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Periodic supercell models of electric double layers formed at the interface between a charged surface and an electrolyte are subject to serious finite size errors and require certain adjustments in the treatment of the long-range…

Chemical Physics · Physics 2024-07-10 Thomas Sayer , Chao Zhang , Michiel Sprik

Freezing of charged colloids on square or triangular two-dimensional periodic substrates has been recently shown to realize a rich variety of orientational orders. We propose a theoretical framework to analyze the corresponding structures.…

Statistical Mechanics · Physics 2009-11-10 R. Agra , F. van Wijland , E. Trizac

We predict a condensation phenomenon in an overall neutral system, consisting of a single charged plate and its oppositely charged counterions. Based on the ``two-fluid'' model, in which the counterions are divided into a ``free'' and a…

Soft Condensed Matter · Physics 2016-08-31 A. W. C. Lau , D. B. Lukatsky , P. Pincus , S. A. Safran

Macromolecules, when immersed in a polar solvent like water, become charged by a fixed surface charge density which is compensated by ``counter-ions'' moving out of the surface. Such classical particle systems exhibit poor screening…

Statistical Mechanics · Physics 2015-11-04 Ladislav Šamaj

A variational theory is developed to study electrolyte solutions, composed of interacting point-like ions in a solvent, in the presence of dielectric discontinuities and charges at the boundaries. Three important and non-linear…

Soft Condensed Matter · Physics 2013-05-29 Sahin Buyukdagli , Manoel Manghi , John Palmeri

Phase separation and criticality are analyzed in $z$:1 charge-asymmetric ionic fluids of equisized hard spheres by generalizing the Debye-H\"{u}ckel approach combined with ionic association, cluster solvation by charged ions, and hard-core…

Statistical Mechanics · Physics 2009-11-10 Jean-Noel Aqua , Shubho Banerjee , Michael E. Fisher

We find that at intermediate temperatures, the metallic temperature dependence of the conductivity \sigma(T) of 2D electrons in silicon is described well by a recent interaction-based theory of Zala et al. (Phys. Rev. B 64, 214204 (2001)).…

Strongly Correlated Electrons · Physics 2007-05-23 A. A. Shashkin , S. V. Kravchenko , V. T. Dolgopolov , T. M. Klapwijk

The effects of image charges (i.e., induced surface charges of polarization) in spherical geometry and their implication for charged colloidal systems are investigated. We study analytically and exactly a single microion interacting with a…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina

Charge disproportionation (CD) and spin differentiation in Na$_{1/2}$CoO$_2$ are studied using the correlated band theory approach. The simultaneous CD and gap opening seen previously is followed through a first order charge…

Strongly Correlated Electrons · Physics 2007-05-23 K. -W. Lee , J. Kunes , P. Novak , W. E. Pickett

We investigate ionization at a solid-water interface in applied electric field. We attach an electrode to a dielectric film bearing silanol or carboxyl groups with an areal density $\Gamma_0$, where the degree of dissociation $\alpha$ is…

Soft Condensed Matter · Physics 2016-09-29 Ryuichi Okamoto , Akira Onuki

We study the electrophoretic mobility of spherical charged colloids in a low-salt suspension as a function of the colloidal concentration. Using an effective particle charge and a reduced screening parameter, we map the data for systems…

Soft Condensed Matter · Physics 2007-05-23 Vladimir Lobaskin , Burkhard Duenweg , Martin Medebach , Thomas Palberg , Christian Holm

The author used synchrotron x-ray reflectivity to study the ion-size effect for alkali ions (Na$^+$, K$^+$, Rb$^+$, and Cs$^+$), with densities as high as $4 \times 10^{18}- 7 \times 10^{18}$ m$^{-2}$, suspended above the surface of a…

Other Condensed Matter · Physics 2009-11-13 Aleksey M. Tikhonov

The collision efficiency of uncharged micron-sized water droplets in air is determined by the breakdown of hydrodynamics at droplet separations of the order of the mean-free path, by van-der-Waals forces, or a combination of the two. In…

Fluid Dynamics · Physics 2025-10-01 A. Dubey , G. P. Bewley , K. Gustavsson , B. Mehlig

The isotropic to nematic transition in a system of soft spherocylinders is studied by means of grand canonical Monte Carlo simulations. The probability distribution of the particle density is used to determine the coexistence density of the…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , T. Schilling

Hydrodynamic fluctuations have been studied in a wide variety of physical, chemical, and biological phenomena in the past decade. In high energy heavy ion collisions, there will be intrinsic fluctuations even if the initial conditions are…

Nuclear Theory · Physics 2013-06-18 Joseph I. Kapusta , Juan M. Torres-Rincon

We consider two charged semipermeable membranes, which bound bulk electrolyte solutions and are separated by a thin film of salt-free liquid. Small counter-ions permeate into the gap, which leads to a steric charge separation in the system.…

Soft Condensed Matter · Physics 2016-11-23 Salim R. Maduar , Olga I. Vinogradova

An approach is proposed which allows to self-consistently calculate the structural and thermodynamic properties of highly charged aqueous colloidal suspensions. The method is based on the renormalized Jellium model with the background…

Soft Condensed Matter · Physics 2009-10-27 Thiago E. Colla , Yan Levin , E. Trizac

We study the influence of the chiral phase transition on the chiral magnetic effect. The chiral electric current density along the magnetic field, the electric charge difference between on each side of the reaction plane, and the azimuthal…

High Energy Physics - Phenomenology · Physics 2015-05-18 Wei-jie Fu , Yu-xin Liu , Yue-liang Wu

Anionic DMPA monolayers spread on LaCl$_3$ solutions reveal strong cation adsorption and a sharp transition to surface overcharging at unexpectedly low bulk salt concentrations. We determine the surface accumulation of La$^{3+}$ with…

Soft Condensed Matter · Physics 2009-11-11 J. Pittler , W. Bu , D. Vaknin , A. Travesset , D. J. McGillivray , M. Losche

Despite decades of intensive studies, the effective interactions between strongly charged colloids still remain elusive. Here we show that a strongly charged surface with a layer of condensed counter- ions behaves effectively as a…

Soft Condensed Matter · Physics 2011-07-12 Xiangjun Xing , Zhenli Xu , Hongru Ma