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The available theoretical approaches aiming at describing Dynamic Nuclear spin Polarization (DNP) in solutions containing molecules of biomedical interest and paramagnetic centers are not able to model the behaviour observed upon varying…

Statistical Mechanics · Physics 2014-06-06 Sonia Colombo Serra , Marta Filibian , Pietro Carretta , Alberto Rosso , Fabio Tedoldi

We report on experiments that quantify the role of a central electronic spin as a relaxation source for nuclear spins in its nanoscale environment. Our strategy exploits hyperpolarization injection from the electron as a means to…

Mesoscale and Nanoscale Physics · Physics 2024-02-27 William Beatrez , Arjun Pillai , Otto Janes , Dieter Suter , Ashok Ajoy

Experimental investigation of nuclear spin effects on the electron spin polarization in singly negatively charged InP quantum dots is reported. Pump-probe photoluminescence measurements of electron spin relaxation in the microsecond…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Bipul Pal , Sergey Yu. Verbin , Ivan V. Ignatiev , Michio Ikezawa , Yasuaki Masumoto

$^{235}$U nuclear spin-lattice ($T_1^{-1}$) and spin-spin ($T_2^{-1}$) relaxation rates in the itinerant antiferromagnet USb$_2$ are reported as a function of temperature in zero field. The heating effect from the intense rf pulses that are…

Strongly Correlated Electrons · Physics 2010-02-24 S. -H. Baek , N. J. Curro , H. Sakai , E. D. Bauer , J. C. Cooley , J. L. Smith

We consider the isotropic $S=1$ Heisenberg chain with a finite Haldane gap $\Delta$ and use state-of-the-art numerical techniques to investigate its dynamical properties at finite temperature, focusing on the nuclear spin-lattice relaxation…

Strongly Correlated Electrons · Physics 2019-09-19 Sylvain Capponi , Maxime Dupont , Anders W. Sandvik , Pinaki Sengupta

Dielectric study on Ca3Mn2O7 features relaxor-like segmented dynamics below the antiferromagnetic ordering. Dipolar relaxations of different origin are spectrally resolved exhibiting distinct H-field alterations. This identifies their…

Materials Science · Physics 2019-09-10 Pooja Sahlot , Gaurav Sharma , Vasant Sathe , Anand Mohan Awasthi

We report on a study of Dynamic Nuclear Polarization and electron and nuclear spin relaxation of atomic hydrogen and deuterium in solid molecular matrices of H$_{2}$, D$_{2}$, and HD mixtures. The electron and nuclear spin relaxation times…

Atomic and Molecular Clusters · Physics 2017-02-08 S. Sheludiakov , J. Ahokas , J. Järvinen , O. Vainio , L. Lehtonen , S. Vasiliev , D. M. Lee , V. V. Khmelenko

Inorganic solid-state battery electrolytes show high ionic conductivities and enable the fabrication of all solid-state batteries. In this work, we present the temperature dependence of spin-lattice relaxation time (T1), spin-spin…

Materials Science · Physics 2023-03-24 Darshan Chalise , Carlos Juarez-Yescas , Beniamin Zahiri , Paul V. Braun , David G. Cahill

The proton nuclear spin-lattice relaxation rate 1/T1 has been measured as a function of temperature and magnetic field (up to 15 T) in the molecular magnetic ring Fe10. Striking enhancement of 1/T1 is observed around magnetic field values…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 M. -H. Julien , Z. H. Jang , A. Lascialfari , F. Borsa , M. Horvatic , A. Caneschi , D. Gatteschi

We have studied the low temperature a.c. magnetic susceptibility of the diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y or Lu. We…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , Ari Mizel , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

Measurements of the spin-lattice relaxation rate 1/T_1 by nuclear magnetic resonance for the one-dimensional Heisenberg antiferromagnet Sr_2CuO_3 have provided evidence for a diffusion-like contribution at finite temperature and small…

Strongly Correlated Electrons · Physics 2007-05-23 J. Sirker

We investigate nuclear spin-lattice relaxation data in the normal state of optimally doped YBaCuO_7 by analyzing the contributions to the relaxation rate of the copper, planar oxygen and yttrium along the directions perpendicular to the…

Superconductivity · Physics 2009-11-11 A. Uldry , P. F. Meier

The magnetization processes of the spin-3/2 antiferromagnet LiInCr4O8 comprising a "breathing" pyrochlore lattice, which is an alternating array of small and large tetrahedra, are studied under ultrahigh magnetic fields of up to 130 T using…

The hole-doped kagome lattice of Cu2+ ions in LaCuO2.66 was investigated by nuclear quadrupole resonance (NQR), electron spin resonance (ESR), electrical resistivity, bulk magnetization and specific heat measurements. For temperatures above…

Strongly Correlated Electrons · Physics 2013-09-05 M. -H. Julien , V. Simonet , B. Canals , R. Ballou , A. K. Hassan , M. Affronte , V. O. Garlea , C. Darie , P. Bordet

Heterometallic molecular chromium wheels are fascinating new magnetic materials. We reexamine the available experimental susceptibility data on MCr7 wheels in terms of a simple isotropic Heisenberg Hamiltonian for M=Fe, Ni, Cu, and Zn and…

Materials Science · Physics 2007-08-09 M. Allalen , J. Schnack

We have performed field-swept 59Co NMR measurements on the 'exotic' spin-chain material, Ca3Co2O6, crystallizing in K4CdCl6-type rhombohedral structure, believed to exhibit two magnetic transition temperatures (around 24 and 12 K). This is…

Strongly Correlated Electrons · Physics 2009-11-10 E. V. Sampathkumaran , N. Fujiwara , S. Rayaprol , P. K. Madhu , Y. Uwatoko

Field-inhomogeneity-induced relaxation of atomic spins confined in vapor cells with depolarizing walls is studied. In contrast to nuclear spins, such as noble-gas spins, which experience minimal polarization loss at cell walls, atomic spins…

Quantum Physics · Physics 2024-12-10 Yue Chang , Shuangai Wan , Shichao Dong , Jie Qin

The magnetic state of the single-component molecular compound, [Cu(tmdt)$_{2}$], is investigated by means of $^{1}$H-NMR. An abrupt spectral broadening below 13 K and a sharp peak in nuclear spin-lattice relaxation rate, $T_{1}^{-1}$, at 13…

Strongly Correlated Electrons · Physics 2012-05-31 Rina Takagi , Kazuya Miyagawa , Kazushi Kanoda , Biao Zhou , Akiko Kobayashi , Hayao Kobayashi

We present a study of the magnetic-field effect on spin correlations in the charge ordered triangular Ising system LuFe2O4+{\delta} through single crystal neutron diffraction. In the absence of a magnetic field, the strong diffuse neutron…

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…