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We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can…

Quantum Physics · Physics 2021-12-01 Alberto Castro , Adrian Garcia Carrizo , David Zueco , Fernando Luis

The coherent control of small quantum system is considered. For a two-level system coupled to an arbitrary bath we consider a pulse of finite duration. We derive the leading and the next-leading order corrections to the evolution operator…

Quantum Physics · Physics 2008-03-11 S. Pasini , T. Fischer , P. Karbach , G. S. Uhrig

Semiclassical catastrophes in the dynamics of a quantum rotor (molecule) driven by a strong time-varying field are considered. We show that for strong enough fields, a sharp peak in the rotor angular distribution can be achieved via…

Quantum Physics · Physics 2007-05-23 I. Sh. Averbukh , R. Arvieu , M. Leibscher

High-fidelity operation of quantum computers requires precise knowledge of the physical system through characterization. For motion-mediated entanglement generation in trapped ions, it is crucial to have precise knowledge of the…

Quantum Physics · Physics 2024-04-22 Qiyao Liang , Mingyu Kang , Ming Li , Yunseong Nam

At the core of attosecond science lies the ability to generate laser pulses of sub-femtosecond duration. In tabletop devices the process relies on high-harmonic generation, where a major challenge is to obtain high yields and high cutoff…

Atomic Physics · Physics 2014-11-05 J. Solanpää , J. A. Budagosky , N. I. Shvetsov-Shilovski , A. Castro , A. Rubio , E. Räsänen

A system consisting of a doubly clamped beam with an attached body (slider) free to move along the beam has been studied recently by multiple research groups. Under harmonic base excitation, the system has the capacity to passively adapt…

Adaptation and Self-Organizing Systems · Physics 2022-08-02 Florian Müller , Maximilian Beck , Malte Krack

We introduce a systematic expansion tailored to systems with strong local interactions and capable of computing response functions, including finite DC transport, analytically. The expansion is controlled by a small parameter $s^2$ that…

Strongly Correlated Electrons · Physics 2026-05-20 Pavel A Nosov , Eslam Khalaf , Patrick Ledwith

A moderately intense $450$ fs laser pulse is used to create rotational wave packets in gas phase $\rm{I_2}$ molecules. The ensuing time-dependent alignment, measured by Coulomb explosion imaging with a delayed probe pulse, exhibits the…

We investigate optimal control strategies for state to state transitions in a model of a quantum dot molecule containing two active strongly interacting electrons. The Schrodinger equation is solved nonperturbatively in conjunction with…

Quantum Physics · Physics 2016-08-14 R. Nepstad , L. Sælen , I. Degani , J. P. Hansen

Controlling molecular reactivity by shaped laser pulses is a long-standing goal in chemistry. Here we suggest a direct optimal control approach which combines external pulse optimization with other control parameters arising in the upcoming…

Quantum Physics · Physics 2024-01-03 A. R. Ramos Ramos , E. W. Fischer , P. Saalfrank , O. Kühn

In the framework of nuclear magnetic resonance, we consider the general problem of the coherent control of a spin coupled to a bath by means of composite or continuous pulses of duration $\tau_\mathrm{p}$. We show explicity that it is…

Quantum Physics · Physics 2010-03-16 S. Pasini , P. Karbach , C. Raas , G. S. Uhrig

We use atomistic tight-binding theory with a configuration interaction description of Coulomb and exchange effects to describe excitons in symmetric quantum dots in a vertical electric field. We show that field-induced manipulation of…

Mesoscale and Nanoscale Physics · Physics 2012-12-20 Garnett W. Bryant , Natalia Malkova , James Sims

On the basis of optimal control theory, we numerically study how to optimally manipulate molecular vibrational dynamics by using cycle-averaged polarizability interactions induced by mildly intense non-resonant laser (NR) pulses. As the…

Quantum Physics · Physics 2024-09-05 Reon Ishii , Tomotaro Namba , Hiroyuki Katsuki , Kenji Ohmori , Yukiyoshi Ohtsuki

In this paper, we present a unified computational method based on pseudospectral approximations for the design of optimal pulse sequences in open quantum systems. The proposed method transforms the problem of optimal pulse design, which is…

Chemical Physics · Physics 2009-08-17 Jr-Shin Li , Justin Ruths , Dionisis Stefanatos

In this article, we develop a numerical method to find optimal control pulses that accounts for the separation of timescales between the variation of the input control fields and the applied Hamiltonian. In traditional numerical…

Quantum Physics · Physics 2011-09-19 F. Motzoi , J. M. Gambetta , S. T. Merkel , F. K. Wilhelm

Coherent control of a system involves steering an interaction to a final coherent state by controlling the phase of an applied field. Plasmas support coherent wave structures that can be generated by intense laser fields. Here, we…

Plasma Physics · Physics 2015-06-02 Z. -H. He , B. Hou , V. Lebailly , J. A. Nees , K. Krushelnick , A. G. R. Thomas

Single particle states in the atomic trap employing the rotating magnetic field are found using the full time-dependent instantaneous trapping potential. These states are compared with those of the effective time-averaged potential. We show…

A common way to manipulate a quantum system, for example spins or artificial atoms, is to use properly tailored control pulses. In order to accomplish quantum information tasks before coherence is lost, it is crucial to implement the…

Quantum sensors can show unprecedented sensitivities, provided they are controlled in a very specific, optimal way. Here, we consider a spin sensor of time-varying fields in the presence of dephasing noise, and we show that the problem of…

Quantum Physics · Physics 2024-07-10 S. Hernández-Gómez , F. Balducci , G. Fasiolo , P. Cappellaro , N. Fabbri , A. Scardicchio

We study the interplay between rotating wave approximation and optimal control. In particular, we show that for a wide class of optimal control problems one can choose the control field such that the Hamiltonian becomes time-independent…

Quantum Physics · Physics 2016-03-21 Maximilian Keck , Matthias M. Müller , Tommaso Calarco , Simone Montangero