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Phase transitions significantly differ between two-dimensional and three-dimensional systems, but the influence of dimensionality on the glass transition is unresolved. We use microscopy to study colloidal systems as they approach their…

Soft Condensed Matter · Physics 2017-05-26 Skanda Vivek , Colm P. Kelleher , Paul M. Chaikin , Eric R. Weeks

We construct a framework for the study of fluctuations in the nonequilibrium relaxation of glassy systems with and without quenched disorder. We study two types of two-time local correlators with the aim of characterizing the heterogeneous…

Molecular-dynamics simulations are presented for two correlation functions formed with the partial density fluctuations of binary hard-sphere mixtures in order to explore the effects of mixing on the evolution of glassy dynamics upon…

Soft Condensed Matter · Physics 2007-05-23 G. Foffi , W. Gotze , F. Sciortino , P. Tartaglia , Th. Voigtmann

We present a quantitative theory for a relaxation function in a simple glass-forming model (binary mixture of particles with different interaction parameters). It is shown that the slowing down is caused by the competition between locally…

Materials Science · Physics 2009-11-13 Edan Lerner , Itamar Procaccia

We analyse numerically thermal fluctuations of the static overlap between equilibrium configurations in a glass-forming liquid approaching the glass transition. We find that the emergence of slow dynamics near the onset temperature…

Statistical Mechanics · Physics 2013-08-23 Ludovic Berthier

Dynamical four-point susceptibilities measure the extent of spatial correlations in the dynamics of glass forming systems. We show how these susceptibilities depend on the length scales that necessarily form part of their definition. The…

Statistical Mechanics · Physics 2007-05-23 David Chandler , Juan P. Garrahan , Robert L. Jack , Lutz Maibaum , Albert C. Pan

Generic glass formers exhibit at least two characteristic changes in their relaxation behavior, first to an Arrhenius-type relaxation at some characteristic temperature, and then at a lower characteristic temperature to a super-Arrhenius…

Disordered Systems and Neural Networks · Physics 2012-03-08 H. George E. Hentschel , Smarajit Karmakar , Itamar Procaccia , Jacques Zylberg

The emergence of nanoscience has increased the importance of experiments able to probe the very local structure of materials, especially for disordered and heterogeneous systems. This is technologically important; for example, the nanoscale…

Soft Condensed Matter · Physics 2015-05-13 R. Casalini , C. M. Roland

We show by means of a Monte Carlo simulation study that three-dimensional models with long-range frustration display the generic phenomena seen in fragile glassforming liquids. Due to their properties (absence of quenched disorder, physical…

Statistical Mechanics · Physics 2009-11-07 M. Grousson , G. Tarjus , P. Viot

Molecular dynamics simulations are performed to investigate heterogeneous dynamics in amorphous glassy materials under oscillatory shear strain. We consider three-dimensional binary Lennard-Jones mixture well below the glass transition…

Soft Condensed Matter · Physics 2013-05-10 Nikolai V. Priezjev

Glassy behavior is a generic feature of electrons close to disorder-driven metal-insulator transitions. Deep in the insulating phase, electrons are tightly bound to impurities, and thus classical models for electron glasses have long been…

Strongly Correlated Electrons · Physics 2009-11-10 V. Dobrosavljevic

Local stresses and pressures always exist in glasses. In this letter we consider their effects on the structure and structural correlations in simple glasses. We find that extreme values of local pressures are related to well defined local…

Condensed Matter · Physics 2016-08-31 Tamar Kustanovich , Zeev Olami

Amorphous materials have a rich relaxation spectrum, which is usually described in terms of a hierarchy of relaxation mechanisms. In this work, we investigate the local dynamic modulus spectra in a model glass just above the glass…

Disordered Systems and Neural Networks · Physics 2019-03-27 Baoshuang Shang , Jörg Rottler , Pengfei Guan , Jean-Louis Barrat

A discrete--dynamics model, which is specified solely in terms of the system's equilibrium structure, is defined for the density correlators of a simple fluid. This model yields results for the evolution of glassy dynamics which are…

Disordered Systems and Neural Networks · Physics 2011-08-12 T. Franosch , W. Götze , M. R. Mayr , A. P. Singh

Universal scaling laws of fluctuations (the $\Delta$-scaling laws) can be derived for equilibrium and off-equilibrium systems when combined with the finite-size scaling analysis. In any system in which the second-order critical behavior can…

High Energy Physics - Phenomenology · Physics 2009-10-31 Robert Botet , Marek Ploszajczak

Dynamical heterogeneities have been introduced in the context of the glass transition of molecular liquids and the lengthscale associated with them has been argued to be at the origin of the observed quasi-universal behaviour of glassy…

Soft Condensed Matter · Physics 2015-03-17 Olivier Dauchot , Douglas J. Durian , Martin van Hecke

We consider the stationary state of a fluid comprised of inelastic hard spheres or disks under the influence of a random, momentum-conserving external force. Starting from the microscopic description of the dynamics, we derive a nonlinear…

Statistical Mechanics · Physics 2013-02-25 W. T. Kranz , M. Sperl , A. Zippelius

We introduce a new quantity to probe the glass transition. This quantity is a linear generalized compressibility which depends solely on the positions of the particles. We have performed a molecular dynamics simulation on a glass forming…

Disordered Systems and Neural Networks · Physics 2009-11-07 Herve M. Carruzzo , Clare C. Yu

The volume fluctuations in statistical mechanics are discussed. First, the volume fluctuations in ensembles with a fixed external pressure, the so called pressure ensembles, are considered. Second, a generalization of the pressure ensembles…

Nuclear Theory · Physics 2008-11-26 Mark I. Gorenstein

Despite decades of studies on the grand problem of the glass transition the question of well-defined universal patterns, including the key problem of the previtreous behavior of the primary (structural) relaxation time, remains elusive.…

Soft Condensed Matter · Physics 2018-09-18 Aleksandra Drozd-Rzoska
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