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We examine the vitrification and melting of asymmetric star polymers mixtures by combining rheological measurements with mode coupling theory. We identify two types of glassy states, a {\it single} glass, in which the small component is…

We study the glass transition of binary mixtures of dipolar particles in two dimensions within the framework of mode-coupling theory, focusing in particular on the influence of composition changes. In a first step, we demonstrate that the…

Soft Condensed Matter · Physics 2011-02-09 David Hajnal , Martin Oettel , Rolf Schilling

We study the influence of composition changes on the glass transition of binary hard disc and hard sphere mixtures in the framework of mode coupling theory. We derive a general expression for the slope of a glass transition line. Applied to…

Soft Condensed Matter · Physics 2010-09-15 D. Hajnal , J. M. Brader , R. Schilling

We extend the replica liquid theory in order to describe the multiple glass transitions of binary mixtures with large size disparities, by taking into account the two-step replica symmetry breaking (2RSB). We determine the glass phase…

Soft Condensed Matter · Physics 2021-03-03 Harukuni Ikeda , Kunimasa Miyazaki , Hajime Yoshino , Atsushi Ikeda

We report on the results of a molecular dynamics simulation study of binodal glassy systems, formed in the process of isochoric rapid quenching from a high-temperature fluid phase. The transition to vitreous state occurs due to concurrent…

Soft Condensed Matter · Physics 2018-02-21 Maxim A. Makeev , Nikolai V. Priezjev

Within the mode-coupling theory for idealized glass transitions, we study the evolution of structural relaxation in binary mixtures of hard spheres with size ratios $\delta$ of the two components varying between 0.5 and 1.0. We find two…

Soft Condensed Matter · Physics 2009-11-07 W. Götze , Th. Voigtmann

Multiple distinct glass states occur in binary hard-sphere mixtures with constituents of very disparate sizes according to the mode-coupling theory of the glass transition (MCT), distinguished by considering whether small particles remain…

Soft Condensed Matter · Physics 2015-05-20 Th. Voigtmann

We present a theory for the dynamics of a binary mixture with particle size swaps. The theory is based on a factorization approximation similar to that employed in the mode-coupling theory of glassy dynamics. The theory shows that, in…

Soft Condensed Matter · Physics 2018-11-14 Grzegorz Szamel

Using molecular dynamics simulation we examine changeovers among crystal, glass, and liquid at high density in a two dimensional binary mixture. We change the ratio between the diameters of the two components and the temperature. The…

Soft Condensed Matter · Physics 2009-11-11 Toshiyuki Hamanaka , Akira Onuki

Extensive molecular dynamics simulations show that a short-range central potential, suited to model C60, undergoes a high temperature transition to a glassy phase characterized by the positional disorder of the constituent particles.…

Soft Condensed Matter · Physics 2007-05-23 Maria C. Abramo , Carlo Caccamo , Dino Costa , Romina Ruberto

Using molecular dynamics simulation, we investigate the slow dynamics of a supercooled binary mixture of soft particles interacting with a generalized Hertzian potential. At low density, it displays typical slow dynamics near its glass…

Soft Condensed Matter · Physics 2016-10-18 Ryoji Miyazaki , Takeshi Kawasaki , Kunimasa Miyazaki

We study by molecular dynamics computer simulation a binary soft-sphere mixture that shows a pronounced decoupling of the species' long-time dynamics. Anomalous, power-law-like diffusion of small particles arises, that can be understood as…

Statistical Mechanics · Physics 2013-05-29 Th. Voigtmann , J. Horbach

We analyze the glassy dynamics of a binary mixtures of hard disks in two dimensions. Predictions of the Mode-Coupling theory(MCT) are tested with extensive Brownian dynamics simulations. Measuring the collective particle density correlation…

Soft Condensed Matter · Physics 2011-04-27 Fabian Weysser , David Hajnal

The binary hard-sphere mixture is one of the simplest representations of a many-body system with competing time and length scales. This model is relevant to fundamentally understand both the structural and dynamical properties of materials,…

Vitrification in colloidal systems typically occurs at high densities driven by sharply varying, short-ranged interactions. The possibility of glassy behavior arising from smoothly varying, long-ranged particle interactions has received…

Disordered Systems and Neural Networks · Physics 2009-11-13 Emanuela Zaccarelli , Stefan Andreev , Francesco Sciortino , David R. Reichman

We report extensive molecular-dynamics simulation results for binary mixtures of hard spheres for different size disparities and different mixing percentages,for packing fractions up to 0.605 and over a characteristic time interval spanning…

Soft Condensed Matter · Physics 2007-05-23 G. Foffi , W. Gotze , F. Sciortino , P. Tartaglia , Th. Voigtmann

The glass transition is considered within two toys models, a mean field spin glass and a directed polymer in a correlated random potential. In the spin glass model there occurs a dynamical transition, where the system condenses in a state…

Disordered Systems and Neural Networks · Physics 2009-10-30 Th. M. Nieuwenhuizen

The dynamics of glass formation in monatomic and binary liquids are studied numerically using a microscopic field theory for the evolution of the time-averaged atomic number density. A stochastic framework combining phase field crystal free…

Materials Science · Physics 2015-05-27 Joel Berry , Martin Grant

The transition from a flowing to a static state in a granular material is studied using large-scale, 3D particle simulations. Similar to glasses, this transition is manifested in the development of a plateau in the contact normal force…

Statistical Mechanics · Physics 2007-05-23 L. E. Silbert , D. Ertas , G. S. Grest , T. C. Halsey , D. Levine

We study the equilibrium statistical properties of the potential energy landscape of several glass models in a temperature regime so far inaccessible to computer simulations. We show that unstable modes of the stationary points undergo a…

Statistical Mechanics · Physics 2019-12-11 Daniele Coslovich , Andrea Ninarello , Ludovic Berthier
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