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The magnetic ground state of two isostructural coordination polymers (i) the quasi two-dimensional S = 1/2 square-lattice antiferromagnet [Cu(HF$_{2}$)(pyrazine)$_{2}$]SbF$_{6}$; and (ii) a new compound…

Antiferromagnetically coupled moments on the frustrated triangular lattice typically order in a coplanar state at low temperature. Here, we demonstrate that the presence of not-very-large easy axis single ion anisotropy leads to an…

Strongly Correlated Electrons · Physics 2010-07-27 Arnab Sen , Fa Wang , Kedar Damle

Topological orbital moments can arise in non-coplanar spin structures even in the absence of spin-orbit coupling and a net topological orbital magnetization occurs for the triple-Q state and for isolated skyrmions. For atomic-scale skyrmion…

Elastic neutron scattering, ac susceptibility, and specific heat experiments on the pyrochlores Er$_{2}$Ge$_{2}$O$_{7}$ and Yb$_{2}$Ge$_{2}$O$_{7}$ show that both systems are antiferromagnetically ordered in the $\Gamma_5$ manifold. The…

Strongly Correlated Electrons · Physics 2015-10-12 Z. L. Dun , X. Li , R. S. Freitas , E. Arrighi , C. R. Dela Cruz , M. Lee , E. S. Choi , H. B. Cao , H. J. Silverstein , C. R. Wiebe , J. G. Cheng , H. D. Zhou

In the pyrochlore lattice Heisenberg antiferromagnet, for large spin length $S$, the massive classical ground state degeneracy is partly lifted by the zero-point energy of quantum fluctuations at harmonic order in spin-waves. However, there…

Strongly Correlated Electrons · Physics 2013-05-29 Uzi Hizi , Christopher L. Henley

The antiferromagnetic Heisenberg model on an anisotropic kagome lattice may be a good minimal model for real magnetic systems as well as a limit from which the isotropic case can be better understood. We therefore study the nearest-neighbor…

Strongly Correlated Electrons · Physics 2009-08-05 E. M. Stoudenmire , Leon Balents

Monoaxial chiral magnets can form a noncollinear twisted spin structure called the chiral helimagnetic state. We study magnetic properties of such a chiral helimagnetic state, with emphasis on the effect of itinerant electrons. Modeling a…

Strongly Correlated Electrons · Physics 2018-05-23 Shun Okumura , Yasuyuki Kato , Yukitoshi Motome

We theoretically investigate an antiferromagnetic structure in a hexagonal zigzag-chain compound Ce$_3$TiBi$_5$, which shows a linear magnetoelectric effect in metals and an unfamiliar temperature dependence of magnetic susceptibility. We…

Strongly Correlated Electrons · Physics 2023-01-19 Satoru Hayami , Hiroaki Kusunose

Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

Strongly Correlated Electrons · Physics 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

Tl$_{2}$Mn$_{2}$O$_{7}$ pyrochlores present colossal magnetoresistance (CMR) around the long range ferromagnetic ordering temperature (T$_{C}$). The character of this magnetic phase transition has been determined to be first order, by…

Materials Science · Physics 2009-11-07 P. Velasco , J. Mira , F. Guinea , J. Rivas , M. J. Martinez-Lope , J. A. Alonso , J. L. Martinez

Antiferromagnetic and ferro/ferrimagnetic orders are typically exclusive in nature, thus, their co-existence in atomic-scale proximity is expected only in heterostructures. Breaking this paradigm and broadening the range of unconventional…

Most works on pyrochlore magnets deal with the interacting spin-1/2 local moments. We here study the spin-one local moments on the pyrochlore lattice, and propose a generic interacting spin model on a pyrochlore lattice. Our spin model…

Strongly Correlated Electrons · Physics 2018-07-11 Fei Ye Li , Gang Chen

Magnetic properties of the pyrovanadate CaCoV$_2$O$_7$ have been studied by means of the bulk magnetization and neutron powder diffraction measurements. Magnetic susceptibility in the paramagnetic phase shows Curie-Weiss behavior with…

Materials Science · Physics 2021-08-03 Ryo Murasaki , Kazuhiro Nawa , Daisuke Okuyama , Maxim Avdeev , Taku J Sato

The static magnetic and dynamic properties of the compound (NH3)2(CH2)3CoCl4 are investigated in the temperature interval 0.5-50 K. It is shown that at TN =2.05 K this compound undergoes a transition to a magnetically ordered…

Materials Science · Physics 2009-11-11 A. S. Cherny , K. G. Dergachev , M. I. Kobets , E. N. Khatsko

The classical Heisenberg antiferromagnet on the pyrochlore lattice is macroscopically and continuously degenerate and the system remains disordered at all temperatures, even in the presence of weak dilution with nonmagnetic ions. We show…

Disordered Systems and Neural Networks · Physics 2009-10-31 L. Bellier-Castella , M. J. P. Gingras , P. C. W. Holdsworth , R. Moessner

Experiments in the antiferromagnetic phase of a quasi 2D $S=1/2$ quasi-square lattice antiferromagnet Cu(pz)2(ClO4)2 reveal a biaxial type of the anisotropy, instead of the easy-plane one, considered before. The weak in-plane anisotropy,…

Strongly Correlated Electrons · Physics 2013-06-12 K. Yu. Povarov , A. I. Smirnov , C. P. Landee

The consecutive magnetic ordering of the Ho and Ru ions in the pyrochlore Ho2Ru2O7 and their interplay are investigated by neutron scattering, magnetic and specific heat measurements. The Ru moments order at 95 K into a $\Gamma_5$…

We study noncoplanar magnetic ordering in frustrated itinerant magnets. For a family of Kondo square lattice models with classical local moments, we find that a double-$Q$ noncoplanar vortex crystal has lower energy than the single-$Q$…

Strongly Correlated Electrons · Physics 2016-09-26 Ryo Ozawa , Satoru Hayami , Kipton Barros , Gia-Wei Chern , Yukitoshi Motome , Cristian D. Batista

We present a strategy to design structures for which a polar lattice distortion induces weak ferromagnetism. We identify a large class of multiferroic oxides as potential realizations and use density-functional theory to screen several…

Materials Science · Physics 2013-05-29 Craig J. Fennie

Easy axis antiferromagnets are robust against external magnetic fields of moderate strength. Spin reorientations in strong fields can provide an insight into more subtle properties of antiferromagnetic materials, which are often hidden by…