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Motivated by the experimental realizations of nearly one-dimensional spin-1/2 Heisenberg model found in chain cuprates SrCuO$_2$ and Sr$_2$CuO$_3$, which remain in a quantum-critical Luttinger liquid state down to temperatures that are much…

Strongly Correlated Electrons · Physics 2016-08-31 A. M. Tsvelik , I. A. Zaliznyak

The nature of the magnetic ground state of highly frustrated systems remained puzzling to this day. Here, we have performed multifrequency electron spin resonance (ESR) measurements on a putative quantum spin liquid compound…

We present a numerical study of the spin-1/2 bilayer Heisenberg antiferromagnet with random interlayer dimer dilution. From the temperature dependence of the uniform susceptibility and a scaling analysis of the spin correlation length we…

Disordered Systems and Neural Networks · Physics 2009-11-07 O. P. Vajk , M. Greven

CoO has an odd number of electrons in its unit cell, and therefore is expected to be metallic. Yet, CoO is strongly insulating owing to significant electronic correlations, thus classifying it as a Mott insulator. We investigate the…

$\gamma$-${\rm Ba}_{3}{\rm CoNb}_{2}{\rm O}_{9}$ realizes a disordered simple-cubic spin-$1/2$ lattice in which Co$^{2+}$ ions randomly occupy one third of the sites, placing the system close to the site-percolation threshold for magnetic…

We develop a microscopic theory of multipole interactions and orderings in 5$d^2$ transition metal ion compounds. In a cubic environment, the ground state of 5$d^2$ ions is a non-Kramers $E_g$ doublet, which is nonmagnetic but hosts…

Strongly Correlated Electrons · Physics 2021-08-25 Giniyat Khaliullin , Derek Churchill , P. Peter Stavropoulos , Hae-Young Kee

Inelastic neutron scattering study has been performed in an S=3/2 bilayer honeycomb lattice compound Bi3Mn4O12(NO3) at ambient and high magnetic fields. Relatively broad and monotonically dispersive magnetic excitations were observed at…

Strongly Correlated Electrons · Physics 2020-01-08 M. Matsuda , S. E. Dissanayake , D. L. Abernathy , Y. Qiu , J. R. D. Copley , N. Kumada , M. Azuma

Static electrical and magnetic properties of single crystal BaVS_3 were measured over the structural (T_S=240K), metal-insulator (T_MI=69K), and suspected orbital ordering (T_X=30K) transitions. The resistivity is almost isotropic both in…

Strongly Correlated Electrons · Physics 2009-10-31 G. Mihaly , I. Kezsmarki , F. Zamborszky , M. Miljak , K. Penc , P. Fazekas , H. Berger , L. Forro

CeRh$_3$Si$_2$ has been reported to exhibit metamagnetic transitions below 5~K, a giant crystal field splitting, and anisotropic magnetic properties from single crystal magnetization and heat capacity measurements. Here we report results of…

We calculate the static and dynamic properties of single crystal, single molecule magnets consisting of equal spin $S=1/2$ or 5/2 dimers. The spins in each dimer interact with each other via the Heisenberg exchange interaction and with the…

Statistical Mechanics · Physics 2009-11-07 Dmitri V. Efremov , Richard A. Klemm

We report polarized- and unpolarized-neutron scattering measurements of magnetic excitations in single-crystal Na0.75CoO2. The data confirm ferromagnetic correlations within the cobalt-layers and reveal antiferromagnetic correlations…

Strongly Correlated Electrons · Physics 2007-05-23 L. M. Helme , A. T. Boothroyd , R. Coldea , D. Prabhakaran , D. A. Tennant , A. Hiess , J. Kulda

Exploring the physics of low-dimensional spin systems and their pressure-driven electronic and magnetic transitions are thriving research field in modern condensed matter physics. In this context, recently antiferromagnetic Cr-based…

Strongly Correlated Electrons · Physics 2024-01-02 Kuldeep Kargeti , Aadit Sen , S. K. Panda

We study the $S>1/2$ antiferromagnetic Heisenberg model on the 1/5-depleted square lattice as a function of the ratio of the intra-plaquette coupling to the inter-plaquette coupling. Using stochastic series expansion quantum Monte Carlo…

Strongly Correlated Electrons · Physics 2022-09-08 Jun-Han Huang , Zenan Liu , Han-Qing Wu , Dao-Xin Yao

Inelastic neutron scattering was used to determine the spin Hamiltonian for the singlet ground state system of fully deuterated BPCB, (C$_{5}$D$_{12}$N)$_{2}$CuBr$_{4}$. A 2-leg spin-1/2 ladder model, with $J_\bot = (1.09 \pm 0.01)$ meV and…

Although chromium trihalides are widely regarded as a promising class of two-dimensional magnets for next-generation devices, an accurate description of their electronic structure and magnetic interactions has proven challenging to achieve.…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 Ravi Yadav , Lei Xu , Michele Pizzochero , Jeroen van den Brink , Mikhail I. Katsnelson , Oleg V. Yazyev

We report on the use of the polarized $^3$He gas filter and neutron resonant enhancement techniques for the measurement of spin-polarized diffuse neutron scattering due to ferromagnetic domains. A CoO/Co exchange biased bilayer was grown on…

Materials Science · Physics 2007-05-23 F. Radu , A. Vorobiev , J. Major , H. Humblot , K. Westerholt , H. Zabel

In this article, we report on inelastic neutron scattering measurements on a quasi-1D antiferromagnet BaCo$_2$V$_2$O$_8$ under a transverse magnetic field applied along the (0,1,0) direction. Combining results of inelastic neutron…

Strongly Correlated Electrons · Physics 2024-07-30 Xiao Wang , Konrad Puzniak , Karin Schmalzl , C. Balz , M. Matsuda , Akira Okutani , M. Hagiwara , Jie Ma , Jianda Wu , Bella Lake

Kitaev interactions underlying a quantum spin liquid have been long sought, but experimental data from which their strengths can be determined directly is still lacking. Here, by carrying out inelastic neutron scattering measurements on…

This work reports the synthesis, structure and magnetic properties of the single crystal of a facile spin 1/2 one dimensional Heisenberg antiferromagnet bis(4-aminopyridinium) bis(oxalato)cuprate(II) dihydrate, (C 5 H 7 N 2 ) 2 [Cu(C 2 O 4…

Ba3Yb2Zn5O11 is unique among breathing pyrochlore compounds for being in the nearly decoupled limit where inter-tetrahedron interactions are weak, hosting isolated clusters or "molecular magnet" like tetrahedra of magnetic ytterbium (Yb3+)…