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High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4 K, terbium titanate is a highly…

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

Er_2Ti_2O_7 has been suggested to be a realization of the frustrated < 111 > XY pyrochlore lattice antiferromagnet, for which theory predicts fluctuation-induced symmetry breaking in a highly degenerate ground state manifold. We present a…

We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…

The spin dynamics in the geometrically frustrated pyrochlore antiferromagnet $\rm Gd_2Sn_2O_7$ is studied by means of the electron spin resonance. In the ordered phase ($T_N = 1$ K), we have detected three gapped resonance modes. Their…

Strongly Correlated Electrons · Physics 2013-05-29 S. S. Sosin , L. A. Prozorova , P. Bonville , M. E. Zhitomirsky

Geometric frustration inhibits magnetic systems from ordering, opening a window to unconventional phases of matter. The paradigmatic frustrated lattice in three dimensions to host a spin liquid is the pyrochlore, although there remain few…

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

We report on the origin of spin freezing in the disordered fluorite Ho$_2$Zr$_2$O$_7$. The system is investigated by low-temperature heat capacity as well as by DC and AC magnetization. While the system does not show a long-range magnetic…

Strongly Correlated Electrons · Physics 2024-07-19 A. Elghandour , Sheeta , C. S. Yadav , R. Klingeler

The charge ordered structure of ions and vacancies characterizing rare-earth pyrochlore oxides serves as a model for the study of geometrically frustrated magnetism. The organization of magnetic ions into networks of corner-sharing…

We report synchrotron radiation diffraction and muon spin rotation (muSR) measurements on the frustrated pyrochlore magnet Tb2Ti2O7. The powder diffraction study of a crushed crystal fragment does not reveal any structural change down to 4…

Strongly Correlated Electrons · Physics 2014-12-22 P. Dalmas de Reotier , A. Yaouanc , A. Bertin , C. Marin , S. Vanishri , D. Sheptyakov , A. Cervellino , B. Roessli , C. Baines

A frustrated system is one whose symmetry precludes the possibility that every pairwise interaction (``bond'') in the system can be satisfied at the same time. Such systems are common in all areas of physical and biological science. In the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Steven T. Bramwell , Michel J. -P. Gingras

We report the physical properties of Tb2Hf2O7 based on ac magnetic susceptibility \chi_ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H), and heat capacity C_p(T) measurements combined with muon spin relaxation…

Strongly Correlated Electrons · Physics 2018-03-06 V. K. Anand , L. Opherden , J. Xu , D. T. Adroja , A. D. Hillier , P. K. Biswas , T. Herrmannsdörfer , M. Uhlarz , J. Hornung , J. Wosnitza , E. Canevet , B. Lake

Muon spin relaxation on Nd$_2$Ti$_2$O$_7$ (NTO) and NdLaTi$_2$O$_7$ (NLTO) compounds are presented. The time spectra for both compounds are as expected for the paramagnetic state at high temperatures, but deviate from the exponential…

Strongly Correlated Electrons · Physics 2014-10-21 Hanjie Guo , Hui Xing , Jun Tong , Qian Tao , Isao Watanabe , Zhu-an Xu

Structural disorder in the magnetically frustrated pyrochlore system leads to intriguing magnetic states. We present the thermodynamic behavior and short range magnetic correlations in Tb$_{2}$Zr$_{2}$O$_{7}$ and…

Strongly Correlated Electrons · Physics 2026-04-16 Sujata Singh , Leon Carstens , M. Duc Le , R. Klingeler , C. S. Yadav

The frustrated pyrochlore magnet Yb$_2$Ti$_2$O$_7$ has the remarkable property that it orders magnetically, but has no propagating magnons over wide regions of the Brillouin zone. Here we use inelastic neutron scattering to follow how the…

Strongly Correlated Electrons · Physics 2017-08-08 J. D. Thompson , P. A. McClarty , D. Prabhakaran , I. Cabrera , T. Guidi , R. Coldea

Although materials that exhibit nearest-neighbor-only antiferromagnetic interactions and geometrical frustration theoretically should not magnetically order in the absence of disorder, few such systems have been observed experimentally. One…

Strongly Correlated Electrons · Physics 2016-08-31 S. -W. Han , J. S. Gardner , C. H. Booth

We report neutron diffraction measurements of the magnetic structures in two pyrochlore iridates, Yb2Ir2O7 and Lu2Ir2O7. Both samples exhibit the all-in-all-out magnetic structure on the Ir4+ sites below TN~ 150,K, with a low temperature…

Electron spin resonance study of frustrated pyrochlore Gd2Ti2O7 is performed in a wide frequency band for a temperature range 0.4-30 K, which covers paramagnetic and magnetically ordered phases. The paramagnetic resonance reveals the…

Strongly Correlated Electrons · Physics 2012-02-02 S. S. Sosin , A. I. Smirnov , L. A. Prozorova , G. Balakrishnan , M. E. Zhitomirsky

Strongly correlated electron systems host a variety of poorly understood correlations in their high temperature normal state. Unlike ordered phases defined by order parameters, these normal state phases are often defined through…

Inelastic neutron scattering is used to characterize spin fluctuations in the $d$-electron heavy fermion spinel $\rm LiV_2O_4$. The spin relaxation rate, $\Gamma_Q$, for $Q=0.6$ \AA$^{-1}$ is 1.5(1) meV at low temperatures and increases…

Strongly Correlated Electrons · Physics 2009-11-07 S. -H. Lee , Y. Qiu , C. Broholm , Y. Ueda , J. J. Rush