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The multilayer multiconfiguration time-dependent Hartree theory within second quantization representation of the Fock space is applied to study correlated electron transport in models of single-molecule junctions. Extending previous work,…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Haobin Wang , Michael Thoss

A finite temperature many-particle theory of condensed matter systems is formulated using the functional Schroedinger picture. Using the interacting electron gas as a model system, we solve the equation of motion for the density matrix…

Strongly Correlated Electrons · Physics 2008-02-03 Hyun Sik Noh , Sang Koo You , Chul Koo Kim

The multilayer multiconfiguration time-dependent Hartree method is employed to study vibrationally coupled charge transport in models of single molecule junctions. To increase the efficiency of the simulation method, a representation of the…

Mesoscale and Nanoscale Physics · Physics 2013-02-12 Haobin Wang , Michael Thoss

A density-matrix formalism is developed based on the one-particle density-matrix of a single-determinantal reference-state. The v-representable problem does not appear in the proposed method, nor the need to introduce functionals defined by…

Chemical Physics · Physics 2009-11-10 James P. Finley

Free classical particles have well-defined momentum and position, while free quantum particles have well-defined momentum but a position fully delocalized over the sample volume. We develop a many-body formalism based on wave-packet…

Quantum Physics · Physics 2017-11-07 Aurélia Chenu , Monique Combescot

Conceiving a molecule as composed of smaller molecular fragments, or subunits, is one of the pillars of the chemical and physical sciences, and leads to productive methods in quantum chemistry. Using a fragmentation scheme, efficient…

Chemical Physics · Physics 2015-04-14 Martín A. Mosquera , Adam Wasserman

A time-dependent current-density-functional theory for many-particle systems in interaction with arbitrary external baths is developed. We prove that, given the initial quantum state $|\Psi_0>$ and the particle-bath interaction operator,…

Mesoscale and Nanoscale Physics · Physics 2007-06-13 Massimiliano Di Ventra , Roberto D'Agosta

The theoretical framework for higher-order correlation functions involving multiple times and multiple points in a classical, many-body system developed by Van Zon and Schofield [Phys. Rev. E 65, 011106 (2002)] is extended here to include…

Statistical Mechanics · Physics 2007-05-23 Ramses van Zon , Jeremy Schofield

Many-body localization for a system of bosons trapped in a one dimensional lattice is discussed. Two models that may be realized for cold atoms in optical lattices are considered. The model with a random on-site potential is compared with…

Disordered Systems and Neural Networks · Physics 2018-04-24 Piotr Sierant , Jakub Zakrzewski

We describe the time-dependent restricted-active-space self-consistent-field (TD-RASSCF) method for a system of interacting bosons. We provide the theory of the method and discuss its numerical implementation. The method provides a general…

Quantum Physics · Physics 2017-04-28 Camille Lévêque , Lars Bojer Madsen

The nuclear time-dependent density functional theory (TDDFT) is a tool of choice for describing various dynamical phenomena in atomic nuclei. In a recent study, we reported an extension of the framework - the multiconfigurational TDDFT…

Nuclear Theory · Physics 2024-01-24 Petar Marević , David Regnier , Denis Lacroix

A unified view on linear response of interacting systems utilizing multicongurational time-dependent Hartree methods is presented. The cases of one-particle and two-particle response operators for identical particles and up to all-system…

Quantum Physics · Physics 2014-10-20 Ofir E. Alon , Alexej I. Streltsov , Lorenz S. Cederbaum

We present a method to calculate many-body states of interacting carriers in million atom quantum nanostructures based on atomistic tight-binding calculations and a combination of iterative selection of configurations and perturbation…

Mesoscale and Nanoscale Physics · Physics 2020-05-27 Moritz Cygorek , Matthew Otten , Marek Korkusinski , Pawel Hawrylak

A finite-temperature many-body perturbation theory is presented that expands in power series the electronic grand potential, chemical potential, internal energy, and entropy on an equal footing. Sum-over-states and sum-over-orbitals…

Chemical Physics · Physics 2020-07-15 So Hirata , Punit K. Jha

Here we present a many-body theory based on a solution of the $N$-representability problem in which the ground-state two-particle reduced density matrix (2-RDM) is determined directly without the many-particle wave function. We derive an…

Quantum Physics · Physics 2023-04-19 David A. Mazziotti

A theory of temperature dynamics in many-body systems driven by time-dependent external sources is introduced. The formalism based on the combination of the perturbation theory and the fluctuational-electrodynamics approach in many-body…

Mesoscale and Nanoscale Physics · Physics 2021-07-14 Alireza Naeimi , Moladad Nikbakht

In the author's previous works, it is derived from the Dirac equation that particles can have negative kinetic energy (NKE) solutions, and they should be treated on an equal footing as the positive kinetic energy (PKE) solutions. More than…

General Physics · Physics 2023-07-24 Huai-Yu Wang

The widely used thermal Hartree-Fock (HF) theory is generalized to include the effect of electron correlation while maintaining its quasi-independent-particle framework. An electron-correlated internal energy (or grand potential) is…

Statistical Mechanics · Physics 2024-08-22 So Hirata

A comprehensive and detailed account is presented for the finite-temperature many-body perturbation theory for electrons that expands in power series all thermodynamic functions on an equal footing. Algebraic recursions in the style of the…

Statistical Mechanics · Physics 2021-09-21 So Hirata

The lecture notes on "Many-body Quantum Dynamics with MCTDH-X," adapted from the 2023 Heidelberg MCTDH Summer School, provide an in-depth exploration of the Multiconfigurational Time-Dependent Hartree approach for indistinguishable…

Quantum Physics · Physics 2025-04-01 Paolo Molignini , Sunayana Dutta , Elke Fasshauer