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Imaging the quantum motion of electrons not only in real-time, but also in real-space is essential to understand for example bond breaking and formation in molecules, and charge migration in peptides and biological systems. Time-resolved…

Atomic Physics · Physics 2012-07-20 Gopal Dixit , Oriol Vendrell , Robin Santra

Time-resolved photoemission spectroscopy is the key technique to probe the real-time non-equilibrium dynamics of electronic states. Theoretical predictions of the time dependent spectral function for realistic systems is however, a…

Computational Physics · Physics 2024-05-24 Cian Reeves , Vojtech Vlcek

The interaction of electrons with quantized phonons and photons underlies the ultrafast dynamics of systems ranging from molecules to solids, and it gives rise to a plethora of physical phenomena experimentally accessible using…

Strongly Correlated Electrons · Physics 2021-07-21 Daniel Karlsson , Robert van Leeuwen , Yaroslav Pavlyukh , Enrico Perfetto , Gianluca Stefanucci

Time-resolved photoemission spectroscopy provides a unique and direct way to explore the real-time nonequilibrium dynamics of electrons and holes. The formal theory of the spectral function evolution requires inclusion of electronic…

Materials Science · Physics 2025-05-09 Thomas Blommel , Enrico Perfetto , Gianluca Stefanucci , Vojtěch Vlček

We study the nonequilibrium dynamics of photoinduced phase transitions in charge ordered (CO) systems with a strong electron-lattice interaction and analyze the interplay between electrons, periodic lattice distortions, and a phonon thermal…

Strongly Correlated Electrons · Physics 2018-03-22 Linghua Zhu , Tsezar F. Seman , Michel van Veenendaal , Keun Hyuk Ahn

Recent experiments access the time-resolved photoelectron signal originating from plasmon satellites in correlated materials and address their build-up and decay in real time. Motivated by these developments, we present the Kadanoff-Baym…

Strongly Correlated Electrons · Physics 2016-02-24 Michael Schüler , Jamal Berakdar , Yaroslav Pavlyukh

One of the challenges in many-body physics is determining the effects of phonons on strongly correlated electrons. The difficulty arises from strong correlations at differing energy scales -- for band metals, Migdal-Eliashberg theory…

Strongly Correlated Electrons · Physics 2021-10-08 R. D. Nesselrodt , J. K. Freericks

The spinless Falicov-Kimball model exhibits outside the particle-hole symmetric point different stable nonhomogeneous charge orderings. These include the well known charge stripes and a variety of orderings with phase separated domains,…

Strongly Correlated Electrons · Physics 2020-05-07 Rudolf Smorka , Martin Žonda , Michael Thoss

The competition between electron localization and de-localization in Mott insulators underpins the physics of strongly-correlated electron systems. Photo-excitation, which re-distributes charge between sites, can control this many-body…

Strongly Correlated Electrons · Physics 2015-08-05 S. Wall , D. Brida , S. R. Clark , H. P. Ehrke , D. Jaksch , A. Ardavan , S. Bonora , H. Uemura , Y. Takahashi , T. Hasegawa , H. Okamoto , G. Cerullo , A. Cavalleri

The time-dependent thermopower is analyzed through an interacting quantum dot coupled to a time-dependent gate voltage and under the influence of an external magnetic field using the Keldysh nonequilibrium Green's function formalism. Formal…

Mesoscale and Nanoscale Physics · Physics 2012-06-12 M. Bagheri Tagani , H. Rahimpour Soleimani

Time- and angle-resolved photoemission spectroscopy accesses the ultrafast evolution of quasiparticles and many-body interactions in solid-state systems. However, the momentum- and energy-resolved transient photoemission intensity may not…

We put forward a gauge-invariant theoretical framework for studying time-resolved thermoelectric transport in an arbitrary multiterminal electronic quantum system described by a non-interacting tight-binding model. The system is driven out…

Mesoscale and Nanoscale Physics · Physics 2020-06-18 Adel Kara Slimane , Phillipp Reck , Geneviève Fleury

Nonequilibrium quantum mechanics can be solved with the Keldysh formalism, which evolves the quantum mechanical states forward in time in the presence of a time-dependent field, and then evolves them backward in time, undoing the effect of…

Strongly Correlated Electrons · Physics 2007-05-23 J. K. Freericks , V. Turkowski , V. Zlatic

We derive formal expressions of time-dependent energy and heat currents through a nanoscopic device using the Keldysh nonequilibrium Green function technique. Numerical results are reported for a metal/dot/metal junction where the dot level…

Mesoscale and Nanoscale Physics · Physics 2012-05-16 Adeline Crépieux , Fedor Simkovic , Benjamin Cambon , Fabienne Michelini

We report an exhaustive study of the performance of different variants of Green function methods for the spherium model in which two electrons are confined to the surface of a sphere and interact via a genuine long-range Coulomb operator.…

Chemical Physics · Physics 2018-07-23 Pierre-François Loos , Pina Romaniello , J. A. Berger

Floquet engineering offers a powerful route to enhance emission in time-modulated media. Here, we investigate the influence of time-modulated permittivity in silicon carbide on its intensity spectrum. We consider both the nonequilibrium…

Mesoscale and Nanoscale Physics · Physics 2026-02-27 Yuhua Ren , Hui Pan , Jian-Sheng Wang

The dynamics of electrons in the presence of a positive ion is considered for conditions of weak electron-electron couping but strong electron-ion coupling. The equilibrium electron density and electric field time correlation functions are…

Statistical Mechanics · Physics 2007-05-23 James W. Dufty , Ilya V. Pogorelov , Bernard Talin , Annette Calisti

We investigate a photoinduced insulator-metal transition in the Falicov-Kimball model with the dynamical mean-field theory (DMFT) extended to nonequilibrium systems in periodic modulations in time. When the photon energy of the pump light…

Strongly Correlated Electrons · Physics 2015-05-13 Naoto Tsuji , Takashi Oka , Hideo Aoki

A nonequilibrium Green's functions (NEGF) approach for spatially inhomogeneous, strongly correlated artificial atoms is presented and applied to compute the time-dependent properties while starting from a (correlated) initial few-electron…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 K Balzer , M Bonitz

The effect of correlated hopping on the charge and heat transport of strongly correlated particles is studied for the Falicov-Kimball model on the Bethe lattice. Exact solutions for the one particle density of states (DOS) and two particle…

Strongly Correlated Electrons · Physics 2017-03-29 D. A. Dobushovskyi , A. M. Shvaika , V. Zlatić