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In spectroscopy, it is conventional to treat pulses much stronger than the linewidth as delta-functions. In NMR, this assumption leads to the prediction that pi pulses do not refocus the dipolar coupling. However, NMR spin echo measurements…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Dale Li , Yanqun Dong , R. G. Ramos , J. D. Murray , K. MacLean , A. E. Dementyev , S. E. Barrett

NMR spin echo measurements of C-13 in C60, Y-89 in Y2O3, and Si-29 in silicon are shown to defy conventional expectations when more that one pi pulse is used. Multiple pi-pulse echo trains may either freeze our or accelerate the decay of…

Quantum Physics · Physics 2007-05-23 Dale Li , A. E. Dementyev , Yanqun Dong , R. G. Ramos , S. E. Barrett

Puzzling anomalies previously observed in multipulse NMR experiments in natural abundance 29Si [A.E. Dementyev, D. Li, K. MacLean, and S.E. Barrett, Phys. Rev. B 68, 153302 (2003)] such as long-lived spin echoes and even-odd asymmetries,…

Statistical Mechanics · Physics 2009-11-11 M. B. Franzoni , P. R. Levstein

We report an observation of extremely long-lived spin states in systems of dipolar-coupled nuclear spins in solids. The 'suspended echo' experiment uses a simple stimulated echo pulse sequence and creates non-equilibrium states which live…

Mesoscale and Nanoscale Physics · Physics 2013-06-17 A. Turanov , A. K. Khitrin

NMR spin echo measurements of $^{29}$Si in Silicon powders have uncovered a variety of surprising phenomena that appear to be independent of doping. These surprises include long tails and even-odd asymmetry in Carr-Purcell-Meiboom-Gill…

Condensed Matter · Physics 2009-11-10 A. E. Dementyev , D. Li , K. MacLean , S. E. Barrett

The application of Carr-Purcell-Meiboom-Gill (CPMG) $\pi-$trains for dynamically decoupling a system from its environment has been extensively studied in a variety of physical systems. When applied to dipolar solids, recent experiments have…

Other Condensed Matter · Physics 2015-06-18 Clark D. Ridge , Lauren F. O'Donnell , Jamie D. Walls

New NMR experiments reveal the origin of the "pseudocoherence" that leads to long tails in some Carr-Purcell-Meiboom-Gill (CPMG) sequences in contrast with the decay of a standard Hahn echo. We showed in [M.B Franzoni and P.R. Levstein,…

Statistical Mechanics · Physics 2008-10-09 Maria Belen Franzoni , Patricia R. Levstein , Jesus Raya , Jerome Hirschinger

Solids and rigid tissues such as bone, ligaments, and tendons, typically appear dark in magnetic resonance imaging (MRI), which is due to the extremely short-lived proton nuclear magnetic resonance (NMR) signals. This short lifetime is due…

Medical Physics · Physics 2013-06-11 Boyang Zhang , Jae-Seung Lee , Anatoly Khitrin , Alexej Jerschow

We demonstrate that CPMG and XYXY decoupling sequences with non-ideal $\pi$ pulses can reduce dipolar interactions between spins of the same species in solids. Our simulations of pulsed electron spin resonance (ESR) experiments show that…

Mesoscale and Nanoscale Physics · Physics 2018-07-16 Evan S. Petersen , A. M. Tyryshkin , K. M. Itoh , Joel W. Ager , H. Riemann , N. V. Abrosimov , P. Becker , H. -J. Pohl , M. L. W. Thewalt , S. A. Lyon

Dense spin ensembles in solids present a natural platform for studying quantum many-body dynamics. Multiple-pulse coherent control can be used to manipulate the magnetic dipolar interaction between the spins to engineer their dynamics.…

Quantum Physics · Physics 2024-12-24 Linta Joseph , Wynter Alford , Chandrasekhar Ramanathan

Recently several long-period radio transients have been discovered, with strongly polarised coherent radio pulses appearing on timescales between tens to thousands of seconds [1,2]. In some cases the radio pulses have been interpreted as…

We study the properties of spin systems realized by cold polar molecules interacting via dipole-dipole interactions in two dimensions. Using a spin wave theory, that allows for the full treatment of the characteristic long-distance tail of…

Quantum Gases · Physics 2012-07-12 David Peter , Steffen Müller , Stefan Wessel , Hans Peter Büchler

Based on a modified Anderson-Weiss approximation (N. Fatkullin, A. Gubaidullin, C. Mattea, S.Stapf, J. Chem. Phys. 137 (2012), 224907) an improved theory of proton spin solid echo in polymer melts is formulated, taking into account…

Chemical Physics · Physics 2015-08-27 N. Fatkullin , A. Lozovoi , C. Mattea , S. Stapf

We show experimentally and describe theoretically how a conventional magnetic resonance Hahn echo sequence can lead to a self-stimulated pulse echo train when an inhomogeneously broadened spin ensemble is coupled to a resonator. Effective…

Quantum Physics · Physics 2020-09-23 Kamanasish Debnath , Gavin Dold , John J. L. Morton , Klaus Mølmer

The work is devoted to the problem of multiple signals of nuclear spin echoes in magnets, excited by a series of radio-frequency (RF) arbitrary duration pulses exceeding the free induction decay time. The quantum-statistical approach based…

Other Condensed Matter · Physics 2012-06-19 M. D Zviadadze , G. I. Mamniashvili , T. O. Gegechkori , A. M. Akhalkatsi , T. A. Gavasheli

It is demonstrated that the time evolution of the electron-nuclear polarization transfer process during pulsed dynamic nuclear polarization (DNP) can be reversed on a microsecond timescale, leading to the observation of DNP echoes. The DNP…

Chemical Physics · Physics 2024-06-28 Nino Wili , Anders B. Nielsen , José P. Carvalho , Niels Chr. Nielsen

Quantum correlations are investigated theoretically in a two-spin system with the dipole-dipole interactions in the NMR multiple-pulse spin-locking experiments. We consider two schemes of the multiple-pulse spin-locking. The first scheme…

Quantum Physics · Physics 2018-02-27 S. A. Gerasev , A. V. Fedorova , E. B. Fel'dman , E. I. Kuznetsova

The ability to probe the spin properties of solid state systems electrically underlies a wide variety of emerging technology. Here, we extend electrical readout of the nuclear spin states of phosphorus donors in silicon to the coherent…

Other Condensed Matter · Physics 2015-05-30 D. R. McCamey , C. Boehme , G. W. Morley , J. van Tol

Electron spin resonance scanning tunneling microscopy (ESR-STM) has become a powerful tool for probing spin dynamics and coherence of individual atoms and molecules on surfaces. In this work, we perform Rabi oscillation and Hahn echo pulse…

Mesoscale and Nanoscale Physics · Physics 2026-03-30 Paul Greule , Wantong Huang , Máté Stark , Kwan Ho Au-Yeung , Christoph Wolf , Soo-hyon Phark , Andreas J. Heinrich , Philip Willke

We note the existence of a set of magnetic field values where a simple Hahn echo sequence refocuses the dynamics of the full dipolar interaction, for spin systems of electron donors in silicon. As the refocussing occurs for both arbitrary…

Quantum Physics · Physics 2014-12-09 T. S. Monteiro
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