Related papers: Probing Dynamics of Single Molecules: Non-linear S…
This work models the propagation of an optical pulse in a 4-level atomic system in the electromagnetic induced transparency regime. By demonstrating that linear and nonlinear optical properties can be externally controlled and tailored by a…
Single-molecule tracking is a powerful way to look at the dynamic organization of plasma membranes. However, there are some limitations to its use. For example, it was recently observed, using numerical simulation, that time-averaging…
Nonlinear effects in pulse propagation through a medium consisting of four-level double-$\Lambda$-type systems are studied theoretically. We apply three continous-wave driving fields and a pulsed probe field such that they form a closed…
Non-linear wave-driven processes in plasmas are normally described by either a monochromatic pump wave that couples to other monochromatic waves, or as a random phase wave coupling to other random phase waves. An alternative approach…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…
We analyze Photo-Electron Spectra (PES) for a variety of excitation mechanisms from a simple mono-frequency laser pulse to involved combination of pulses as used, e.g., in attosecond experiments. In the case of simple pulses, the peaks in…
Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…
Single-molecule pulling techniques have emerged as versatile tools for probing the noncovalent forces holding together the secondary and tertiary structure of macromolecules. They also constitute a way to study at the single-molecule level…
Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…
The strong non-linearity plays a significant role in physics, particularly, in designing novel quantum sources of light and matter as well as in quantum chemistry or quantum biology. In simple systems, the photon-photon interaction can be…
Soliton molecules are the manifestation of attractive and repulsive interaction between optical pulses mediated by a nonlinear medium. However, the formation and breakup of soliton molecules are difficult to observe due to the transient…
Spectroscopy has played the key role in revealing, and thereby understanding, the structure of atoms and molecules. A central drive in this field is the pursuit of higher precision and accuracy so that ever more subtle effects might be…
Single-beam spectrally controlled (SBSC) two-dimensional (2D) Raman spectroscopy is a unique 2D vibrational measurement technique utilizing trains of short pulses that are generated from a single broadband pulse by pulse shaping. This…
It has been established for some time that high-power pump can trap a probe beam of lower intensity that is simultaneously propagating in a Kerr-type optical medium, inducing a focusing of the probe with the emergence of modes displaying…
This is the first in a series of two papers investigating the effect of electron-phonon coupling in two-dimensional Fourier transformed electronic spectroscopy. We present a series of one- and two-dimensional nonlinear spectroscopic…
The effect of the pulse-shape on pump-probe spectroscopies is examined for the simplest model of noninteracting fermions on an infinite-dimensional hypercubic lattice. The probe-modified density of states follows the time evolution of the…
Photon statistical measurements on a semiconductor microlaser, obtained using single-photon counting techniques, show that a newly discovered spontaneous pulsed emission regime possesses superthermal statistical properties. The observed…
We present a new scheme for performing optical spectroscopy on single molecules. A glass capillary with a diameter of 600 nm filled with an organic crystal tightly guides the excitation light and provides a maximum spontaneous emission…
The emergence of confined structures and pattern formation are exceptional manifestations of concurring nonlinear interactions found in a variety of physical, chemical and biological systems[1]. Optical solitons are a hallmark of extreme…
We derive the moment generating function for photon emissions from a single molecule driven by laser excitation. The frequencies of the fluoresced photons are explicitly considered. Calculations are performed for the case of a two level dye…