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Nowadays powerful X-ray sources like synchrotrons and free-electron lasers are considered as ultimate tools for probing microscopic properties in materials. However, the correct interpretation of such experiments requires a good…

Materials Science · Physics 2018-02-28 B. Ruta , F. Zontone , Y. Chushkin , G. Baldi , G. Pintori , G. Monaco , B. Rufflé , W. Kob

Over the past decade, ultrafast electron dynamics in the solid state have been extensively studied using various strong light-matter interaction techniques, such as high-harmonic generation. These studies lead to multiple interpretations of…

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

Refraction is a well-known optical phenomenon that alters the direction of light waves propagating through matter. Microscopes, lenses and prisms based on refraction are indispensable tools for controlling the properties of light beams at…

The ion heating mechanism in the context of laser interacting with plasma immersed in a strong magnetic field is studied. The magnetic field is chosen to be strong for laser electromagnetic field propagation inside the plasma to be governed…

The goal of the present article is to review the major developments that have led to the current understanding of molecule-field interactions and experimental methods for manipulating molecules with electromagnetic fields. Molecule-field…

Atomic Physics · Physics 2013-09-18 Mikhail Lemeshko , Roman V. Krems , John M. Doyle , Sabre Kais

Laser-driven rescattering of electrons is the basis of many strong-field phenomena in atoms and molecules. Here, we will show how this mechanism operates in extended atomic systems, giving rise to effective energy absorption. Rescattering…

Atomic and Molecular Clusters · Physics 2008-04-07 Ulf Saalmann , Jan M. Rost

A new perspective on how to manipulate molecules by means of very strong laser pulses is emerging with insights from the so-called light-induced potentials, which are the adiabatic potential energy surfaces of molecules severely distorted…

Chemical Physics · Physics 2016-03-03 Bo Y. Chang , Ignacio R. Sola , Seokmin Shin

Absorption covers the physical processes which convert intense photon flux into energetic particles when a high-power laser illuminates optically-thick matter. It underpins important petawatt-scale applications today, e.g., medical-quality…

Approaching energy coupling in laser-irradiated metals, we point out the role of electron-electron collision as an efficient control factor for ultrafast optical absorption. The high degree of laser-induced electron-ion nonequilibrium…

We explore the coherent control of nonlinear absorption of intense laser fields in four-level atomic systems. For instance, in a four-level ladder system, a coupling field creates electromagnetically induced transparency (EIT) with…

Quantum Physics · Physics 2016-09-05 Pardeep Kumar , Shubhrangshu Dasgupta

Modern X-ray spectroscopy has proven itself as a robust tool for probing the electronic structure of atoms in complex environments. Despite working on energy scales that are much larger than those corresponding to nuclear motions, taking…

Chemical Physics · Physics 2017-06-28 Sven Karsten , Sergey I. Bokarev , Saadullah G. Aziz , Sergei D. Ivanov , Oliver Kühn

A deep understanding of molecular photo-transformations is challenging because of the complex interaction between the configurations of electrons and nuclei. An initial optical excitation dissipates energy into electronic and structural…

We have studied the Stark effect in the soft x-ray region for various small molecules by calculating the field-dependent x-ray absorption spectra. This effect is explained in terms of the response of molecular orbitals (core and valence),…

Chemical Physics · Physics 2025-03-26 Avdhoot Datar , Catherine Wright , Devin A. Matthews

Upcoming high-intensity laser systems will be able to probe the quantum-induced nonlinear regime of electrodynamics. So far unobserved QED phenomena such as the discovery of a nonlinear response of the quantum vacuum to macroscopic…

High Energy Physics - Phenomenology · Physics 2009-10-29 Holger Gies

High resolution spectroscopic observations of Seyfert galaxies with Chandra and XMM-Newton allows us to study the detailed ionization and thermal structures of the X-ray absorbing/emitting material in the circumnuclear environment. The vast…

X-ray absorption spectroscopy and X-ray magnetic circular dichroism have long served as indispensable tools for probing the electronic and magnetic properties of transition-metal compounds with elemental selectivity. In recent years, the…

Materials Science · Physics 2026-05-11 Hiroki Wadati , Kohei Yamamoto , Kohei Yamagami

Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…

Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the…

Atomic Physics · Physics 2021-09-03 Liat Levin , Daniel M. Reich , Moran Geva , Ronnie Kosloff , Christiane P. Koch , Zohar Amitay