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Single molecules trapped in the solid state at liquid helium temperatures are promising quantum emitters for the development of quantum technologies owing to their remarkable photostability and their lifetime-limited optical coherence time…

We present recent results on the coherent control of an optical transition in a single rubidium atom, trapped in an optical tweezer. We excite the atom using resonant light pulses that are short (4 ns) compared with the lifetime of the…

A major challenge in generating single photons with a single emitter is to excite the emitter while avoiding laser leakage into the collection path. Ideally, any scheme to suppress this leakage should not result in a loss in efficiency of…

The interaction of a quantum two-level system with a resonant driving field results in the emergence of Rabi oscillations, which are the hallmark of a controlled manipulation of a quantum state on the Bloch sphere. This all-optical coherent…

In an experiment on three-photon laser excitation $5S_{1/2} \to 5P_{3/2} \to 6S_{1/2} \to 37P_{3/2}$ of a single $^{87}$Rb Rydberg atom in an optical dipole trap, we have observed for the first time three-photon Rabi oscillations between…

The controlled preparation of the excited state in a quantum emitter is a prerequisite for its usage as single-photon sources - a key building block for quantum technologies. In this paper we propose a coherent excitation scheme using…

Coherent conversion between a Raman pump field and its Stokes field is observed in a Raman process with a strong atomic spin wave initially prepared by another Raman process operated in the stimulated emission regime. The oscillatory…

Quantum Physics · Physics 2015-05-19 L. Q. Chen , Guo-Wan Zhang , Cheng-ling Bian , Chun-Hua Yuan , Z. Y. Ou , Weiping Zhang

A single Ca+ ion in a Paul trap has been cooled to the ground state of vibration with up to 99.9% probability. Starting from this Fock state |n=0> we have demonstrated coherent quantum state manipulation on an optical transition. Up to 30…

Quantum Physics · Physics 2009-10-31 Ch. Roos , Th. Zeiger , H. Rohde , H. C. Naegerl , J. Eschner , D. Leibfried , F. Schmidt-Kaler , R. Blatt

We demonstrate the coherent excitation of a mesoscopic ensemble of about 100 ultracold atoms to Rydberg states by driving Rabi oscillations from the atomic ground state. We employ a dedicated beam shaping and optical pumping scheme to…

Atomic Physics · Physics 2009-11-13 Markus Reetz-Lamour , Thomas Amthor , Johannes Deiglmayr , Matthias Weidemüller

The energy states in semiconductor quantum dots are discrete as in atoms, and quantum states can be coherently controlled with resonant laser pulses. Long coherence times allow the observation of Rabi-flopping of a single dipole transition…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 C. -M. Simon , T. Belhadj , B. Chatel , T. Amand , P. Renucci , A. Lemaitre , O. Krebs , P. A. Dalgarno , R. J. Warburton , X. Marie , B. Urbaszek

We demonstrate coherent one-color photoassociation of a Bose-Einstein condensate, which results in Rabi oscillations between atomic and molecular condensates. We attain atom-molecule Rabi frequencies that are comparable to decoherence rates…

Atomic Physics · Physics 2013-10-11 Mi Yan , B. J. DeSalvo , Ying Huang , P. Naidon , T. C. Killian

We propose free-electron Rabi oscillation by creating an isolated two-level system in a synthetic energy space induced by laser. The {\pi}/2-pulse and {\pi}-pulse in synthetic Rabi dynamics can function as 'beam splitters' and 'mirrors' for…

Quantum Physics · Physics 2023-04-25 Yiming Pan , Bin Zhang , Daniel Podolsky

Single dye molecules at cryogenic temperatures display many spectroscopic phenomena known from free atoms and are thus promising candidates for fundamental quantum optical studies. However, the existing techniques for the detection of…

Quantum Physics · Physics 2008-02-12 Gert Wrigge , Ilja Gerhardt , Jaesuk Hwang , Gert Zumofen , Vahid Sandoghdar

Rabi oscillations of quantum population are known to occur in two-level systems driven by spectrally narrow laser fields. In this work we study Rabi oscillations induced by shaped broadband femtosecond laser pulses. Due to the broad…

Quantum Physics · Physics 2015-05-30 S. Zhdanovich , J. W. Hepburn , V. Milner

We propose a method to reconstruct the vibrational quantum state of molecules excited by a general excitation laser pulse. Unlike existing methods, we do not require the molecules before excitation to be in a pure state, allowing us to…

Quantum Physics · Physics 2007-06-12 Anders S. Mouritzen , Olga Smirnova , Stefanie Grafe , Rune Lausten , Albert Stolow

We report on coherent resonant emission of the fundamental exciton state in a single semiconductor GaAs quantum dot. Resonant regime with picoseconde laser excitation is realized by embedding the quantum dots in a waveguiding structure. As…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 R. Melet , V. Voliotis , A. Enderlin , D. Roditchev , X. L. Wang , T. Guillet , R. Grousson

Efficient excitation of a single two-level system usually requires that the driving field is at the same frequency as the atomic transition. However, the scattered laser light in solid-state implementations can dominate over the single…

The electronic excitation of molecules triggers diverse phenomena such as luminescence and photovoltaic effects, which are the bases of various energy-converting devices. Understanding and control of the excitations at the single-molecule…

Chemical Physics · Physics 2017-07-12 Hiroshi Imada , Kuniyuki Miwa , Miyabi Imai-Imada , Shota Kawahara , Kensuke Kimura , Yousoo Kim

We use Rabi spectroscopy to explore the low-energy excitation spectrum of a finite-temperature Bose gas of rubidium atoms across the phase transition to a Bose-Einstein condensate (BEC). To record this spectrum, we coherently drive the…

Quantum Physics · Physics 2016-05-02 Baptiste Allard , Matteo Fadel , Roman Schmied , Philipp Treutlein

We investigate the interaction between a single atom and optical pulses in a coherent state with a controlled temporal envelope. In a comparison between a rising exponential and a square envelope, we show that the rising exponential…

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