek , Nikolai A. Sinitsyn

In this article, for the first time in the context of TOP trap, the necessary and sufficient conditions for the adiabatic evolution of weak field seeking states have been quantitatively examined. It has been well accepted since decades that…

Quantum Physics · Physics 2017-11-10 Nirupam Dutta , Anirban Dey , Prasanta K. Panigrahi

We present a versatile electric trap for the exploration of a wide range of quantum phenomena in the interaction between polar molecules. The trap combines tunable fields, homogeneous over most of the trap volume, with steep gradient fields…

Quantum Physics · Physics 2012-08-02 B. G. U. Englert , M. Mielenz , C. Sommer , J. Bayerl , M. Motsch , P. W. H. Pinkse , G. Rempe , M. Zeppenfeld

We report the magnetic trapping of metastable $^3P_2$ atomic strontium. Atoms are cooled in a magneto-optical trap (MOT) operating on the dipole allowed $^1S_0-^1P_1$ transition at 461 nm. Decay via $^1P_1\to {^1D_2}\to {^3P_2}$…

Atomic Physics · Physics 2009-11-07 S. B. Nagel , C. E. Simien , S. Laha , P. Gupta , V. S. Ashoka , T. C. Killian

We study the dynamic behavior of ultracold neutral atoms in a macroscopic ac electric trap. Confinement in such a trap is achieved by switching between two saddle-point configurations of the electric field. The gradual formation of a stably…

Atomic Physics · Physics 2008-04-14 Sophie Schlunk , Adela Marian , Wieland Schoellkopf , Gerard Meijer

Using a theory of polarizable fluids, we extend a variational treatment of an excess electron to the many-electron case corresponding to finite metal concentrations in metal-ammonia solutions (MAS). We evaluate dielectric, optical, and…

Statistical Mechanics · Physics 2009-11-13 Gennady N. Chuev , Pascal Quemerais , Jason Crain

The problem of escape of a Brownian particle in a cusp-shaped metastable potential is of special importance in nonadiabatic and weakly-adiabatic rate theory for electron transfer (ET) reactions. Especially, for the weakly-adiabatic…

Statistical Mechanics · Physics 2009-11-07 Bartlomiej Dybiec , Ewa Gudowska-Nowak , Pawel F. Gora

In radiation damage cascade displacement spikes ions and electrons can reach very high temperatures and be out of thermal equilibrium. Correct modelling of cascades with molecular dynamics should allow for the non-adiabatic exchange of…

Materials Science · Physics 2015-10-29 Daniel Mason

Atoms confined in a magnetic trap can escape by making spin-flip Majorana transitions due to a breakdown of the adiabatic approximation. Several papers have studied this process for atoms with spin $F = 1/2$ or $F= 1$. The present paper…

Quantum Physics · Physics 2009-11-13 D. M. Brink , C. V. Sukumar

In a Stark decelerator, polar molecules are slowed down and focussed by an inhomogeneous electric field which switches between two configurations. For the decelerator to work, it is essential that the molecules follow the changing electric…

Atomic Physics · Physics 2015-05-18 T. E. Wall , S. K. Tokunaga , E. A. Hinds , M. R. Tarbutt

A Lagrangian formalism is developed for a general nondissipative quasiperiodic nonlinear wave with trapped particles in collisionless plasma. The adiabatic time-averaged Lagrangian density $\mcc{L}$ is expressed in terms of the…

Plasma Physics · Physics 2015-05-28 I. Y. Dodin , N. J. Fisch

We study, experimentally and theoretically, the controlled transfer of harmonically trapped ultracold gases between different quantum states. In particular we experimentally demonstrate a fast decompression and displacement of both a…

Quantum Gases · Physics 2015-05-28 Jean-François Schaff , Pablo Capuzzi , Guillaume Labeyrie , Patrizia Vignolo

A central issue in the quest to understand the superconductivity in cuprates is the nature and origin of the pseudogap state, which harbours anomalous electronic states such as Fermi arc, charge density wave (CDW), and $d$-wave…