Related papers: Nucleation, Growth, and Coarsening -- A Global Vie…
The emergence upon cooling of an ordered solid phase from a liquid is a remarkable example of self-assembly, which has also major practical relevance. Here, we use a recently developed committor-based enhanced sampling method [Kang et al.,…
Nucleation at large metastability is still largely an unsolved problem, although is a problem of tremendous current interest, with wide practical value. It is well-accepted that the classical nucleation theory (CNT) fails to provide a…
When a system is brought to a metastable state, nuclei of the equilibrium phase form and grow. This is the well-known nucleation and growth of first-order phase transitions. Near a critical point of a continuous phase transition, critical…
The initial purpose of this work is to provide a probabilistic explanation of a recent result on a version of Smoluchowski's coagulation equations in which the number of aggregations is limited. The latter models the deterministic evolution…
We introduce an extended Smoluchowski equation describing coagulation processes for which clusters of mass s grow between collisions with $ds/dt=As^\beta$. A physical example, dropwise condensation is provided, and its collision kernel K is…
Using state-of-the-art rare-event sampling simulations, we precisely characterize the nucleation of liquid droplets from a supersaturated Lennard-Jones gas and uncover a key physical feature: critical clusters nucleate with a density that…
Neutral grains made of the same dielectric material can attain considerable charges due to collisions and generate long-range interactions. We perform molecular dynamic simulations in three dimensions for a dilute, freely-cooling granular…
We propose a model of mass-conserving heterogeneous nucleation to describe the dynamics of ligand-receptor binding in closed cellular compartments. When the ligand dissociation rate is small, competition among receptors for free ligands…
We present an experiment on crystallization of packings of macroscopic granular spheres. This system is often considered to be a model for thermally driven atomic or colloidal systems. Cyclically shearing a packing of frictional spheres, we…
We study a class of growth processes in which clusters evolve via exchange of particles. We show that depending on the rate of exchange there are three possibilities: I) Growth: Clusters grow indefinitely; II) Gelation: All mass is…
We consider in this work a model for aggregation, where the coalescing particles initially have a certain number of potential links (called arms) which are used to perform coagulations. There are two types of arms, male and female, and two…
This model describes cluster aggregation in a stirred colloidal solution Interacting clusters compete for growth in this 'winner-takes-all' model; for finite assemblies, the largest cluster always wins, i.e. there is a uniform sediment. In…
The classical theory of grain nucleation suffers from both theoretical and predictive deficiencies. We strive to alleviate these deficiencies in our understanding of dust formation and growth by utilizing an atomistic model of nucleation.…
We study the solutions of the Smoluchowski coagulation equation with a regularisation term which removes clusters from the system when their mass exceeds a specified cut-off size, M. We focus primarily on collision kernels which would…
The empirical observation of aggregation of dielectric particles under the influence of electrostatic forces lies at the origin of the theory of electricity. The growth of clusters formed of small grains underpins a range of phenomena from…
To explain the rich structure of voids, clusters, sheets, and filaments apparent in the Universe, we present evidence for the convergence of the two classic approaches to gravitational clustering, the ``pancake'' and ``hierarchical''…
The present paper deals with the existence and uniqueness of global classical solutions to the continuous coagulation and nonlinear multiple fragmentation equations for large classes of unbounded coagulation, collision and breakup kernels.…
The phase separation mechanism of a binary liquid mixture off-critically quenched in its miscibility gap is nucleation and growth, its homogeneous phase reaching a metastable equilibrium state. The successive stages of growth of the…
We present a model for sticky particles in which cluster sizes after a reaction have $\ell$ fewer total particles than the sum of their reactants. The finite particle system is modeled as a Markov process under a mean-field assumption for…
We study hydrodynamic limits of the cluster coagulation model; a coagulation model introduced by Norris [$\textit{Comm. Math. Phys.}$, 209(2):407-435 (2000)]. In this process, pairs of particles $x,y$ in a measure space $E$, merge to form a…