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We show theoretically that it is possible to create and manipulate a pair of bound states in continuum in ultracold atoms by two lasers in the presence of a magnetically tunable Feshbach resonance. These bound states are formed due to…

Atomic and Molecular Clusters · Physics 2016-09-15 Bimalendu Deb , G. S. Agarwal

Photoionization spectroscopy of cold cesium dimers obtained by photoassociation of cold atoms in a magneto-optical trap is reported here. In particular, we report on the observation and on the spectroscopic analysis of all the excited…

We report on the state-selective detection of near-dissociation ultracold KRb molecules in the ground $X^1\Sigma^+$ state and the metastable $a^3\Sigma^+$ state. The molecules are produced by photoassociation of ultracold atoms followed by…

Atomic Physics · Physics 2009-11-11 D. Wang , E. E. Eyler , P. L. Gould , W. C. Stwalley

The creation of ultracold molecules is currently limited to diatomic species. In this letter we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus…

Atomic Physics · Physics 2015-09-02 Jesús Pérez-Ríos , Maxence Lepers , Olivier Dulieu

We produce an ultracold and dense sample of rovibronic ground state Cs_2 molecules close to the regime of quantum degeneracy, in a single hyperfine level, in the presence of an optical lattice. The molecules are individually trapped, in the…

Long-range metastable molecules consisting of two cesium atoms in high Rydberg states have been observed in an ultracold gas. A sequential three-photon two-color photoassociation scheme was employed to form these molecules in states which…

Atomic Physics · Physics 2016-11-17 Heiner Saßmannshausen , Johannes Deiglmayr

We report the production of ultracold RbCs molecules in the rovibronic ground state, i.e., $X^1\Sigma^+ (v=0, J=0)$, by short-range photoassociation to the $2^3\Pi_{0}$ state followed by spontaneous emission. We use narrowband depletion…

Atomic Physics · Physics 2015-06-22 Toshihiko Shimasaki , Michael Bellos , C. D. Bruzewicz , Zack Lasner , David DeMille

A theoretical model is proposed for the formation of ultracold ground-state triatomic molecules in weakly bound energy levels. The process is driven by the electric component of a microwave field, which induces the association of an…

Atomic Physics · Physics 2026-01-16 Baraa Shammout , Leon Karpa , Silke Ospelkaus , Eberhard Tiemann , Olivier Dulieu

Optical Feshbach resonances [Phys. Rev. Lett. 94, 193001 (2005)] and pump-dump photoassociation with short laser pulses [Phys. Rev. A 73, 033408 (2006)] have been proposed as means to coherently form stable ultracold alkali dimer molecules.…

Atomic Physics · Physics 2009-01-05 Christiane P. Koch

We demonstrate that judicious shaping of a nanosecond-time-scale frequency chirp can dramatically enhance the formation rate of ultracold $^{87}$Rb$_{2}$ molecules. Starting with ultracold $^{87}$Rb atoms, we apply pulses of…

Atomic Physics · Physics 2016-02-26 J. L. Carini , S. Kallush , R. Kosloff , P. L. Gould

In a combined experimental and theoretical effort, we demonstrate a novel type of dipolar system made of ultracold bosonic dipolar molecules with large magnetic dipole moments. Our dipolar molecules are formed in weakly bound Feshbach…

We describe experiments and associated quantum simulations involving the production of ultracold $^{87}$Rb$_{2}$ molecules with nanosecond pulses of frequency-chirped light. With appropriate chirp parameters, the formation is dominated by…

Atomic Physics · Physics 2016-06-07 J. L. Carini , S. Kallush , R. Kosloff , P. L. Gould

We investigate the formation of ultracold NaCs molecules by photoassociation of Na and Cs atoms.

Chemical Physics · Physics 2010-08-09 Xuan Li

We demonstrate the formation of a single RbCs molecule during the merging of two optical tweezers, one containing a single Rb atom and the other a single Cs atom. Both atoms are initially predominantly in the motional ground states of their…

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

Quantum Physics · Physics 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

We report on the creation of heterospecies bosonic molecules, associated from an ultracold Bose-Bose mixture of 41K and 87Rb, by using a resonantly modulated magnetic field close to two Feshbach resonances. We measure the binding energy of…

Other Condensed Matter · Physics 2009-01-29 C. Weber , G. Barontini , J. Catani , G. Thalhammer , M. Inguscio , F. Minardi

We calculate the momentum distribution and the second-order correlation function in momentum space, $g^{(2)}({\bf p},{\bf p}',t)$ for molecular dimers that are coherently formed from an ultracold atomic gas by photoassociation or a Feshbach…

Other Condensed Matter · Physics 2009-11-10 D. Meiser , C. P. Search , P. Meystre

We observe that when an ultracold ground state cesium (Cs) atom becomes bound within the electronic cloud of an extended Cs electronic orbit, ultralong-range molecules with giant (kilo-Debye) permanent electric dipole moments form. Large…

Atomic Physics · Physics 2015-06-23 Donald Booth , Seth Rittenhouse , Jin Yang , Hossein Sadeghpour , James Shaffer

We report on the creation of ultracold 84Sr2 molecules in the electronic ground state. The molecules are formed from atom pairs on sites of an optical lattice using stimulated Raman adiabatic passage (STIRAP). We achieve a transfer…

Quantum Gases · Physics 2012-09-18 Simon Stellmer , Benjamin Pasquiou , Rudolf Grimm , Florian Schreck

Since the realization of Bose-Einstein condensates (BEC) in atomic gases an experimental challenge has been the production of molecular gases in the quantum regime. A promising approach is to create the molecular gas directly from an…

Condensed Matter · Physics 2009-11-10 C. A. Regal , C. Ticknor , J. L. Bohn , D. S. Jin