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Two beta-pyrochlore oxide superconductors, CsOs2O6 and RbOs2O6, are studied thermodynamically by measuring specific heat on polycrystalline samples. It is found that a Sommerfeld coefficient ? is nearly equal, 20 mJ/K2 mol Os, in the two…

Superconductivity · Physics 2009-11-11 Zenji Hiroi , Shigeki Yonezawa , Takaki Muramatsu , Jun-Ichi Yamaura , Yuji Muraoka

To assess electron correlation and electron-phonon coupling in the recently discovered beta-pyrochlores KOs2O6 and RbOs2O6, we have performed specific heat measurements in magnetic fields up to 14 T. We present data from high quality single…

Superconductivity · Physics 2009-11-11 M. Brühwiler , S. M. Kazakov , J. Karpinski , B. Batlogg

We report the single-crystal X-ray analysis of the structure of the pyrochlore oxide superconductor KOs$_2$O$_6$. The structure was identified as the $\beta$-pyrochlore structure with space group $Fd\bar{3}m$ and lattice constant $a$ =…

Superconductivity · Physics 2009-11-11 Jun-Ichi Yamaura , Shigeki Yonezawa , Yuji Muraoka , Zenji Hiroi

We report the basic thermodynamic properties of the new geometrically frustrated beta-pyrochlore bulk superconductor RbOs2O6 with a critical temperature Tc = 6.4 K. Specific heat measurements are performed in magnetic fields up to 12 T. The…

Superconductivity · Physics 2009-11-10 M. Brühwiler , S. M. Kazakov , N. D. Zhigadlo , J. Karpinski , B. Batlogg

Transition metal oxides of the $4d$ and $5d$ block have recently become the targets of materials discovery, largely due to their strong spin-orbit coupling that can generate exotic magnetic and electronic states. Here we report the high…

Rattling-induced superconductivity in the {\beta}-pyrochlore oxide KOs2O6 is investigated under high pressure up to 5 GPa. Resistivity measurements in a high-quality single crystal reveal a gradual decrease in the superconducting transition…

The superconducting transition of the ?-pyrochlore oxide KOs2O6 with Tc = 9.60 K is studied by resistivity measurements under various magnetic fields using a high-quality single crystal. The reentrant behavior of superconductivity is…

Superconductivity · Physics 2009-11-11 Zenji Hiroi , Shigeki Yonezawa

Magnetotransport properties in a nanocrystalline La$_{0.67}$Sr$_{0.33}$MnO$_{3}$/micron sized Al$_{2}$O$_{3}$ granular composite with different concentrations of Al$_{2}$O$_{3}$ have been studied. The resistivity curves in absence of…

Materials Science · Physics 2007-05-23 Soumik Mukhopadhyay , I. Das

We have prepared the oxyhydrate Na03RhO206H2O by extracting Na+ cations from NaRhO2 and intercalating water molecules using an aqueous solution of Na2S2O8. Synchrotron X-ray powder diffraction, thermogravimetric analysis (TGA), and…

Materials Science · Physics 2009-11-11 S. Park , K. Kang , W. Si , W. -S. Yoon , Y. Lee , A. R. Moodenbaugh , L. H. Lewis , T. Vogt

Here we report an unconventional magnetic and transport phenomenon in a layered cobalt oxide, NaxCoO2. Only for x = 0.75, a magnetic transition of the second order was clearly detected at Tm ~ 22 K where an apparent specific-heat jump, an…

Strongly Correlated Electrons · Physics 2009-11-07 T. Motohashi , R. Ueda , E. Naujalis , T. Tojo , I. Terasaki , T. Atake , M. Karppinen , H. Yamauchi

The electrical resistivity, magnetic susceptibility, and heat capacity of sintered samples of Ca2Ir2O7, in which pentavalent Ir atoms with 5d4 electron configuration form a pyrochlore structure, have been studied. The obtained experimental…

Strongly Correlated Electrons · Physics 2022-11-18 Yuki Nakayama , Yoshihiko Okamoto , Daigorou Hirai , Koshi Takenaka

We develop a general procedure for the analysis of bulk thermodynamic data of a superconductor for samples containing a metallic non-superconducting second phase. The method is based on the condensation energy and it allows the extraction…

Superconductivity · Physics 2009-11-11 M. Brühwiler , S. M. Kazakov , J. Karpinski , B. Batlogg

We make the first report that a metallic pyrochlore oxide \Cd2Re2O7, exhibits type II superconductivity at 1.1 K. The pyrochlore oxide is known to be a geometrical frustrated system, which includes the tetrahedral network of magnetic ions.…

Strongly Correlated Electrons · Physics 2016-08-16 H. Sakai , K. Yoshimura , H. Ohno , H. Kato , S. Kambe , R. E. Walstedt , T. D. Matsuda , Y. Haga , Y. Ōnuki

The crystal structure and magnetic ordering pattern of PdAs2O6 were investigated by neutron powder diffraction. While the magnetic structure of PdAs2O6 is identical to the one of its isostructural 3d-homologue NiAs2O6, its N\'{e}el…

Strongly Correlated Electrons · Physics 2015-06-04 M. Reehuis , T. Saha-Dasgupta , D. Orosel , J. Nuss , B. Rahaman , B. Keimer , O. K. Andersen , M. Jansen

The results of the LSDA+U calculations for pyroxenes with diverse magnetic properties (Li,Na)TM(Si,Ge)$_2$O$_6$, where TM is the transition metal ion (Ti,V,Cr,Mn,Fe), are presented. We show that the anisotropic orbital ordering results in…

Strongly Correlated Electrons · Physics 2008-02-05 S. V. Streltsov , D. I. Khomskii

In this study, I have investigated the magnetic and critical properties of manganese pyrochlore fluoride NaSrMn$_{2}$F$_{7}$, which exhibits a glass transition at T$_\text{f}$$=$2.5 (K) due to charge disorder. A DFT+$U$+SOC framework is…

Strongly Correlated Electrons · Physics 2023-05-09 Mohammad Amirabbasi

We report a first-principles density-functional calculation of the electronic structure and properties of the recently discovered superconducting beta-pyrochlore oxide KOs_2O_6. We find that the electronic structure near the Fermi energy…

Superconductivity · Physics 2009-11-10 R. Saniz , J. E. Medvedeva , Lin-Hui Ye , T. Shishidou , A. J. Freeman

Powder Na$_{x}$CoO$_{2}$ ($0.70\leq x\leq 0.84$) samples were synthesized and characterized carefully by X-ray diffraction analysis, inductive-coupled plasma atomic emission spectroscopy, and redox titration. It was proved that…

Materials Science · Physics 2009-11-10 H. Sakurai , S. Takenouchi , N. Tsujii , E. Takayama-Muromachi

We performed high-pressure transport measurements on high-quality single crystals of KOs2O6, a beta-pyrochlore superconductor. While the resistivity at high temperatures might approach saturation, there is no sign of saturation at low…

Superconductivity · Physics 2007-05-23 A. Akrap , E. Tutis , S. M. Kazakov , N. D. Zhigadlo , J. Karpinski , L. Forro

The superconducting properties of two beta-pyrochlore oxides, CsOs2O6 and RbOs2O6, are studied by thermodynamic and transport measurements using high-quality single crystals. It is shown that the character of superconductivity changes…

Superconductivity · Physics 2009-08-05 Yohei Nagao , Jun-ichi Yamaura , Hiroki Ogusu , Yoshihiko Okamoto , Zenji Hiroi