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By performing first-principles calculations, we systematically explore the effect of epitaxial strain on the structure and properties of multiferroic TbMnO3. We show that, although the unstrained bulk TbMnO3 displays a non-collinear…

Materials Science · Physics 2015-05-20 Yusheng Hou , Jihui Yang , Xingao Gong , Hongjung Xiang

Using configuration-state-constrained electronic structure calculations based on the generalized gradient approximation plus Hubbard U method, we sought the origin of the giant tetragonal ferroelectric distortion in the ambient phase of the…

Strongly Correlated Electrons · Physics 2011-05-25 Ting Jia , Hua Wu , Guoren Zhang , Xiaoli Zhang , Ying Guo , Zhi Zeng , Hai-Qing Lin

Two-dimensional (2D) magnets have broad application prospects in the spintronics, but how to effectively control them with a small electric field is still an issue. Here we propose that 2D magnets can be efficiently controlled in a…

Mesoscale and Nanoscale Physics · Physics 2022-02-01 Ping Li , Xue-Song Zhou , Zhi-Xin Guo

Logical devices based on spin waves offer the potential to avoid dissipation mechanisms that limit devices based on either the charge or spin of mobile electrons. Multiferroic magnetoelectrics, which are materials that combine ferroelectric…

Materials Science · Physics 2008-04-10 Rogerio de Sousa , Joel E. Moore

We report x-ray diffraction, electrical resistivity, and magnetoresistance measurements on Bi2Se3 under high pressure and low temperature conditions. Pressure induces profound changes in both the room temperature value of the electrical…

Materials Science · Physics 2015-06-03 J. J. Hamlin , J. R. Jeffries , N. P. Butch , P. Syers , D. A. Zocco , S. T. Weir , Y. K. Vohra , J. Paglione , M. B. Maple

Multiferroic BiFeO3 ceramics have been doped with Ca. The smaller ionic size of Ca compared with Bi means that doping acts as a proxy for hydrostatic pressure, at a rate of 1%Ca=0.3GPa. It is also found that the magnetic Neel temperature…

Materials Science · Physics 2013-05-29 G. Catalan , K. Sardar , N. S. Church , J. F. Scott , R. J. Harrison , S. A. T. Redfern

Magnetoelectric, dielectric and magnetic susceptibility tensors of multiferroic TbMnO3 with cycloidal antiferromagnetic structure in external electric and magnetic fields have been investigated with taking into account dynamics of spin,…

Materials Science · Physics 2013-04-17 Igor V. Bychkov , Dmitry A. Kuzmin , Sergey J. Lamekhov , Vladimir G. Shavrov

We have successfully induced multiferroic behavior in the A-type antiferromagnet SmMnO3 by the substitution of Y at the Sm site. A magnetic transition develops at 24 K for Sm1-xYxMnO3 (x=0.4,0.5) which is not present in the parent compound.…

Strongly Correlated Electrons · Physics 2011-05-17 D. O'Flynn , C. V. Tomy , M. R. Lees , A. Daoud-Aladine , G. Balakrishnan

We show that inducing structural softness in regular magnetoelectric (ME) multiferroics -- i.e., tuning the materials to make their structure strongly reactive to applied fields -- makes it possible to obtain very large ME effects. We…

Materials Science · Physics 2012-04-17 Jacek C. Wojdeł , Jorge Íñiguez

A theoretical description of the sequence of magnetic phases in Co3TeO6 is presented. The strongly first-order character of the transition to the commensurate multiferroic ground state, induced by coupled order parameters corresponding to…

Strongly Correlated Electrons · Physics 2012-07-06 Pierre Tolédano , Vera Carolus , Matthias Hudl , Thomas Lottermoser , Dmitry D. Khalyavin , Sergey A. Ivanov , Manfred Fiebig

Cross-coupling of ordering parameters in multiferroic materials by multiple external stimuli other than electric field and magnetic field is highly desirable from both practical application and fundamental study points of view. Recently,…

Materials Science · Physics 2016-09-27 Tingting Jia , Hideo Kimura , Zhenxiang Cheng , Hongyang Zhao

We report the first high pressure measurement of the Fe K-edge in hematite (Fe$_2$O$_3$) by X-ray absorption spectroscopy in partial fluorescence yield geometry. The pressure-induced evolution of the electronic structure as Fe$_2$O$_3$…

The effects of high magnetic fields applied perpendicular to the spontaneous ferroelectric polarization on single crystals of BiFeO$_3$ were investigated through magnetization, magnetostriction, and neutron diffraction measurements. The…

We study the influence of external pressure on the electronic and magnetic structure of EuMnO3 from first-principles calculations. We find a pressure-induced insulator-metal transition at which the magnetic order changes from A-type…

Computational Physics · Physics 2017-06-30 R. Qiu , E. Bousquet , A. Cano

Recently, the perovskite BiCoO$_3$ has been shown experimentally to be isostructural with PbTiO$_3$, while simultaneously the $d^6$ Co$^{3+}$ ion has a high spin ground state with $C$-type antiferromagnetic ordering. Using hybrid density…

Materials Science · Physics 2016-05-04 Leigh Weston , Xiangyuan Cui , Simon P. Ringer , Catherine Stampfl

The incommensurate magnetic structures and phase diagrams of multiferroics has been explored on the basis of accurate micromagnetic analysis taking into account the spin flexoelecric interaction (Lifshitz invariant). The objects of the…

Materials Science · Physics 2015-06-15 Z. V. Gareeva , A. F. Popkov , S. V. Soloviov , A. K. Zvezdin

We present a first principles study of an unusual heterostructure, an atomic-scale checkerboard of BiFeO3-BiMnO3, and compare its properties to the two bulk constituent materials, BiFeO3 and BiMnO3. The "nanocheckerboard" is found to have a…

Materials Science · Physics 2015-05-19 L. Palova , P. Chandra , K. M. Rabe

Epitaxial strain has emerged as a powerful tool to tune magnetic and ferroelectric properties in functional materials such as in multiferroic perovskite oxides. Here, we use first-principles calculations to explore the evolution of magnetic…

Materials Science · Physics 2023-11-23 Sebastian Meyer , Bin Xu , Laurent Bellaiche , Bertrand Dupé

We analyze the coupling between the ferroelectric and magnetic order parameters in the magnetoelectric multiferroic BiFeO_3 using density functional theory within the local spin density approximation and the LSDA+U method. We show that weak…

Materials Science · Physics 2007-05-23 Claude Ederer , Nicola A. Spaldin

We present an ab initio study of the BFCO solid solution formed by multiferroics BiFeO3 (BFO) and BiCoO3 (BCO). We find that BFCO presents a strongly discontinuous morphotropic transition between BFO-like and BCO-like ferroelectric phases.…

Materials Science · Physics 2011-08-23 Oswaldo Diéguez , Jorge Íñiguez