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The formation and rupture of atomic-sized contacts is modelled by means of molecular dynamics simulations. Such nano-contacts are realized in scanning tunnelling microscope and mechanically controlled break junction experiments. These…

Mesoscale and Nanoscale Physics · Physics 2015-01-26 W. Dednam , C. Sabater , M. A. Fernandez , C. Untiedt , J. J. Palacios , M. J. Caturla

Conductance of submicron constrictions of PbTe:Bi was studied up to 8T and between 4.2K and 50mK. The structures were fabricated by electron beam lithography and chemical etching of high--electron mobility films grown by MBE on BaF_2. In…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 G. Grabecki , J. Wrobel , T. Dietl , K. Byczuk , E. Papis , E. Kaminska , A. Piotrowska , G. Springholz , M. Pinczolits , G. Bauer

In this work, we investigate the relative importance of electronic and phononic energy dissipation during the molecular adsorption of CO on Cu(110). Initial sticking probabilities as a function of impact energy for CO impinging at normal…

We present the carrier transport properties in the vicinity of a doping-driven Mott transition observed at a field-effect transistor (FET) channel using a single crystal of the typical two-dimensional organic Mott insulator…

Strongly Correlated Electrons · Physics 2017-01-13 Yoshiaki Sato , Yoshitaka Kawasugi , Masayuki Suda , Hiroshi M. Yamamoto , Reizo Kato

We show that the observed repulsive interaction between CO molecules on the Pt(111) surface can be explained by the coupling of the Pt--CO separation with Pt-Pt coordinates in the substrate. The observed long range of the interaction and…

Condensed Matter · Physics 2009-10-30 R. Brako , D. Sokcevic

We study the interference of interacting electrons in toroidal single-wall carbon nanotubes coupled to metallic electrodes by tunnel junctions. The dc conductance shows resonant features as a function of the gate voltage and the magnetic…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Joerg Rollbuehler , Arkadi A. Odintsov

We present a state-of-the-art first-principles analysis of electronic transport in a Pt nanocontact in the presence of H2 which has been recently reported by Smit et al. in Nature 419, 906 (2002). Our results indicate that at the last…

Materials Science · Physics 2009-11-10 Yamila Garcia , J. J. Palacios , E. San Fabian , J. A. Verges , A. J. Perez-Jimenez , E. Louis

The relaxation dynamics of correlated electron transport (ET) along molecular chains is studied based on a substantially improved numerically exact path integral Monte Carlo (PIMC) approach. As archetypical model we consider a Hubbard chain…

Statistical Mechanics · Physics 2009-11-11 L. Muehlbacher , J. Ankerhold , A. Komnik

Electrical conductance through various nanocontacts between gold electrodes is studied by using the density functional theory, scalar-relativistic pseudopotentials, generalized gradient approximation for the exchange-correlation energy and…

Materials Science · Physics 2009-11-13 O. Lopez-Acevedo , D. Koudela , H. Häkkinen

We report a detailed theoretical study of the bonding and conduction properties of an hydrogen molecule joining either platinum or palladium electrodes. We show that an atomic arrangement where the molecule is placed perpendicular to the…

Materials Science · Physics 2007-05-23 V. M. Garcia-Suarez , A. R. Rocha , S. W. Bailey , C. J. Lambert , S. Sanvito , J. Ferrer

Molecular devices, as future electronics, seek low-resistivity contacts for the energy saving. At the same time, the contacts should intensify desired properties of tailored electronic elements. In this work, we focus our attention on two…

Mesoscale and Nanoscale Physics · Physics 2015-06-02 Malgorzata Wierzbowska , Michal F. Rode , Mikolaj Sadek , Andrzej L. Sobolewski

The magnetic coupling between single Co atoms adsorbed on a copper surface is determined by probing the Kondo resonance using low-temperature scanning tunneling spectroscopy. The Kondo resonance, which is due to magnetic correlation effects…

Strongly Correlated Electrons · Physics 2007-05-23 P. Wahl , P. Simon , L. Diekhoener , V. S. Stepanyuk , P. Bruno , M. A. Schneider , K. Kern

The influence of an intramolecular proton transfer reaction on the conductance of a molecular junction is investigated employing a generic model, which includes the effects of the electric field of the gate and leads electrodes and the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Chriszandro Hofmeister , Pedro B. Coto , Michael Thoss

Using ab initio methods, we examine the the charge distribution at the interface of alpha-alumina-supported Pt films, and we consider the influence of this interface on CO adsorption. We demonstrate that a combination of electrostatic…

Materials Science · Physics 2012-03-12 Valentino R. Cooper , Alexie M. Kolpak , Yashar Yourdshahyan , Andrew M. Rappe

We explore electron transport properties for the model of benzene-1, 4-dithiolate (BDT) molecule and for some other geometric models of benzene molecule attached to two semi-infinite one-dimensional metallic electrodes using the Green's…

Mesoscale and Nanoscale Physics · Physics 2010-04-13 Santanu K. Maiti

Conductance measurements of a molecular wire, contacted between an epitaxial molecule-metal bond and the tip of a scanning tunneling microscope, are reported. Controlled retraction of the tip gradually de-hybridizes the molecule from the…

Strongly Correlated Electrons · Physics 2024-02-05 R. Temirov , A. C. Lassise , F. Anders , F. S. Tautz

Electric-field effect control of two-dimensional electron gases (2-DEG) has enabled the exploration of nanoscale electron quantum transport in semiconductors. Beyond these classical materials, transition metal-oxide-based structures have…

Mesoscale and Nanoscale Physics · Physics 2019-03-29 A. Jouan , G. Singh , E. Lesne , D. C. Vaz , M. Bibes , A. Barthélémy , C. Ulysse , D. Stornaiuolo , M. Salluzzo , S. Hurand , J. Lesueur , C. Feuillet-Palma , N. Bergeal

In atoms spin-orbit coupling (SOC) cannot raise the angular momentum above a maximum value or lower it below a minimum. Here we show that this need not be the case in materials built from nanoscale structures including multi-nuclear…

Strongly Correlated Electrons · Physics 2017-03-15 A. L. Khosla , A. C. Jacko , J. Merino , B. J. Powell

We present a simplified density functional theory (DFT) method to com- pute vertical electron and hole attachment energies to frontier orbitals of molecules absorbed on insulating films supported by a metal substrate. The adsorbate and the…

Mesoscale and Nanoscale Physics · Physics 2017-08-29 Ivan Scivetti , Mats Persson

We consider electronic transport through semiconducting nanowires (W) with spin-orbit interaction (SOI), in a hybrid N-W-N setup where the wire is contacted by normal-metal leads (N). We investigate the conductance behavior of the system as…

Mesoscale and Nanoscale Physics · Physics 2014-12-16 Diego Rainis , Daniel Loss