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We derive the first two moment sum rules of the conduction electron retarded self-energy for both the Falicov-Kimball model and the Hubbard model coupled to an external spatially uniform and time-dependent electric field (this derivation…

Strongly Correlated Electrons · Physics 2008-08-14 V. Turkowski , J. K. Freericks

The dynamics of an electronic system interacting with an electromagnetic field is investigated within mixed quantum-classical theory. Beyond the classical path approximation (where we ignore all feedback from the electronic system on the…

Chemical Physics · Physics 2019-02-11 Hsing-Ta Chen , Tao E. Li , Maxim Sukharev , Abraham Nitzan , Joseph E. Subotnik

The essential quantum many-body physics of an ultracold quantum gas relies on the single-particle Green's functions.\ We demonstrate that it can be extracted by the spectrum of electromagnetically induced transparency (EIT).\ The…

Quantum Gases · Physics 2014-11-03 H. H. Jen , Daw-Wei Wang

Managing light-matter interactions on timescales faster than the loss of electronic coherence is key for achieving full quantum control of the final products in solid-solid transformations. In this work, we demonstrate coherent electronic…

We present a construction of a mean-field theory for thermodynamic and spectral properties of correlated electrons reliable in the strong-coupling limit. We introduce an effective interaction determined self-consistently from the reduced…

Strongly Correlated Electrons · Physics 2017-04-19 Václav Janiš , Vladislav Pokorný , Anna Kauch

Transition metal complexes for photochemical applications often feature a high density of electron-vibrational states characterized by nonadiabatic and spin-orbit couplings. Overall, the dynamics after photoexcitation is shaped by rapid…

Chemical Physics · Physics 2023-05-16 Olga Bokareva , Oliver Kühn

We consider the dependence of the electron transfer in photosynthetic complexes on correlation properties of random fluctuations of the protein environment. The electron subsystem is modeled by a finite network of connected electron…

Biological Physics · Physics 2015-06-23 Alexander I. Nesterov , Gennady P. Berman

We use nonequilibrium dynamical mean-field theory in combination with a recently implemented strong-coupling impurity solver to investigate the relaxation of a Mott insulator after a laser excitation with frequency comparable to the Hubbard…

Strongly Correlated Electrons · Physics 2013-05-29 Martin Eckstein , Philipp Werner

Time-resolved photoemission orbital tomography (tr-POT) offers unique possibilities for tracing molecular electron dynamics. The recorded pump-induced changes of the angle-resolved photoemission intensities allow to characterize unoccupied…

We present an overview of electronic device modeling using non-equilibrium Green function techniques. The basic approach developed in the early 1970s has become increasingly popular during the last 10 years. The rise in popularity was…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Roger K. Lake , Rajeev R. Pandey

Ultrafast optical excitation of metals induces a non-equilibrium energy distribution in the electronic system, with a characteristic step-structure determined by Pauli blocking. On a femtosecond timescale, electron-electron scattering…

Recent advancements in time-resolved electron and photon detection enable novel correlative measurements of electrons and their associated cathodoluminescence (CL) photons within a transmission electron microscope. These studies are pivotal…

Simulating electron-ion dynamics using time-dependent density functional theory within an Ehrenfest dynamics scheme can be done in two ways that are in principle exact and identical: propagating time-dependent electronic Kohn-Sham equations…

Chemical Physics · Physics 2021-07-01 Lionel Lacombe , Neepa T. Maitra

A method for deriving quantum kinetic equations with initial correlations is developed on the basis of the nonequilibrium Green's function formalism. The method is applicable to a wide range of correlated initial states described by…

Statistical Mechanics · Physics 2009-10-31 V. G. Morozov , G. Röpke

We explore a new fashion, named energy-resolved population image (EPI), to represent on an equal footing the temporary electronic transition and nuclear motion during laser-molecular interaction. By using the EPI we have intuitively…

Atomic and Molecular Clusters · Physics 2015-06-19 Kunlong Liu , Pengfei Lan , Cheng Huang , Qingbin Zhang , Peixiang Lu

We use a non-Markovian master equation to describe the transport of Coulomb interacting electrons through an electromagnetic cavity with one quantized photon mode. The central system is a finite parabolic quantum wire that is coupled weakly…

Mesoscale and Nanoscale Physics · Physics 2012-03-15 Vidar Gudmundsson , Olafur Jonasson , Chi-Shung Tang , Hsi-Sheng Goan , Andrei Manolescu

Time-dependent (current) density functional theory for many-electron systems strongly coupled to quantized electromagnetic modes of a microcavity is proposed. It is shown that the electron-photon wave function is a unique functional of the…

Mesoscale and Nanoscale Physics · Physics 2013-12-10 I. V. Tokatly

We study the dynamics of the Fermi-Hubbard model driven by a time-periodic modulation of the interaction within nonequilibrium Dynamical Mean-Field Theory. For moderate interaction, we find clear evidence of thermalization to a genuine…

Strongly Correlated Electrons · Physics 2018-05-09 Francesco Peronaci , Marco Schiró , Olivier Parcollet

A strong-coupling expansion for models of correlated electrons in any dimension is presented. The method is applied to the Hubbard model in $d$ dimensions and compared with numerical results in $d=1$. Third order expansion of the Green…

Strongly Correlated Electrons · Physics 2009-10-30 Stéphane Pairault , David Sénéchal , A. -M. S. Tremblay

We study theoretically the simultaneous, photo-induced two-particle excitations of strongly correlated systems on the basis of the Hubbard model. Under certain conditions specified in this work, the corre- sponding transition probability is…

Strongly Correlated Electrons · Physics 2015-05-18 B. D. Napitu , J. Berakdar