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An appropriate model for the random energy landscape in organic glasses is a spatially correlated Gaussian field, generated by randomly located and oriented dipoles and quadrupoles. Correlation properties of energetic disorder directly…

Materials Science · Physics 2013-03-21 S. V. Novikov

A number of computer-generated models of water, methanol and ethanol are considered at room temperature and ambient pressure, and also as a function of temperature (for water and ethanol), and the potential model (for water only). The…

Chemical Physics · Physics 2019-06-12 I. Bakó , I. Pethes , Sz. Pothoczki , L. Pusztai

An analytically tractable model is introduced which exhibits both, a glass--like freezing transition, and a collection of double--well configurations in its zero--temperature potential energy landscape. The latter are generally believed to…

Condensed Matter · Physics 2009-10-28 Reimer Kuehn

The aim of this paper is to discuss some basic notions regarding generic glass forming systems composed of particles interacting via soft potentials. Excluding explicitly hard-core interaction we discuss the so called `glass transition' in…

Disordered Systems and Neural Networks · Physics 2009-11-13 Jean-Pierre Eckmann , Itamar Procaccia

A new class of lattice gas models with trivial interactions but constrained dynamics are introduced. These are proven to exhibit a dynamical glass transition: above a critical density, rho_c, ergodicity is broken due to the appearance of an…

Statistical Mechanics · Physics 2009-11-11 Cristina Toninelli , Giulio Biroli , Daniel S. Fisher

The dynamical behavior of a kind of models with hierarchically constrained dynamics is investigated. The models exhibit many properties resembling real structural glasses. In particular, we focus on the study of time-dependent temperature…

Statistical Mechanics · Physics 2009-11-07 A. Prados , J. J. Brey

We consider a generalized version of the Random Energy Model in which the energy of each configuration is given by the sum of $N$ independent contributions ("local energies") with finite variances but otherwise arbitrary statistics. Using…

Statistical Mechanics · Physics 2013-07-25 Florian Angeletti , Eric Bertin , Patrice Abry

We use the results derived in the framework of the replica approach to study the liquid-glass thermodynamic transition. The main results are rederived without using replicas and applied to the study of the Lennard-Jones binary mixture…

Soft Condensed Matter · Physics 2009-10-31 Barbara Coluzzi , Giorgio Parisi , Paolo Verrocchio

Using molecular dynamics computer simulations we investigate the out-of-equilibrium dynamics of a Lennard-Jones system after a quench from a high temperature to one below the glass transition temperature. By studying the radial distribution…

Statistical Mechanics · Physics 2009-10-31 Walter Kob , Jean-Louis Barrat , Francesco Sciortino , Piero Tartaglia

Using molecular dynamics computer simulations we investigate the dependence of bulk properties of a Lennard-Jones glass on the cooling rate with which the glass was produced. By studying the clusters formed by the nearest neighbor shells of…

Condensed Matter · Physics 2009-10-28 K. Vollmayr , W. Kob , K. Binder

In the free energy landscape picture of glassy systems, the slow dynamics characteristic of these systems is believed to be due to the existence of a complicated free-energy landscape with many local minima. We show here that for a…

Soft Condensed Matter · Physics 2009-11-11 Sara Jabbari-Farouji , Gerard H. Wegdam , Daniel Bonn

In this paper, we will investigate critical phenomena by considering a model spin-glass on scale-free networks. For this purpose, we consider the Ghatak-Sherrington (GS) model, a spin-1 spin-glass model with a crystal field, instead of the…

Disordered Systems and Neural Networks · Physics 2014-03-14 Do-Hyun Kim

We develop a modified "two-state" model with Gaussian widths for the site energies of both ground and excited states, consistent with expectations for a disordered system. The thermodynamic properties of the system are analyzed in…

Soft Condensed Matter · Physics 2009-11-11 Dmitry V. Matyushov , C. A. Angell

We perform simulations to investigate how the energy carried by a molecule transfers to others in an equilibrium gas model. For this purpose we consider a microcanonical ensemble of equilibrium gas systems, each of them contains a tagged…

Classical Physics · Physics 2015-05-27 Jinghua Yang , Yong Zhang , Jiao Wang , Hong Zhao

Global climate warming poses a significant challenge to humanity; it is associated with, e.g., rising sea level and declining Arctic sea ice. Increasing extreme events are also considered to be a result of climate…

Physics and Society · Physics 2019-01-23 Jingfang Fan , Jun Meng , Yosef Ashkenazy , Shlomo Havlin , Hans Joachim Schellnhuber

How do we search for the entire family tree without unwanted random guesses, starting from a high-index and high-energy stationary state on the energy landscape? Here we introduce a general numerical method that constructs the pathway map…

Computational Physics · Physics 2021-04-21 Jianyuan Yin , Yiwei Wang , Jeff Z. Y. Chen , Pingwen Zhang , Lei Zhang

Generative models are a promising tool to address the sampling problem in multi-body and condensed-matter systems in the framework of statistical mechanics. In this work, we show that normalizing flows can be used to learn a transformation…

Computational Physics · Physics 2022-08-23 Alessandro Coretti , Sebastian Falkner , Phillip Geissler , Christoph Dellago

We numerically study the zero-temperature relaxation dynamics of several glass-forming models to their inherent structures, following quenches from equilibrium configurations sampled across a wide range of initial temperatures. In a…

Statistical Mechanics · Physics 2022-04-07 Yoshihiko Nishikawa , Misaki Ozawa , Atsushi Ikeda , Pinaki Chaudhuri , Ludovic Berthier

During the last few years, a number of works in computer simulation have focused on the clustering and percolation properties of simple fluids based in an energetic connectivity criterion proposed long ago by T.L. Hill [J. Chem. Phys. 23,…

Soft Condensed Matter · Physics 2009-11-07 Luis A. Pugnaloni , Ileana F. Marquez , Fernando Vericat

The stress-strain relations and the yield behavior of model glass (a 80:20 binary Lennard-Jones mixture) is studied by means of MD simulations. First, a thorough analysis of the static yield stress is presented via simulations under imposed…

Soft Condensed Matter · Physics 2009-11-10 F. Varnik , L. Bocquet , J. -L. Barrat