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We report first principles analysis of electron-phonon coupling in molecular devices under external bias voltage and during current flow. Our theory and computational framework are based carrying out density functional theory within the…

Materials Science · Physics 2009-11-11 N. Sergueev , D. Roubtsov , Hong Guo

Equilibrium molecular dynamics simulation and the Green-Kubo formalism were used to calculate self-diffusion coefficient, shear viscosity,and thermal conductivity for 30 different quadrupolar two-center Lennard-Jones fluids along the bubble…

Chemical Physics · Physics 2009-06-18 G. A. Fernandez , J. Vrabec , H. Hasse

We present an efficient implemention of a non-equilibrium Green function (NEGF) method for self-consistent calculations of electron transport and forces in nanostructured materials. The electronic structure is described at the level of…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Jingzhe Chen , Kristian S. Thygesen , Karsten W. Jacobsen

Typical experimental measurement is set up as a study of the system's response to a stationary external excitation. This approach considers any random fluctuation of the signal as spurious contribution which is to be eliminated via…

Electron transport in periodic quantum dot arrays in the presence of interactions with phonons was investigated using the formalism of nonequilibrium Green's functions. The self-consistent Born approximation was used to model the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Nenad Vukmirović , Zoran Ikonić , Dragan Indjin , Paul Harrison

We present a conceptually simple method for treating electron-phonon scattering and phonon limited mobilities. By combining Green's function based transport calculations and molecular dynamics (MD), we obtain a temperature dependent…

Mesoscale and Nanoscale Physics · Physics 2017-06-28 Troels Markussen , Mattias Palsgaard , Daniele Stradi , Tue Gunst , Mads Brandbyge , Kurt Stokbro

We study thermoelectric transport through double quantum dots system with spin-dependent interdot coupling and ferromagnetic electrodes by means of the non-equilibrium Green function in the linear response regime. It is found that the…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Qiang Wang , Haiqing Xie , Hujun Jiao , Zhi-Jian Li , Yi-Hang Nie

We investigate the thermoelectric transport properties of an interacting parallel double quantum dot in the Coulomb-blockade regime. Building on an analytical solution based on an equation-of-motion technique, we extend the formalism for…

Mesoscale and Nanoscale Physics · Physics 2025-10-24 Nahual Sobrino

We study dynamic nonequilibrium electron charging phenomena in ballistic molecular devices at room temperature that compromise their response to bias and whose nature is evidently distinguishable from static Schottky-type potential…

Mesoscale and Nanoscale Physics · Physics 2008-05-13 Ioannis Deretzis , Antonino La Magna

We study electron transport through a quantum interferometer with side-coupled quantum dots. The interferometer, threaded by a magnetic flux $\phi$, is attached symmetrically to two semi-infinite one-dimensional metallic electrodes. The…

Mesoscale and Nanoscale Physics · Physics 2010-12-17 Santanu K. Maiti

Electronic transport in a model molecular device coupled to local phonon modes is theoretically analyzed. The method allows for obtaining an accurate approximation of the system's quantum state irrespective of the electron and phonon energy…

Mesoscale and Nanoscale Physics · Physics 2007-10-10 Antonino La Magna , Ioannis Deretzis

Transport in molecular electronic devices is different from that in semiconductor mesoscopic devices in two important aspects: (1) the effect of the electronic structure and (2) the effect of the interface to the external contact. A…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Yongqiang Xue , Supriyo Datta , Mark A. Ratner

Nonequilibrium electronic transport through a molecular level weakly coupled to a single coherent phonon/vibration mode has been studied for superconducting leads. The Keldysh Green function formalism is used to compute the current for the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. Zazunov , R. Egger , C. Mora , T. Martin

An integrated piecewise thermal equilibrium approach based on the first-principles calculation method has been developed to calculate bias dependent electronic structures and current- and differential conductance-voltage characteristics of…

Other Condensed Matter · Physics 2009-11-13 M. -H. Tsai , T. -H. Lu , Y. -H. Tang

We theoretically investigate the transport properties of a molecule embedded in one arm of a mesoscopic Aharonov-Bohm interferometer. Due to the presence of phonons the molecule level position ($\epsilon_d$) and the electron-electron…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Jong Soo Lim , Rosa Lopez , Gloria Platero , Pascal Simon

A model is developed describing the energy distribution of quasi-particles in a quasi-one dimensional, normal metal wire, where the transport is diffusive, connected between equilibrium reservoirs. When an ac bias is applied to the wire by…

Mesoscale and Nanoscale Physics · Physics 2017-02-20 Robbert-Jan Dikken

We model a small quantum dot with a magnetic impurity by the Anderson Hamiltonian with a supplementary exchange interaction term. The transport calculations are performed by means of the Green functions within the equation of motion scheme,…

Materials Science · Physics 2015-06-25 Mugurel Tolea , Bogdan R. Bulka

We theoretically study the electronic transport in the monolayer of dithiolated phenylene vinylene oligomeres coupled to the (111) surfaces of gold electrodes. We use non-equilibrium Green functions (NEGF) and density functional theory(DFT)…

Materials Science · Physics 2009-11-10 Z. Crljen , A. Grigoriev , G. Wendin , K. Stokbro

The conductance through a molecular device including electron-electron and electron-phonon interactions is calculated using the Numerical Renormalization Group method. At low temperatures and weak electron-phonon coupling the properties of…

Strongly Correlated Electrons · Physics 2007-05-23 P. S. Cornaglia , H. Ness , D. R. Grempel

Correlation effects in the transport properties of a single quantum level coupled to electron reservoirs are discussed theoretically using a non-equilibrium Green functions approach. Our method is based on the introduction of a second-order…

Condensed Matter · Physics 2016-08-14 A. Levy Yeyati , A. Martín-Rodero , F. Flores