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Using Gibbs ensemble Monte Carlo simulations and density functional theory we investigate the fluid-fluid demixing transition in inhomogeneous colloid-polymer mixtures confined between two parallel plates with separation distances between…

Soft Condensed Matter · Physics 2009-11-11 Andrea Fortini , Matthias Schmidt , Marjolein Dijkstra

Patchy colloidal model with three and four equivalent patches, confined in the attractive random porous media, undergo re-entrant gas-liquid phase separation with the possibility for the liquid phase density to approach zero. This unusual…

Soft Condensed Matter · Physics 2022-05-11 Taras Hvozd , Yurij V. Kalyuzhnyi , Vojko Vlachy , Peter T. Cummings

We consider fluid wetting on a corrugated substrate using effective interfacial Hamiltonian theory and show that breaking the translational invariance along the wall can induce an 'unbending' phase transition in addition to unbinding. Both…

Soft Condensed Matter · Physics 2009-10-31 C. Rascon , A. O. Parry , A. Sartori

We consider a model fluid with long-ranged, dispersion interparticle potentials confined between competing parallel walls. One wall is solvophilic and would be completely wet at bulk liquid-gas coexistence while the other is solvophobic and…

Soft Condensed Matter · Physics 2015-06-05 M. C. Stewart , R. Evans

The entropy of strongly coupled Yukawa fluids is discussed from several perspectives. First, it is demonstrated that a vibrational paradigm of atomic dynamics in dense fluids can be used to obtain a simple and accurate estimate of the…

Soft Condensed Matter · Physics 2024-09-18 Sergey Khrapak

Effect of ionic solute on a near-critical binary aqueous mixture confined between charged walls with different adsorption preferences is considered within a simple density functional theory. For the near-critical system containing small…

Soft Condensed Matter · Physics 2015-05-28 F. Pousaneh , A. Ciach

We present a study of the structural properties of the crystalline phases for a planar bilayer of particles interacting via repulsive Yukawa potentials in the weak screening region. The study is done with Monte Carlo computations and the…

Soft Condensed Matter · Physics 2010-09-08 Martial Mazars

Density functional theory is used to study binary colloidal fluids consisting of hard spheres and thin platelets in their bulk and near a planar hard wall. This system exhibits liquid-liquid coexistence of a phase that is rich in spheres…

Soft Condensed Matter · Physics 2009-11-10 L. Harnau , S. Dietrich

Immiscible two-phase flow in porous media with mixed wet conditions was examined using a capillary fiber bundle model, which is analytically solvable, and a dynamic pore network model. The mixed wettability was implemented in the models by…

Fluid Dynamics · Physics 2021-08-31 Hursanay Fyhn , Santanu Sinha , Subhadeep Roy , Alex Hansen

We present a theoretical study of wetting phenomena and interactions between liquid-vapor interfaces based on the density functional theory. The focus is mostly on the impact of long-range van der Waals interactions both within the fluid…

Chemical Physics · Physics 2011-11-10 Arik Yochelis , Len M. Pismen

We present a quantitative comparison between extensive Monte Carlo simulations and self-consistent field calculations on the phase diagram and wetting behavior of a symmetric, binary (AB) polymer blend confined into a film. The flat walls…

Statistical Mechanics · Physics 2009-10-31 M. Mueller , K. Binder

We study non-equilibrium analogues of surface phase transitions in a minimal model of active particles in contact with a purely repulsive potential barrier that mimics a thin porous membrane. Under conditions of bulk motility-induced phase…

Statistical Mechanics · Physics 2021-12-15 Francesco Turci , Nigel B. Wilding

We consider binary mixtures of soft repulsive spherical particles and calculate the depletion interaction between two big spheres mediated by the fluid of small spheres, using different theoretical and simulation methods. The validity of…

We analyse the $r \to \infty$ asymptotic decay of the total correlation function, $h(r)$, for a fluid composed of particles interacting via a (point) Yukawa pair potential. Such a potential provides a simple model for dusty plasmas. The…

Soft Condensed Matter · Physics 2007-05-23 P. Hopkins , A. J. Archer , R. Evans

While the density functional theory with integral equations techniques are very efficient tools in numerical analysis of complex fluids, an analytical insight into the phenomenon of effective interactions is still limited. In this paper we…

Soft Condensed Matter · Physics 2014-09-24 M. Majka , P. F. Góra

We study phase behaviour of a model fluid confined between two unlike parallel walls in the presence of long range (dispersion) forces. Predictions obtained from macroscopic (geometric) and mesoscopic arguments are compared with numerical…

Statistical Mechanics · Physics 2016-03-15 Alexandr Malijevský

We investigate the solvation of a hard spherical cavity, of radius $R$, immersed in a fluid for which the interparticle forces are short ranged. For thermodynamic states lying close to the liquid binodal, where the chemical potential…

Soft Condensed Matter · Physics 2009-11-10 R. Evans , J. R. Henderson , R. Roth

We adopt a field theoretical approach to study the structure and thermodynamics of a homogeneous Maier-Saupe nematogenic fluid interacting with anisotropic Yukawa potential. In the mean field approximation we retrieve the standard…

Soft Condensed Matter · Physics 2012-02-22 M. Holovko , D. di Caprio , I. Kravtsiv

Using fundamental-measure density functional theory we investigate entropic wetting in an asymmetric binary mixture of hard spheres with positive non-additivity. We consider a general planar hard wall, where preferential adsorption is…

Soft Condensed Matter · Physics 2015-05-28 Paul Hopkins , Matthias Schmidt

We study the interplay between wetting and miscibility of a symmetric polymer mixture via MC simulations and SCF calculations. The film surfaces interact with the monomers via short ranged potentials and the wetting transition is of first…

Soft Condensed Matter · Physics 2007-05-23 Marcus Mueller , Kurt Binder