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We show that the asymmetric crystal environment of the V site in the ladder compound NaV$_{2}$O$_{5}$ leads to a strong coupling of vanadium 3d electrons to phonons. This coupling causes fluctuations of the charge on the V ions, and favors…

Strongly Correlated Electrons · Physics 2009-10-31 E. Ya. Sherman , M. Fischer , P. Lemmens , P. H. M. van Loosdrecht , G. Güntherodt

The lattice dynamic properties and spin-phonon coupling in DyMn$_2$O$_5$ are studied by using the density-functional theory. The calculated phonon frequencies are in very good agreement with experiments. We then compare the phonon modes…

Materials Science · Physics 2009-11-13 Tianqi Shen , Kun Cao , Guang-Can Guo , Lixin He

We observe charge-order fluctuations in the quasi-two-dimensional organic superconductor $\beta^{\prime\prime}$-(BEDT-TTF)2 SF5 CH2 CF2 SO3 both by means of vibrational spectroscopy, locally probing the fluctuating charge order, and…

Strongly Correlated Electrons · Physics 2010-11-15 S. Kaiser , M. Dressel , Y. Sun , A. Greco , J. A. Schlueter , G. L. Gard , N. Drichko

We have investigated the charge ordering phase of the quasi one dimensional quantum antiferromagnet (TMTTF)$_2X$ ($X=$ SbF$_6$, AsF$_6$ and PF$_6$) using high fields/frequencies electron paramagnetic resonance. In addition to the uniform…

Strongly Correlated Electrons · Physics 2021-05-07 C-E Dutoit , A. Stepanov , J. VanTol , M. Orio , S. Bertaina

Spin scalar chiral ordering gives rise to nontrivial topological characters and peculiar transport properties. We here examine how quantum spin fluctuations affect the spin scalar chiral ordering in itinerant electron systems. We take the…

Strongly Correlated Electrons · Physics 2015-06-17 Yutaka Akagi , Masafumi Udagawa , Yukitoshi Motome

Charge ordering phenomenon in $\theta$-(BEDT-TTF)$_2$X is studied by using 1/4-filled extended Hubbard model on an anisotropic triangular lattice through mean-field approximation. It is found that a metallic charge ordered state with…

Strongly Correlated Electrons · Physics 2009-11-11 Masato Kaneko , Masao Ogata

Charge order affects most of the electronic properties but is believed not to alter the spin arrangement since the magnetic susceptibility remains unchanged. We present electron-spin-resonance experiments on quasi-one-dimensional (TMTTF)2X…

Strongly Correlated Electrons · Physics 2013-03-19 M. Dressel , M. Dumm , T. Knoblauch , B. Köhler , B. Salameh , S. Yasin

Based on recently proposed anti-ferromagnetic spin fluctuation exchange models for $d_{x^2-y^2}$-superconductors, we show that coupling to harmonic phonons {\it{cannot}} account for the observed isotope effect in the cuprate high-$T_c$…

Condensed Matter · Physics 2009-10-28 H. -B. Schüttler , C. -H. Pao

We theoretically investigate charge order and nonlinear conduction in a quasi-two-dimensional organic conductor \beta-(meso-DMBEDT-TTF)2PF6 [DMBEDT-TTF=dimethylbis(ethylenedithio)tetrathiafulvalene]. Within the Hartree-Fock approximation,…

Strongly Correlated Electrons · Physics 2013-10-28 Yasuhiro Tanaka , Kenji Yonemitsu

Motivated by the various physical properties observed in $\theta$-(BEDT-TTF)$_2$X, we study the ground state of extended Hubbard model on two-dimensional anisotropic triangular lattice at 1/4-filling with variational Monte Carlo method. It…

Strongly Correlated Electrons · Physics 2007-05-23 Hiroshi Watanabe , Masao Ogata

The Mott-insulator \kappa-(BEDT-TTF)_2Cu_2(CN)_3 is the prime candidate of a quantum spin liquid with puzzling magnetic properties. Our THz and infrared investigations reveal that also the charge dynamics does not follow the expectations…

Strongly Correlated Electrons · Physics 2012-11-06 Sebastian Elsasser , Dan Wu , Martin Dressel , John A. Schlueter

We examine the various instabilities of quarter-filled strongly correlated electronic chains in the presence of a coupling to the underlying lattice. To mimic the physics of the (TMTTF)$_2$X Bechgaard-Fabre salts we also include…

Strongly Correlated Electrons · Physics 2009-11-07 Jose Riera , Didier Poilblanc

We investigate a simple model of a frustrated classical spin chain coupled to adiabatic phonons under an external magnetic field. A thorough study of the magnetization properties is carried out both numerically and analytically. We show…

Strongly Correlated Electrons · Physics 2007-05-23 D. C. Cabra , M. Moliner , F. Stauffer

We present a systematic investigation of the low-frequency charge carrier dynamics in different charge states of the organic conductors $\theta$-(BEDT-TTF)$_2$$M$Zn(SCN)$_4$ with $M$=Rb,Tl, which result from quenching or relaxing the charge…

Strongly Correlated Electrons · Physics 2022-05-25 Tatjana Thomas , Tim Thyzel , Hungwei Sun , Kenichiro Hashimoto , Takahiko Sasaki , Hiroshi M. Yamamoto , Jens Müller

We uncover four new spin-charge ordered ground states in the strong coupling limit of the Kondo lattice model on triangular geometry. Two of the states at one-third electronic filling ($n=1/3$) consist of decorated ferromagnetic chains…

Strongly Correlated Electrons · Physics 2015-06-23 Sahinur Reja , Rajyavardhan Ray , Jeroen van den Brink , Sanjeev Kumar

We theoretically investigate the effects of charge order and spin frustration on the spin ordering in TMTTF salts. Using first-principles band calculations, we find that a diagonal inter-chain transfer integral $t_{q1}$, which causes spin…

Strongly Correlated Electrons · Physics 2012-02-06 Kazuyoshi Yoshimi , Hitoshi Seo , Shoji Ishibashi , Stuart E. Brown

The spatial charge arrangement of a typical quasi-two-dimensional organic conductor alpha-(BEDT-TTF)2I3 is revealed by single crystal structure analysis using synchrotron radiation. The results show that the horizontal stripe type…

Strongly Correlated Electrons · Physics 2009-11-13 Toru Kakiuchi , Yusuke Wakabayashi , Hiroshi Sawa , Toshihiro Takahashi , Toshikazu Nakamura

The crystal structure and lattice phonons of (BEDT-TTF)_2I_3 superconducting \beta-phase are computed and analyzed by the Quasi Harmonic Lattice Dynamics (QHLD) method. Whereas the crystal structure and its temperature and pressure…

Superconductivity · Physics 2024-11-26 A. Girlando , M. Masino , G. Visentini , R. G. Della Valle , A. Brillante , E. Venuti

Triangular-lattice systems attract a lot of attention due to various frustration-induced and strongly correlated effects. Here, we focus on the charge-ordering phenomenon by means of investigation of the extended Hubbard model with…

Strongly Correlated Electrons · Physics 2026-05-19 Aleksey Alekseev , Agnieszka Cichy , Konrad Jerzy Kapcia

We have theoretically investigated the spin and charge fluctuations in the quasi-one dimensional organic superconductor (TMTSF)2ClO4. Using the extended multi-site Hubbard model, which contains four sites in a unit cell and the transfer…

Superconductivity · Physics 2015-05-20 Yusuke Mizuno , Akito Kobayashi , Yoshikazu Suzumura