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We describe a molecular dynamics framework for the direct calculation of the short-ranged structural forces underlying grain-boundary premelting and grain-coalescence in solidification. The method is applied in a comparative study of (i) a…

Materials Science · Physics 2015-05-14 Saryu Fensin , David Olmsted , Dorel Buta , Mark Asta , Alain Karma , J. J. Hoyt

We investigate the ability of a multi-order parameter phase field model with obstacle potentials to describe grain boundary premelting in equilibrium situations. In agreement with an energetic picture we find that the transition between dry…

We predict the structural interaction of crystalline solid-melt interfaces using amplitude equations which are derived from classical density functional theory or phase-field-crystal modeling. The solid ordering decays exponentially on the…

Materials Science · Physics 2015-06-12 Robert Spatschek , Ari Adland , Alain Karma

We investigate a model which couples diffusional melting and nanoscale structural forces via a combined nano-mesoscale description. Specifically, we obtain analytic and numerical solutions for melting processes at grain boundaries…

Materials Science · Physics 2015-06-19 C. Hüter , F. Twiste , R. Spatschek , J. Neugebauer , E. A. Brener

We characterize both analytically and numerically short-range forces between spatially diffuse interfaces in multi-phase-field models of polycrystalline materials. During late-stage solidification, crystal-melt interfaces may attract or…

Materials Science · Physics 2015-05-14 N. Wang , R. Spatschek , A. Karma

Using statistical field theory supplemented with molecular dynamics simulations, we consider premelting on the surface of ice as a generic consequence of broken hydrogen bonds at the boundary between the condensed and gaseous phases. A…

Statistical Mechanics · Physics 2015-06-22 David T. Limmer , David Chandler

This paper explores the friction forces encountered by droplets on non-wetting surfaces, specifically focusing on superhydrophobic and superheated substrates. Employing a combination of experimental techniques, including inclined plane…

We describe an optical scattering study of grain boundary premelting in water ice. Ubiquitous long ranged attractive polarization forces act to suppress grain boundary melting whereas repulsive forces originating in screened Coulomb…

Materials Science · Physics 2013-05-23 E. S. Thomson , Hendrik Hansen-Goos , L. A. Wilen , J. S. Wettlaufer

In light of the race towards macroscale superlubricity of graphitic contacts, the effect of grain boundaries on their frictional properties becomes of central importance. Here, we elucidate the unique frictional mechanisms characterizing…

Mesoscale and Nanoscale Physics · Physics 2020-08-04 Xiang Gao , Wengen Ouyang , Oded Hod , Michael Urbakh

The curvature dependence of interfacial free energy, which is crucial in quantitatively predicting nucleation kinetics and the stability of bubbles and droplets, can be described in terms of the Tolman length {\delta}. For solid-liquid…

Statistical Mechanics · Physics 2018-08-01 Bingqing Cheng , Michele Ceriotti

The complicated dynamics of the contact line of a moving droplet on a solid substrate often hamper the efficient modeling of microfluidic systems. In particular, the selection of the effective boundary conditions, specifying the contact…

Microdrop impact and spreading phenomena are explored as an interface formation process using a recently developed computational framework. The accuracy of the results obtained from this framework for the simulation of high deformation…

Fluid Dynamics · Physics 2015-06-04 J. E. Sprittles , Y. D. Shikhmurzaev

The influence of the external pressure and surface energy on the wetting transition at nanotextured interfaces is studied using molecular dynamics and continuum simulations. The surface roughness of the composite interface is introduced via…

Soft Condensed Matter · Physics 2018-07-12 Bishal Bhattarai , Nikolai V. Priezjev

We present a new model of surface transport in premelted films that is applicable to a wide range of materials close to their melting point. We illustrate its use by applying it to the evolution of a grain boundary groove in a high vapour…

Fluid Dynamics · Physics 2012-01-13 Robert W. Style , M. Grae Worster

Throughout computational science, there is a growing need to utilize the continual improvements in raw computational horsepower to achieve greater physical fidelity through scale-bridging over brute-force increases in the number of mesh…

We investigate the effective coupling between heat and fluid dynamics within a thin fluid layer in contact with a solid structure via a rough surface. Moreover, the opposing vertical surfaces of the thin layer are in relative motion. This…

Analysis of PDEs · Mathematics 2026-04-17 Tom Freudenberg , Michael Eden

Liquid wetting of a surface is omnipresent in nature and the advance of micro-fabrication and assembly techniques in recent years offers increasing ability to control this phenomenon. Here, we identify how surface roughness influences the…

The mathematical modelling of species transport in the turbulent boundary layer of fluids that precipitate on the wall, is an important topic at the heart of one of the biggest challenges in efficient energy utilization in all process…

Fluid Dynamics · Physics 2017-03-22 S. G. Johnsen , T. M. Pääkkönen , S. Andersson , S. T. Johansen , B. Wittgens

We report on the onset of fluid entrainment when a contact line is forced to advance over a dry solid of arbitrary wettability. We show that entrainment occurs at a critical advancing speed beyond which the balance between capillary,…

Soft Condensed Matter · Physics 2015-06-16 Rodrigo Ledesma-Aguilar , Aurora Hernández-Machado , Ignacio Pagonabarraga

Using Lifshitz theory we assess the role of van der Waals forces at interfaces of ice and water. The results are combined with measured structural forces from computer simulations to develop a quantitative model of the surface free energy…

Soft Condensed Matter · Physics 2022-11-14 Juan Luengo-Marquez , Fernando Izquierdo-Ruiz , Luis G. MacDowell
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