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We studied the reflectivity spectra of amorphous silicon dioxide detected under vacuum UV synchrotron radiation as a function of temperature between 10 and 300 K. Kramers-Kronig dispersion analysis of reflectivity spectra allowed us to…

Disordered Systems and Neural Networks · Physics 2010-09-21 E. Vella , F. Messina , M. Cannas , R. Boscaino

The optical response of phosphorene can be gradually changed by application of moderate uniaxial compression, as the material undergoes the transition into an indirect gap semiconductor and eventually into a semimetal. Strain tunes not only…

Materials Science · Physics 2015-04-01 L. Seixas , A. S. Rodin , A. Carvalho , A. H. Castro Neto

Crystalline sheets (e.g., graphene and transition metal dichalcogenides) liberated from a substrate are a paradigm for materials at criticality because flexural phonons can fluctuate into the third dimension. Although studies of static…

Materials Science · Physics 2024-01-10 Paul Z. Hanakata , Sourav S. Bhabesh , David Yllanes , David R. Nelson , Mark J. Bowick

Atomistically detailed computational studies of nanocrystals, such as those derived from the promising lead-halide perovskites, are challenging due to the large number of atoms and lack of symmetries to exploit. Here, focusing on…

Materials Science · Physics 2022-10-05 Giulia Biffi , Yeongsu Cho , Roman Krahne , Timothy C. Berkelbach

We present a continuum model describing dissolution and growth of a crystal contact confined against a substrate. Diffusion and hydrodynamics in the liquid film separating the crystal and the substrate are modeled within the lubrication…

Soft Condensed Matter · Physics 2018-01-31 Luca Gagliardi , Olivier Pierre-Louis

The energy spectra and wavefunctions of bound excitons in important two-dimensional (2D) graphene derivatives, i.e., graphyne and graphane, are found to be strongly modified by quantum confinement, making them qualitatively different from…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Shouting Huang , Yufeng Liang , Li Yang

The absorption and emission spectra of silicon nanocrystals up to 1 nm diameter including geometry optimization and the many-body effects induced by the creation of an electron-hole pair have been calculated within a first-principles…

Exciton condensation--an interaction-driven, macroscopically coherent paired-fermion state--offers the prospect for dissipationless energy transport in solids, akin to that in superconductivity. Although their light effective mass and…

We measure the coherent nonlinear response of excitons in a single-layer of molybdenum disulphide embedded in hexagonal boron nitride, forming a $h$-BN/MoS$_2$/$h$-BN heterostructure. Using four-wave mixing microscopy and imaging, we…

The fine structure of the exciton spectrum, containing optically allowed (bright) and forbidden (dark) exciton states, determines the radiation efficiency in nanostructures. We study time-resolved micro-photoluminescence in MoS$_2$…

We study the excitonic recombination dynamics in an ensemble of (9,4) semiconducting single-wall carbon nanotubes by high sensitivity time-resolved photo-luminescence experiments. Measurements from cryogenic to room temperature allow us to…

Other Condensed Matter · Physics 2015-06-25 S. Berger , C. Voisin , G. Cassabois , C. Delalande , Philippe Roussignol , X. Marie

This study investigates the effect of hydrostatic pressure on the luminescence properties of CsPbBr3 single crystals at 12 K. The luminescence at the edge of the band gap reveals a structure attributed to free excitons, phonon replica of…

The geminate annihilation of two triplet excitons created by singlet exciton fission is affected by the dimensionality of transport as determined by typically anisotropic triplet exciton mobilities in organic molecular crystals. We analyze…

Materials Science · Physics 2024-05-16 Eric A. Wolf , Ivan Biaggio

We present a comprehensive experimental and theoretical studies of photoluminescence of single CdMnTe quantum dots with Mn content x ranging from 0.01 to 0.2. We distinguish three stages of the equilibration of the exciton-Mn ion spin…

Mesoscale and Nanoscale Physics · Physics 2013-07-23 Ł. Kłopotowski , Ł. Cywiński , M. Szymura , V. Voliotis , R. Grousson , P. Wojnar , K. Fronc , T. Kazimierczuk , A. Golnik , G. Karczewski , T. Wojtowicz

Using density-functional theory we investigate several properties of Al(111), Al(100), Al(110), and stepped Al(111) surfaces. We report results of formation energies of surfaces, steps, adatoms, and vacancies. For the adsorption and…

mtrl-th · Physics 2008-02-03 Roland Stumpf , Matthias Scheffler

The band structure of bilayer graphene is tunable by introducing a relative twist angle between the two layers, unlocking exotic phases, such as superconductor and Mott insulator, and providing a fertile ground for new physics. At…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Matthew C. DeCapua , Yueh-Chun Wu , Takashi Taniguchi , Kenji Watanabe , Jun Yan

Here we demonstrate the controlled growth of Bi(110) and Bi(111) films on an (insulating) $\alpha$-Al$_2$O$_3$(0001) substrate by surface X-ray diffraction and X-ray reflectivity using synchrotron radiation. At temperatures as low as 40 K,…

Crystallization of rubrene, progressing from an amorphous phase to a triclinic meta-stable and ultimately to the orthorhombic stable phase, offers broad applications not only in organic electronic devices but also for in-depth studies of…

Materials Science · Physics 2025-05-13 Moha Naeimi , Katharina Engster , Ingo Barke , Sylvia Speller

The excimer formation dynamics of pyrene-labeled molecules in lipid bilayers depends on molecular motion over distances of the order of 1-2 nm. From the concentration dependence of the excimer photoemission curve, it is possible to derive a…

Soft Condensed Matter · Physics 2022-04-12 Pierre Ayoub , Fabrice Thalmann

The difficulty of describing excitons in semiconducting SWNTs analytically lies with the fact that excitons can neither be considered strictly 1D nor 2D objects. However, the situation changes in the case of metallic nanotubes where, by…

Mesoscale and Nanoscale Physics · Physics 2019-01-29 L. Shan , M. Agarwal , E. G. Mishchenko