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We discuss the relaxation dynamics of a simple lattice gas model for glass-forming systems and show that with increasing density of particles this dynamics slows down very quickly. By monitoring the trajectory of tagged particles we find…

Soft Condensed Matter · Physics 2010-05-07 Pinaki Chaudhuri , Ludovic Berthier , Srikanth Sastry , Walter Kob

We numerically elucidate the microscopic mechanisms controlling the relaxation dynamics of a three-dimensional lattice glass model that has static properties compatible with the approach to a random first-order transition. At low…

Disordered Systems and Neural Networks · Physics 2024-02-09 Yoshihiko Nishikawa , Ludovic Berthier

We study dynamical heterogeneity and glassy dynamics in a kinetically constrained lattice gas model which has both translational and rotational degrees of freedom. We find that the rotational diffusion constant tracks the structural…

Soft Condensed Matter · Physics 2015-06-25 Albert C. Pan

We numerically study the equilibrium relaxation dynamics of a two-dimensional Mari-Kurchan glass model. The tree-like structure of particle interactions forbids both non-trivial structural motifs and the emergence of a complex free-energy…

Disordered Systems and Neural Networks · Physics 2022-06-27 Yoshihiko Nishikawa , Atsushi Ikeda , Ludovic Berthier

We study the relation between short-time vibrational modes and long-time relaxational dynamics in a kinetically constrained lattice gas with harmonic interactions between neighbouring particles. We find a correlation between the location of…

Statistical Mechanics · Physics 2014-03-14 Douglas J. Ashton , Juan P. Garrahan

One of the central problems of the liquid-glass transition is whether there is a structural signature that can qualitatively distinguish different dynamic behaviors at different degrees of supercooling. Here, we propose a novel structural…

Soft Condensed Matter · Physics 2015-09-24 Yan-Wei Li , You-Liang Zhu , Zhao-Yan Sun

We investigate the relaxation process and the dynamical heterogeneities of the kinetically constrained Kob--Anderson lattice glass model, and show that these are characterized by different timescales. The dynamics is well described within…

Soft Condensed Matter · Physics 2011-09-21 Raffaele Pastore , Massimo Pica Ciamarra , Antonio de Candia , Antonio Coniglio

We study the role of elasticity-induced facilitation on the dynamics of glass-forming liquids by a coarse-grained two-dimensional model in which local relaxation events, taking place by thermal activation, can trigger new relaxations by…

Disordered Systems and Neural Networks · Physics 2023-04-05 Misaki Ozawa , Giulio Biroli

The dynamical arrest of gels is the consequence of a well defined structural phase transition, leading to the formation of a spanning cluster of bonded particles. The dynamical glass transition, instead, is not accompanied by any clear…

Soft Condensed Matter · Physics 2016-07-21 Raffaele Pastore , Antonio de Candia , Anallisa Fierro , Massimo Pica Ciamarra , Antonio Coniglio

Temporal relaxation of density fluctuations in supercooled liquids near the glass transition occurs in multiple steps. The short-time $\beta$-relaxation is generally attributed to spatially local processes involving the rattling motion of a…

Statistical Mechanics · Physics 2016-03-02 Smarajit Karmakar , Chandan Dasgupta , Srikanth Sastry

The elusive connection between dynamics and local structure in supercooled liquids is an important piece of the puzzle in the unsolved problem of the glass transition. The Johari-Goldstein beta relaxation, ubiquitous in glass-forming…

Soft Condensed Matter · Physics 2017-03-08 D. Fragiadakis , C. M. Roland

Glass-like materials are nonequilibrium systems where the relaxation time may exceed reasonable time scales of observations. In the present paper a dynamic percolation model is introduced in order to explain the principal properties of…

Condensed Matter · Physics 2007-05-23 A. Vazquez , O. Sotolongo-Costa

Despite the use of glasses for thousands of years, the nature of the glass transition is still mysterious. On approaching the glass transition, the growth of dynamic heterogeneity has long been thought to play a key role in explaining the…

Soft Condensed Matter · Physics 2018-03-23 Lijin Wang , Ning Xu , W. H. Wang , Pengfei Guan

We study the relaxation process in a two-dimensional lattice gas model, where the interactions come from the excluded volume. In this model particles have three arms with an asymmetrical shape, which results in geometrical frustration that…

Statistical Mechanics · Physics 2009-11-07 A. Diaz-Sanchez , Antonio de Candia , Antonio Coniglio

We identify a link between the glass transition and percolation of mobile regions in configuration space. We find that many hallmarks of glassy dynamics, for example stretched-exponential response functions and a diverging structural…

Statistical Mechanics · Physics 2009-11-13 Gregg Lois , Jerzy Blawzdziewicz , Corey S. O'Hern

We use the ``isoconfigurational ensemble'' [Phys. Rev. Lett. {\bf 93}, 135701 (2004)] to analyze both dynamical and structural properties in simulations of a glass forming molecular liquid. We show that spatially correlated clusters of low…

Materials Science · Physics 2009-11-11 Gurpreet S. Matharoo , M. S. Gulam Razul , Peter H. Poole

Molecular dynamics simulations are performed to investigate heterogeneous dynamics in amorphous glassy materials under oscillatory shear strain. We consider three-dimensional binary Lennard-Jones mixture well below the glass transition…

Soft Condensed Matter · Physics 2013-05-10 Nikolai V. Priezjev

Performing molecular dynamics simulations, we find that the structural relaxation dynamics of viscous silica, the prototype of a strong glass former, are spatially heterogeneous and cannot be understood as a statistical bond breaking…

Disordered Systems and Neural Networks · Physics 2009-11-10 Michael Vogel , Sharon C. Glotzer

Volume and enthalpy relaxation of glasses after a sudden temperature change has been extensively studied since Kovacs seminal work. One observes an asymmetric approach to equilibrium upon cooling versus heating and, more…

Soft Condensed Matter · Physics 2020-03-11 Matteo Lulli , Chun-Shing Lee , Hai-Yao Deng , Cho-Tung Yip , Chi-Hang Lam

We present a quantitative theory for a relaxation function in a simple glass-forming model (binary mixture of particles with different interaction parameters). It is shown that the slowing down is caused by the competition between locally…

Materials Science · Physics 2009-11-13 Edan Lerner , Itamar Procaccia
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