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The spin-gap system with a bond-disorder (CH3)2CHNH3-Cu(ClxBr1-x)3 is reported by experiments on macroscopic quantities of the uniform susceptibility and the specific heat to show a magnetic order at low temperatures when the value of x is…

Strongly Correlated Electrons · Physics 2009-11-13 Takayuki Goto , Takao Suzuki , Keishi Kanada , Takehiro Saito , Akira Oosawa , Isao Watanabe , Hirotaka Manaka

The ground state of the quasi-one-dimensional system with bond-disorder (CH3)2CHNH3Cu(ClxBr1-x)3 with x = 0, 0.25 and 0.3 has been investigated by muSR. The Fourier spectrum of electron spin fluctuation in x =0.25 and 0.3 obtained by…

Statistical Mechanics · Physics 2013-10-09 Takayuki Goto , Takao Suzuki , Isao Watanbe , Hirotaka Manaka , Hubertus Luetkens , Alex Amato

Muon-spin-rotation and relaxation studies have been performed on (CH$_3$)$_2$CHNH$_3$Cu(Cl$_x$Br$_{1-x}$)$_3$ with $x$=0.85 and 0.95, which are solid solutions of the two isomorphic spin-gap systems (CH$_3$)$_2$CHNH$_3$CuCl$_3$ and…

Strongly Correlated Electrons · Physics 2009-11-11 T. Saito , A. Oosawa , T. Goto , T. Suzuki , I. Watanabe

The ground state of the solid solution of the two spin gap systems (CH3)2CHNH3CuCl3 and (CH3)2CHNH3CuBr3 has been investigated by 1H-NMR. The existence of a magnetic ordering in the sample with the Cl-content x=0.85 was clearly demonstrated…

Other Condensed Matter · Physics 2009-11-11 Keishi Kanada , Takehiro Saito , Akira Oosawa , Takayuki Goto , Takao Suzuki , Hirotaka Manaka

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

Strongly Correlated Electrons · Physics 2018-04-04 Seiko Ohira-Kawamura , Keisuke Tomiyasu , Akihiro Koda , Dita P. Sari , Retno Asih , Sungwon Yoon , Isao Watanabe , Kenji Nakajima

The antiferromagnetic ordering in the solid-solution of the two spin-gap systems (CH3)2CHNH3CuCl3 and (CH3)2CHNH3CuBr3 has been investigated by 1H-NMR. The sample with the Cl-content ratio x=0.85 showed a clear splitting in spectra below…

Strongly Correlated Electrons · Physics 2009-11-13 Keishi Kanada , Takehiro Saito , Akira Oosawa , Takayuki Goto , Takao Suzuki

We report muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements on Cu(Cl,Br)La(Nb,Ta)$_{2}$O$_{7}$, which demonstrate: (a) the absence of static magnetism in (CuCl)LaNb$_{2}$O$_{7}$ down to 15 mK confirming a spin-gapped…

Muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements have been performed on the pure and diluted spin 1/2 kagom\'{e} system (Cu$_x$Zn$_{1-x}$)$_{3}$V$_{2}$O$_7$(OH)$_{2}$ 2H$_2$O. In the pure $x=1$ system we found a…

We report the signatures of dynamic spin fluctuations in the layered honeycomb Li$_3$Cu$_2$SbO$_6$ compound, with a 3$d$ S = 1/2 $d^9$ Cu$^{2+}$ configuration, through muon spin rotation and relaxation ($\mu$SR) and neutron scattering…

Cu-NMR study has been performed on the disordered spin-gap system Tl1-xKxCuCl3 In the high-field H > HC=\Delta/\mu_B, where \Delta is the spin-gap, the hyperfine field becomes extremely inhomogeneous at low temperatures due to the…

Strongly Correlated Electrons · Physics 2009-11-11 T. Fujiwara , H. Inoue , A. Oosawa , R. Tsunoda , T. Goto , T. Suzuki , Y. Shindo , H. Tanaka , T. Sasaki , N. Kobayashi , S. Awaji , K. Watanabe

We report results of a muon spin relaxation study of slow magnetic fluctuations in the pseudogap phase of underdoped single-crystalline YBa$_{2}$Cu$_{3}$O$_{y}$, $y = 6.77$ and 6.83. The dependence of the dynamic muon spin relaxation rate…

An inelastic neutron scattering study was performed on a Zn-substituted spin-1/2 Heisenberg 2-leg ladder compound Sr(Cu1-xZnx)2O3 (x < 0.04) to investigate nonmagnetic impurity effects on the quantum spin system with a large spin gap of…

Condensed Matter · Physics 2009-10-30 M. Azuma , M. Takano , R. S. Eccleston

Zero-field muon-spin-relaxation (ZF-{\boldmath $\mu$}SR) measurements were carried out down to 80 mK on the randomness bond system Tl$_{1-x}$K$_x$CuCl$_3$ with $x$ = 0.44. Time spectra are well fitted by the stretched exponential function…

Strongly Correlated Electrons · Physics 2009-11-13 Takao Suzuki , Fumiko Yamada , Isao Watanabe , Takayuki Goto , Akira Oosawa , Hidekazu Tanaka

The disordered pyrochlore oxide Dy$_{2}$Zr$_{2}$O$_{7}$ shows the signatures of field-induced spin freezing with remnant zero-point spin-ice entropy at 5 kOe magnetic field. We have performed zero-field and longitudinal field Muon spin…

Strongly Correlated Electrons · Physics 2023-03-28 Sheetal , Pabitra K. Biswas , K. Yokoyama , D. T. Adroja , C. S. Yadav

We performed nuclear magnetic resonance (NMR) and muon spin relaxation ({\mu}SR) experiments to identify the magnetic ground state of the frustrated quantum A-site spinel, CuAl2O4. Our results verify that the ground state does not exhibit a…

Zero-field muon-spin-relaxation (muSR) and magnetic-susceptibility measurements have been carried out in La_2-x_Sr_x_Cu_1-y_Zn_y_O_4_ with x = 0.10, 0.115 and 0.13 changing the Zn-concentration y finely up to 0.10, with the aim to clarify…

Superconductivity · Physics 2009-11-10 T. Adachi , S. Yairi , K. Takahashi , Y. Koike , I. Watanabe , K. Nagamine

We report muon spin relaxation (muSR) and magnetic susceptibility investigations of two Ti3+ chain compounds which each exhibit a spin gap at low temperature, NaTiSi2O6 and TiOCl. From these we conclude that the spin gap in NaTiSi2O6 is…

Strongly Correlated Electrons · Physics 2010-07-08 P. J. Baker , S. J. Blundell , F. L. Pratt , T. Lancaster , M. L. Brooks , W. Hayes , M. Isobe , Y. Ueda , M. Hoinkis , M. Sing , M. Klemm , S. Horn , R. Claessen

The ground state of the quantum spin system kappa-(BEDT-TTF)2Cu2(CN)3 in which antiferromagnetically-interacting S=1/2 spins are located on a nearly equilateral triangular lattice attracts considerable interest both from experimental and…

Spin-lattice relaxation rate $T_1^{-1}$ of $^1$H-NMR has been measured in (CH$_3$)$_2$CHNH$_3$Cu(Cl$_x$Br$_{1-x}$)$_3$ with $x=0.88$, which has been reported to be gapped system with singlet ground state from the previous macroscopic…

Strongly Correlated Electrons · Physics 2009-11-13 T. Adachi , K. Kanada , T. Saito , A. Oosawa , T. Goto

We carried out zero-field muon-spin-rotation (ZF-$\mu$SR) measurements in hydrostatic pressures in impurity-doped quantum spin gap system Tl(Cu$_{0.985}$Mg$_{0.015}$)Cl$_3$ to investigate microscopic magnetic properties of the…

Strongly Correlated Electrons · Physics 2015-05-18 Takao Suzuki , Isao Watanabe , Fumiko Yamada , Motoki Yamada , Yasuyuki Ishii , Takayuki Kawamata , Takayuki Goto , Hidekazu Tanaka
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