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To clarify a crucial role of a spin-orbit coupling in the emergence of novel spin-orbital states in $5d$-electron compounds such as Sr$_{2}$IrO$_{4}$, we investigate ground state properties of a $t_{\rm 2g}$-orbital Hubbard model on a…

Strongly Correlated Electrons · Physics 2015-06-17 Hiroaki Onishi

The effect of the spin-orbit coupling on the ground state properties of the square-lattice three-band Hubbard model with a single electron per site is studied by a generalized Hartree-Fock approximation. We calculate the full phase diagram…

Strongly Correlated Electrons · Physics 2024-09-30 Petr A. Igoshev , Danil E. Chizhov , Valentin Yu. Irkhin , Sergey V. Streltsov

Here we report on the low-energy excitations within the paramagnetic spin-orbit insulator Sr$_3$Ir$_2$O$_7$F$_2$ studied via resonant inelastic X-ray scattering, \textit{ab initio} quantum chemical calculations, and model-Hamiltonian…

Strongly Correlated Electrons · Physics 2022-09-26 Zach Porter , Paul M. Sarte , Thorben Petersen , Mary H. Upton , Liviu Hozoi , Stephen D. Wilson

Sr2IrO4 is one of the prime candidates for realizing exotic quantum spin orders owing to the subtle combination of spin-orbit coupling and electron correlation. Sensitive local magnetization measurement can serve as a powerful tool to study…

Materials Science · Physics 2025-03-26 Hyeokjun Heo , Jeongha An , Junyoung Kwon , Kwangrae Kim , Youngoh Son , B. J. Kim , Joonho Jang

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

Strongly Correlated Electrons · Physics 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

Spin-orbit coupling (SOC) in noncentrosymmetric materials is the source of incommensurate magnetic structures. In semiconductors, it drives the Rashba spin splitting and spin momentum locking, while in magnetic insulators based on…

Strongly Correlated Electrons · Physics 2026-01-08 Ryo Makuta , Chisa Hotta

Transition metal compounds with the $(t_{2g})^4$ electronic configuration are expected to be nonmagnetic atomic singlets both in the weakly interacting regime due to spin-orbit coupling, as well as in the Coulomb dominated regime with…

Strongly Correlated Electrons · Physics 2017-01-16 Christopher Svoboda , Mohit Randeria , Nandini Trivedi

Sr$_{3}$Cr$_{2}$O$_{8}$ consist of a lattice of spin-1/2 Cr$^{5+}$ ions, which form hexagonal bilayers and which are paired into dimers by the dominant antiferromagnetic intrabilayer coupling. The dimers are coupled three-dimensionally by…

Metamagnetism in antiferromagnets exhibits distinct critical behaviors and dynamics when invoking spin reversal and rotation. Here we show a 0.05% anisotropic strain suffices to in-situ modulate the metamagnetic critical field of the Mott…

Strongly Correlated Electrons · Physics 2020-07-24 H. Zhang , L. Hao , J. Yang , J. Mutch , Z. Liu , Q. Huang , K. Noordhoek , A. F. May , J. -H. Chu , J. W. Kim , P. J. Ryan , H. D. Zhou , Jian Liu

The spin-orbit coupling (SOC) interactions, electron correlation effects and Hund coupling cooperate and compete with each other, leading to novel properties, quantum phase and non-trivial topological electronic behavior in iridium oxides.…

Strongly Correlated Electrons · Physics 2018-12-19 Xing Ming , Xiangang Wan , Carmine Autieri , Jianfeng Wen , Xiaojun Zheng

We consider spin-orbit coupling effects in Na$_4$Ir$_3$O$_8$, a material in which Ir$^{4+}$ spins form an hyper-kagom\'{e} lattice, a three-dimensional network of corner-sharing triangles. We argue that both low temperature thermodynamic…

Strongly Correlated Electrons · Physics 2008-10-03 Gang Chen , Leon Balents

We derive a quantum spin Hamiltonian of the spin-1/2 zigzag chain realized in a rare earth ytterbium-based magnetic insulator, YbCuS2. This material undergoes a transition at 0.95K to an incommensurate magnetic phase with small moments,…

Strongly Correlated Electrons · Physics 2024-08-02 Hidehiro Saito , Hiroki Nakai , Chisa Hotta

By combining 5d transition-metal oxides showing pronounced spin-orbit interactions and oxide-based heterostructures, we propose rutile-based IrO2/TiO2 superlattices as promising candidates for unconventional electronic properties. By means…

Strongly Correlated Electrons · Physics 2017-02-16 Xing Ming , Kunihiko Yamauchi , Tamio Oguchi , Silvia Picozzi

Sr$_2$IrO$_4$ is an extensively studied spin-orbit coupling induced insulator with antiferromagnetic ground state. The delicate balance between competing energy scales plays crucial role for its low temperature phase, and the route of…

Strongly Correlated Electrons · Physics 2017-10-31 Imtiaz Noor Bhatti , R. S. Dhaka , A. K. Pramanik

Frustration-induced strong quantum fluctuations accompanied by spin-orbit coupling and crystal electric field can give rise to rich and diverse magnetic phenomena associated with unconventional low-energy excitations in rare-earth based…

Strongly Correlated Electrons · Physics 2024-02-13 J. Khatua , S. Bhattacharya , A. M. Strydom , A. Zorko , J. S. Lord , A. Ozarowski , E. Kermarrec , P. Khuntia

Spin-orbit coupling (SOC) often gives rise to interesting electronic and magnetic phases in an otherwise ordinary pool of paramagnetic heavy metal oxides. In presence of strong SOC, assumed to be working in $j$-$j$ coupling regime, 5$d^4$…

We present a novel approach to study the ground state and elementary excitations in compounds where spins and orbitals are entangled by on-site relativistic spin-orbit interaction. The appropriate degrees of freedom are localized states…

Strongly Correlated Electrons · Physics 2010-07-13 Gia-Wei Chern , Natalia Perkins

The ground-state properties of the spin-1/2 antiferromagnetic Heisenberg model with spatially anisotropic couplings on a square lattice are investigated by a spin-rotation-invariant Green's-function approach and by Lanczos diagonalizations…

Strongly Correlated Electrons · Physics 2007-05-23 D. Ihle , C. Schindelin , A. Weisse , H. Fehske

We study the magnetic properties of the adatom systems on a semiconductor surface Si(111):\{C,Si,Sn,Pb\} - ($\sqrt{3} \times \sqrt{3}$). On the basis of all-electron density functional theory calculations we construct effective low-energy…

Strongly Correlated Electrons · Physics 2016-12-28 D. I. Badrtdinov , S. A. Nikolaev , M. I. Katsnelson , V. V. Mazurenko

Spin-orbit entangled magnetic dipoles, often referred to as pseudospins, provide a new avenue to explore novel magnetism inconceivable in the weak spin-orbit coupling limit, but the nature of their low-energy interactions remains to be…