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We report that calculating the Gibbs free energy of the alpha-Al_2O_3 (0001) surfaces in equilibrium with a realistic environment containing both oxygen and hydrogen species is essential for obtaining theoretical predictions consistent with…

Materials Science · Physics 2009-10-31 Xiao-Gang Wang , Anne Chaka , Matthias Scheffler

High-entropy alloys are widely modeled as homogeneously mixed surfaces, yet the validity of this assumption for catalytic prediction remains unclear. Here, we reproduce high-throughput experimental measurements using thermodynamic…

Materials Science · Physics 2026-04-29 Taegyeong Kim , Youngtak Kim , Sathya Sheela Subramanian , Geun Ho Gu

Ferritic steels possibly strengthened by oxide dispersion are candidates as structural materials for generation IV and fusion nuclear reactors. Their use is limited by incomplete knowledge of the iron-chromium phase diagram at low…

Materials Science · Physics 2013-03-13 Maximilien Levesque

Using density-functional theory in combination with a thermodynamic formalism we calculate the relative stability of various structural models of the polar O-terminated (000-1)-O surface of ZnO. Model surfaces with different concentrations…

Materials Science · Physics 2009-11-10 B. Meyer

In situ Electro-Chemical Scanning Tunneling Microscopy (ECSTM) and Electron Back-Scatter Diffraction analysis of the same local microstructural region were combined to study the relationships between grain boundary (GB) type and structure…

Engineering liquid metal alloys offers a transformative pathway for plasma-facing components (PFC) by enabling chemically tailored surfaces that can simultaneously optimize plasma-material interactions, reduce divertor heat flux, and…

We study the adsorption geometry of 3,4,9,10-perylene-tetracarboxylic-dianhydride (PTCDA) on Ag(111) and Cu(111) using X-ray standing waves. The element-specific analysis shows that the carbon core of the molecule adsorbs in a planar…

Materials Science · Physics 2011-04-13 A. Gerlach , S. Sellner , F. Schreiber , N. Koch , J. Zegenhagen

The CO_{2} electro-reduction reaction (CORR) is a promising avenue to convert greenhouse gases into high-value fuels and chemicals, in addition to being an attractive method for storing intermittent renewable energy. Although…

Stochastic inhomogeneous oxidation is an inherent characteristic of copper (Cu), often hindering color tuning and bandgap engineering of oxides. Coherent control of the interface between metal and metal oxide remains unresolved. We…

We propose silver-based oxides with layered perovskite structure as candidates of exhibiting intriguing feature of strongly correlated electrons. The compounds show unique covalence between Ag d and O p orbitals with the strong electron…

It has long been argued that the minimal model to describe the low-energy physics of the high-Tc superconducting cuprates must include copper states of other symmetries besides the canonical x2-y2 one, in particular the z2 orbital.…

Strongly Correlated Electrons · Physics 2011-10-12 Liviu Hozoi , Liudmila Siurakshina , Peter Fulde , Jeroen van den Brink

The self-organization of a chemi-sorbed mono-layer is studied as a two dimensional ordering process in presence of surface stress. As proved previously for a single phase separation, a steady surface state is yielded from the competition…

Materials Science · Physics 2009-11-07 Laurent Proville

Fe based alloys are commonly used in almost every sector of human life. For different reasons, the surfaces of the real parts are prepared using different methods, e.g., mirror-like polishing, grit-blasting, etc. The purpose of the present…

Materials Science · Physics 2020-11-19 Wojciech J. Nowak , Daria Serafin , Bartek Wierzba

Aluminum-copper-magnesium-sliver (Al-Cu-Mg-Ag) alloys are extensively utilized in aerospace industries due to the formation of Omega nano-plates.However, the rapid coarsening of these nano-plates above 475 K restricts their application at…

Materials Science · Physics 2025-02-26 Junyuan Bai , Hao Xue , Jiaming Li , Xueyong Pang , Zhihao Zhao , Gang Liu , Gaowu Qin

The results of X-ray photoemission (XPS) and valence bands spectroscopy, optically stimulated electron emission (OSEE) measurements and density functional theory based modeling of graphene oxide (GO) placed on Cu via an electrophoretic…

Using first-principles density functional theory in the implementation of the exact muffin-tin orbitals method and the coherent potential approximation, we studied the surface energy and the surface stress of the thermodynamically most…

Materials Science · Physics 2013-06-21 Stephan Schönecker , Se Kyun Kwon , Börje Johansson , Levente Vitos

We investigated the impact of surface oxygen on the ion yield for He$^+$ ions scattered from different single crystalline surfaces in low-energy ion scattering. Initially clean Al(111) and Ta(111) were exposed to molecular oxygen and ion…

Materials Science · Physics 2019-09-18 Barbara Bruckner , Peter Bauer , Daniel Primetzhofer

We report on experimental evidence for the formation of a two dimensional Si/Au(110) surface alloy. In this study, we have used a combination of scanning tunneling microscopy, low energy electron diffraction, Auger electron spectroscopy and…

Using two different full-potential ab-initio techniques we introduce a simple, universal rule based on the number of broken first-neighbor bonds to determine the surface energies of the three noble metals Cu, Ag and Au. When a bond is…

Condensed Matter · Physics 2009-11-07 I. Galanakis , G. Bihlmayer , V. Bellini , N. Papanikolaou , R. Zeller , S. Bluegel , P. H. Dederichs

Cleaved and polished surfaces of CaCu$_3$Ti$_4$O$_{12}$ ceramics have been investigated by x-ray photoelectron spectroscopy (XPS) and energy dispersive x-ray spectroscopy (EDX), respectively. While EDX technique shows the identical…

Materials Science · Physics 2007-08-20 C. Wang , H. J. Zhang , P. M. He , G. H. Cao