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Low-temperature electron paramagnetic resonance measurements are performed on single crystals of LiY_{1-x}Gd_xF_4 with weak x=0.005 and moderate x=0.05 concentration of Gd ions. Modeling of the experimental spectra allows us to precisely…

Strongly Correlated Electrons · Physics 2023-07-13 S. S. Sosin , A. F. Iafarova , I. V. Romanova , O. A. Morozov , S. L. Korableva , R. G. Batulin , M. Zhitomirsky , V. N. Glazkov

1H nuclear magnetic resonance (NMR) measurements in [YPc2]0, an organic compound formed by radicals stacking along chains, are presented. The temperature dependence of the macroscopic susceptibility, of the NMR shift and of the spin-lattice…

Strongly Correlated Electrons · Physics 2015-05-20 F. Branzoli , P. Carretta , M. Filibian , S. Klyatskaya , M. Ruben

Spin-lattice relaxation is a key open problem to understand the spin dynamics of single-molecule magnets and molecular spin qubits. While modelling the coupling between spin states and local vibrations allows to determine the more relevant…

Atomic and Molecular Clusters · Physics 2021-11-08 Aman Ullah , José J. Baldoví , Alejandro Gaita-Ariño , Eugenio Coronado

The short ranged magnetic correlations and dynamics of hole doped $Pr_{1-x}Ca_{x}MnO_{3}$ (0.33 < x < 0.5) of different crystallite sizes have been investigated using electron spin resonance spectroscopy (ESR). The major contribution to the…

Strongly Correlated Electrons · Physics 2017-04-05 Vinay Kumar Shukla , Soumik Mukhopadhyay

We investigate spin dynamics in antiferromagnetic (AF) molecular rings at finite temperature in the presence of spin-phonon (s-p) interaction. We derive a general expression for the spin susceptibility in the weak s-p coupling limit and…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Leonardo Spanu , Alberto Parola

We investigated the magnetic phase diagram of single crystals of SrNdFeO$_{4}$ by measuring the magnetic properties, the specific heat and the dielectric permittivity. The system has two magnetically active ions, Fe$^{3+}$ and Nd$^{3+}$.…

Materials Science · Physics 2015-06-05 J. M. Hwang , E. S. Choi , H. D. Zhou , Y. Xin , J. Lu , P. Schlottmann

We report 7Li-NMR studies on LiInCr4O8 and LiGaCr4O8, in which Cr3+ ions with spin 3/2 form a breathing pyrochlore lattice, a network of tetrahedra with alternating sizes. In LiInCr4O8 with large alternation, the nuclear relaxation rate…

Strongly Correlated Electrons · Physics 2015-06-23 Yu Tanaka , Makoto Yoshida , Masashi Takigawa , Yoshihiko Okamoto , Zenji Hiroi

We present the results of muon-spin relaxation measurements of spin excitations in the one-dimensional quantum Heisenberg antiferromagnet Cu(pyz)(NO$_{3}$)$_{2}$. Using density-functional theory we propose muon sites and assess the degree…

Strongly Correlated Electrons · Physics 2015-05-20 F. Xiao , J. S. Möller , T. Lancaster , R. C. Williams , F. L. Pratt , S. J. Blundell , D. Ceresoli , A. M. Barton , J. L. Manson

We report on observations of spin dynamics in single Yb$^+$ ions immersed in a cold cloud of spin-polarized $^6$Li atoms. This species combination has been proposed to be the most suitable system to reach the quantum regime in atom-ion…

At temperatures below the magnetic anisotropy energy, monodomain magnetic systems (small particles, nanomagnetic devices, etc.) must relax quantum mechanically. This quantum relaxation must be mediated by the coupling to both nuclear spins…

Condensed Matter · Physics 2009-10-28 N. V. Prokof'ev , P. C. E. Stamp

The spin-reversal in dilute Li$_2$(Li$_{1-x}$Fe$_{x}$)N with $x < 1$ % is dominated by resonant quantum tunneling of spatially well-separated states. We report on the effect of finite couplings between those states that give rise to…

Strongly Correlated Electrons · Physics 2024-11-04 M. Fix , J. H. Atkinson , F. Müller , E. del Barco , A. Jesche

Extensive work on single molecule magnets has identified a fundamental mode of relaxation arising from the nuclear-spin assisted quantum tunnelling of nearly independent and quasi-classical magnetic dipoles. Here we show that nuclear-spin…

Strongly Correlated Electrons · Physics 2019-03-28 C. Paulsen , S. R. Giblin , E. Lhotel , D. Prabhakaran , K. Matsuhira , G. Balakrishnan , S. T. Bramwell

Nuclear relaxation in half-integer spin chains at low temperatures (T << J, the antiferromagnetic exchange constant) is dominated by dissipation from a gas of thermally-excited, overdamped, spinons. The universal low temperature dependence…

Condensed Matter · Physics 2009-10-22 Subir Sachdev

Selective doping with different R-site ions in rare-earth perovskite RFeO3 compounds offers an effective way to achieve atomic-scale tuning of the complex exchange interactions. In this study, the spin reorientation temperature of Tb-doped…

Materials Science · Physics 2025-09-09 Mingzhu Xue , Xin Li , Shilei Ding , Qixin Li , Wenhao Di , Anhua Wu , Bin He , Shishen Yan , Wenyun Yang , Jinbo Yang

We show that the spin-lattice relaxation in n-type insulating GaAs is dramatically accelerated at low magnetic fields. The origin of this effect, that cannot be explained in terms of well-known diffusion-limited hyperfine relaxation, is…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 M. Kotur , R. I. Dzhioev , M. Vladimirova , B. Jouault , V. L. Korenev , K. V. Kavokin

New particles with masses in the sub-eV range have been predicted by various theories beyond the Standard Model. Some can induce new spin-spin interactions between fermions. Existing constraints on such interactions between nucleons with…

Atomic Physics · Physics 2011-03-04 Changbo Fu , W. M. Snow

A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 A. Morello , A. Millán , L. J. de Jongh

The NMR measurements performed on a single orthorhombic crystal of superconducting ferromagnet UCoGe (Y.Ihara et al, Phys. Rev. Lett. v.105, 206403 (2010)) demonstrate strongly anisotropic magnetic properties of this material. The presented…

Strongly Correlated Electrons · Physics 2021-10-04 V. P. Mineev

We have investigated the coupling of lattice with spin via strain interactions in the CoFe2O4/PMN-PT composite system. X-ray diffraction and Raman spectroscopic studies illustrate a remarkable modification in CoFe2O4lattice across Curie…

The nuclear magnetic relaxation in scandium metal is investigated at liquid helium temeprature for both single crystal and powder samples. The obtained temperature and field dependence of the Korringa constant are described by the means of…