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We report that CaMn$_7$O$_{12}$ is a new magnetic multiferroic material. The appearance of a ferroelectric polarization coinciding with the magnetic phase transition ($\sim90$ K) suggests the presence of ferroelectricity induced by…

Materials Science · Physics 2011-11-16 Guoquan Zhang , Shuai Dong , Zhibo Yan , Yanyan Guo , Qinfang Zhang , Seiji Yunoki , Elbio Dagotto , J. -M. Liu

LaMn$_7$O$_{12}$, a quadruple perovskite oxide (AA'$_3$B$_4$O$_{12}$-type), has attracted attention for its notable bifunctional activity in oxygen evolution and reduction reactions. Here, we systematically investigate the magnetic phase…

Strongly Correlated Electrons · Physics 2026-01-19 Haeyoon Jung , Indukuru Ramesh Reddy , Bongjae Kim , Jiyeon Kim , Sooran Kim

We report on the microwave, terahertz (THz), infrared and Raman spectroscopic studies of $BiMn_{7}O_{12}$ ceramics, shedding more light into the nature of two structural phase transitions and their possible relation with ferroelectricity in…

Materials Science · Physics 2024-01-08 A. Maia , M. Kempa , V. Bovtun , R. Vilarinho , C. Kadlec , J. Agostinho Moreira , A. A. Belik , P. Proschek , S. Kamba

By means of neutron powder diffraction, we investigated the effect of the polar Bi$^{3+}$ ion on the magnetic ordering of the Mn$^{3+}$ ions in BiMn$_3$Mn$_4$O$_{12}$, the counterpart with \textit{quadruple} perovskite structure of the…

Strongly Correlated Electrons · Physics 2019-06-05 A. Gauzzi , G. Rousse , F. Mezzadri , G. Calestani , G. André , F. Bourée , M. Calicchio , E. Gilioli , R. Cabassi , F. Bolzoni , A. Prodi , P. Bordet , M. Marezio

Due of its polymorphism, Mn$_2$FeSbO$_6$ can be synthesized at high pressures and temperatures as a ferrimagnetic ilmenite or an antiferromagnetic perovskite. The structural phase transformation is discussed in detail, and magnetic…

Strongly Correlated Electrons · Physics 2013-01-08 R. Mathieu , S. A. Ivanov , I. V. Solovyev , G. V. Bazuev , P. Anil Kumar , P. Lazor , P. Nordblad

A new type of multiferroicity was experimentally discovered in 2003 in a perovskite manganite TbMnO$_3$ where its ferroelectricity is induced by cycloidally ordered Mn spins. Susequently, such spin-cycloid multiferroic phase was also…

Strongly Correlated Electrons · Physics 2025-02-14 Masahito Mochizuki

In this article, we perform the symmetry analysis of perovskite-based multiferroics: bismuth ferrite (BiFeO3)-like, orthochromites (RCrO3), and Ruddlesden-Popper perovskites (Ca3Mn2O7-like), being the typical representatives of…

Materials Science · Physics 2022-01-26 Zukhra Gareeva , Anatoly Zvezdin , Konstantin Zvezdin , Xiang Ming Chen

We performed susceptibility, magnetization, specific heat, and single crystal neutron diffraction measurements on single crystalline BaMn$_2$Si$_2$O$_7$. Based on the results, we revisited its spin structure with a more accurate solution…

Strongly Correlated Electrons · Physics 2019-07-31 G. H. Wang , C. Y. Xu , H. B. Cao , T. Hong , Q. Huang , Q. Y. Ren , J. Q. Xu , H. D. Zhou , W. D. Luo , D. Qian , J. Ma

Using first-principles calculations we predict that the layered-perovskite metal Bi$_5$Mn$_5$O$_{17}$ is a ferromagnet, ferroelectric, and ferrotoroid which may realize the long sought-after goal of a room-temperature ferromagnetic…

Materials Science · Physics 2020-10-02 Andrea Urru , Francesco Ricci , Alessio Filippetti , Jorge Iniguez , Vincenzo Fiorentini

We present results of local spin density approximation (LSDA) pseudopotential calculations for the perovskite structure oxide, bismuth manganite (BiMnO3). The origin of the differences between bismuth manganite and other perovskite…

Materials Science · Physics 2009-10-31 Nicola A. Hill , Karin M. Rabe

We use resonant and non-resonant X-ray diffraction measurements in combination with first-principles electronic structure calculations and Monte Carlo simulations to study the relationship between crystal structure and multiferroic orders…

Many multiferroic materials, with various chemical compositions and crystal structures, have been discovered in the past years. Among these multiferroics, some perovskite manganites with ferroelectricity driven by magnetic orders are of…

Materials Science · Physics 2012-06-05 Shuai Dong , Jun-Ming Liu

The quadruple perovskite CaMn$_7$O$_{12}$ is a topical multiferroic, in which the hierarchy of electronic correlations driving structural distortions, modulated magnetism, and orbital order is not well known and may vary with temperature.…

Materials Science · Physics 2020-06-30 K. Gautam , S. S. Majid , S. Francoual , A. Ahad , K. Dey , M. C. Rahn , R. Sankar , F. C. Chou , D. K. Shukla

Multiferroics where at least two primary ferroic orders are present and coupled in a single system constitute an important class of materials. They attracted special consideration as they present both intriguing fundamental physics problems…

We report a neutron powder diffraction study of $R$Mn$_7$O$_{12}$ quadruple perovskite manganites with $R$ = La, Ce, Nd, Sm, and Eu. We show that in all measured compounds concomitant magnetic ordering of the $A$ and $B$ manganese…

Strongly Correlated Electrons · Physics 2018-08-29 R. D. Johnson , D. D. Khalyavin , P. Manuel , L. Zhang , K. Yamaura , A. A. Belik

This review devoted to multiferroic properties of Bismuth-based perovskites falls into two parts. The first part focuses on BiFeO3 and summarizes the recent progress made in the studies of its pressure-temperature phase diagram and…

Materials Science · Physics 2015-02-03 Mael Guennou , Michel Viret , Jens Kreisel

Despite the great technological and scientific importance, a well-controlled coupled behavior in magnetoelectric multiferroic materials at room temperature remains challenging. We demonstrate that the self-ordered A2BBO6 (e.g., A = La, B =…

Materials Science · Physics 2015-05-14 M. P. Singh , K. D. Truong , S. Jandl , P. Fournier

Through analysis of variable temperature neutron powder diffraction data, we present solutions for the magnetic structures of SrMn$_7$O$_{12}$, CdMn$_7$O$_{12}$, and PbMn$_7$O$_{12}$ in all long-range ordered phases. The three compounds…

Strongly Correlated Electrons · Physics 2017-09-06 R. D. Johnson , D. D. Khalyavin , P. Manuel , P. G. Radaelli , I. S. Glazkova , N. Terada , A. A. Belik

We present a first principles study of the series of multiferroic barium fluorides with the composition BaMF4, where M is Mn, Fe, Co, or Ni. We discuss trends in the structural, electronic, and magnetic properties, and we show that the…

Materials Science · Physics 2009-11-11 Claude Ederer , Nicola A. Spaldin

We use ab initio electronic structure calculations in combination with Monte Carlo simulations to investigate the magnetic and ferroelectric properties of bulk orthorhombic HoMnO$_3$ and ErMnO$_3$. Our goals are to explain the…

Materials Science · Physics 2018-12-12 Natalya S. Fedorova , Amadé Bortis , Christoph Findler , Nicola A. Spaldin
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