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Surface nanobubbles are complex micro- and nanoscale fluid systems. While thermodynamics is believed to dominate nanobubble dynamics, the precise mechanism by which nanobubble evolution is driven by thermodynamics remains unclear. It is…

Soft Condensed Matter · Physics 2025-02-06 Lili Lan , Yongcai Pan , Liang Zhao , Binghai Wen

Surface nanobubbles are stable gaseous phases in liquids that form on solid substrates. While their existence has been confirmed, there are many open questions related to their formation and dissolution processes along with their structures…

Fluid Dynamics · Physics 2022-04-20 Zhizhao Che , Panagiotis E. Theodorakis

It has been recently shown that nanobubbles exhibit a remarkable and unexpected stability. The lifetime of nanobubbles, formed either within liquids or on hydrophobic surfaces, can exceed by more than 10 orders of magnitude the theoretical…

Soft Condensed Matter · Physics 2019-05-14 Caroline Desgranges , Jerome Delhommelle

Experiments have not only revealed the remarkably long lifetime of nanobubbles, but also demonstrated the diffusive instability of bubbles above micrometers, thus a full-scale physical understanding on the stability of bubbles is in urgent…

Soft Condensed Matter · Physics 2021-12-28 Binghai Wen , Yongcai Pan , Lijuan Zhang , Shuo Wang , Limin Zhou , Chunlei Wang , Jun Hu

We study surface nanobubbles using molecular dynamics simulation of ternary (gas, liquid, solid) systems of Lennard-Jones fluids. They form for sufficiently low gas solubility in the liquid, i.e., for large relative gas concentration. For…

Fluid Dynamics · Physics 2012-11-19 J. H. Weijs , J. H. Snoeijer , D. Lohse

The stability and growth or dissolution of a single surface nanobubble on a chemically patterned surface are studied by Molecular Dynamics (MD) simulations of binary mixtures consisting of Lennard-Jones (LJ) particles. Our simulations…

Fluid Dynamics · Physics 2017-07-14 Shantanu Maheshwari , Martin van der Hoef , Xuehua Zhang , Detlef Lohse

The findings of long-lived surface nanobubbles in various experiments brought a puzzle in theory, as they were supposed to be dissolved in microseconds due to the high Laplace pressure. However, an increasing number of studies suggest that…

Soft Condensed Matter · Physics 2018-01-09 Yawei Liu , Xianren Zhang

The observed stability of nanobubbles contradicts the well-known result in classical nucleation theory, that the critical radius is both microscopic and thermodynamically unstable. Here nanoscopic stability is shown to be the combined…

Chemical Physics · Physics 2015-03-17 Phil Attard

Surface nanobubbles emerging at solid-liquid interfaces of submerged hydrophobic surfaces show extreme stability and very small (gas-side) contact angles. In a recent study Ducker (W. A. Ducker, Langmuir 25, 8907 (2009).) conjectured that…

Fluid Dynamics · Physics 2015-05-20 Siddhartha Das , Jacco H. Snoeijer , Detlef Lohse

Surface nanobubbles are nanoscopic spherical-cap shaped gaseous domains on immersed substrates which are stable, even for days. After the stability of a {\it single} surface nanobubble has been theoretically explained, i.e. contact line…

Fluid Dynamics · Physics 2020-02-06 Xiaojue Zhu , Roberto Verzicco , Xuehua Zhang , Detlef Lohse

Understanding the stability mechanism of surface micro/nanobubbles adhered to gas-evolving electrodes is essential for improving the efficiency of water electrolysis, which is known to be hindered by the bubble coverage on electrodes. Using…

Fluid Dynamics · Physics 2024-04-16 Yixin Zhang , Xiaojue Zhu , Jeffery A. Wood , Detlef Lohse

Using molecular dynamics, we study the nucleation and stability of bulk nanobubble clusters. We study the formation, growth, and final size of bulk nanobubbles. We find that, as long as the bubble-bubble interspacing is small enough, bulk…

Fluid Dynamics · Physics 2012-11-19 Joost H. Weijs , James R. T. Seddon , D. Lohse

A model for gas nanobubbles is proposed in which their remarkable stability is explained as due to the presence of a qualitatively different form of water covering the nanobubble surface layer which leads to a reduction of the diffusion…

Mesoscale and Nanoscale Physics · Physics 2014-10-15 Siddhartha Sen , Kumar S. Gupta

In gas evolving electrolysis, bubbles grow at electrodes due to a diffusive influx from oversaturation generated locally in the electrolyte by the electrode reaction. When considering electrodes of micrometer-size resembling catalytic…

Fluid Dynamics · Physics 2024-11-11 Mengyuan Huang , Chao Sun , Kerstin Eckert , Xianren Zhang , Gerd Mutschke

Experimental investigations of hydrophobic/water interfaces often return controversial results, possibly due to the unknown role of gas accumulation at the interfaces. Here, during advanced atomic force microscopy of the initial evolution…

Mesoscale and Nanoscale Physics · Physics 2015-12-29 Ing-Shouh Hwang , Chung-Kai Fang , Hsien-Chen Ko , Chih-Wen Yang , Yi-Hsien Lu

Shock wave induced cavitation experiments and atomic force microscopy measurements of flat polyamide and hydrophobized silicon surfaces immersed in water are performed. It is shown that surface nanobubbles, present on these surfaces, do not…

We provide a model for the remarkable stability of surface nanobubbles to bulk dissolution. The key to the solution is that the gas in a nanobubble is of Knudsen type. This leads to the generation of a bulk liquid flow which effectively…

Fluid Dynamics · Physics 2011-09-09 James Seddon , Harold Zandvliet , Detlef Lohse

Surface nanobubbles (NBs) are stable gaseous phases in liquids that form at the interface with solid substrates. They have been particularly intriguing for their high stability that contradicts theoretical expectations and their potential…

Soft Condensed Matter · Physics 2019-09-09 Panagiotis E. Theodorakis , Zhizhao Che

The mechanism of superstability of nanobubbles in liquid confirmed by many experimental studies is still in debate since the classical diffusion predicts their lifetime on the order of a few microseconds. In this work, we study the…

Chemical Physics · Physics 2018-10-30 Song-Nam Hong , Song-Hyok Choe , Un-Gi Jong , Myong-San Pak , Chol-Jun Yu

The formation and evolution of immersed surface micro- and nanobubbles are essential in various practical applications, such as the usage of superhydrophobic rematerials, drug delivery, and mineral flotation. In this work, we investigate…

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