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We report measurements of 19F nuclear spin-lattice relaxation 1/T1 as a function of temperature and external magnetic field in LiY0.998Ho0.002F4 single crystal, a single-ion magnet exhibiting interesting quantum effects. The 19F 1/T1 is…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. J. Graf , A. Lascialfari , F. Borsa , A. M. Tkachuk , B. Barbara

Staircase hysteresis loops of the magnetization of a LiY_0.998Ho_0.002F_4 single crystal are observed at subkelvin temperatures and low field sweep rates. This behavior results from quantum dynamics at avoided level crossings of the energy…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. Giraud , W. Wernsdorfer , A. M. Tkachuk , D. Mailly , B. Barbara

Measurements of 89Y nuclear spin-lattice relaxation in SrY2O4:Ho3+ crystals for the magnetic field B parallel to the crystal c axis show that 89Y at T < 20 K relaxes due to fluctuating magnetic field created only by Ho13+ transitions…

Strongly Correlated Electrons · Physics 2017-12-11 A. V. Dooglav , I. F. Gilmutdinov , V. I. Katkov , A. G. Kiiamov , I. R. Mukhamedshin

We present measurements of magnetic field and frequency dependences of the low temperature (T = 1.8 K) AC-susceptibility, and temperature and field dependences of the longitudinal field positive muon spin relaxation ({\mu}SR) for…

Strongly Correlated Electrons · Physics 2015-06-05 R. C. Johnson , B. Z. Malkin , J. S. Lord , S. R. Giblin , A. Amato , C. Baines , A. Lascialfari , B. Barbara , M. J. Graf

The temperature dependences of spin-lattice relaxation time $T_1$ of $^{133}$Cs in CsFeCl$_3$ and $^{87}$Rb in RbFeCl$_3$ were measured in the temperature range between 1.5 K and 22 K, at various fields up to 7 T applied parallel (or…

Materials Science · Physics 2009-11-07 Mitsuru Toda , Takao Goto , Meiro Chiba , Naoshi Suzuki

A study of the modifications of the magnetic properties of Ho$_{2-x}$Y$_x$Sn$_2$O$_7$ upon varying the concentration of diamagnetic Y$^{3+}$ ions is presented. Magnetization and specific heat measurements show that the Spin Ice ground-state…

Strongly Correlated Electrons · Physics 2010-11-01 G. Prando , P. Carretta , S. R. Giblin , J. Lago , S. Pin , P. Ghigna

Frequency and dc magnetic field dependences of dynamic susceptibility in diluted paramagnets LiYF$_4$:Ho$^{3+}$ have been measured at liquid helium temperatures in the ac and dc magnetic fields parallel to the symmetry axis of a tetragonal…

Strongly Correlated Electrons · Physics 2009-10-06 S. Bertaina , B. Barbara , R. Giraud , B. Z. Malkin , M. V. Vanuynin , A. I. Pominov , A. L. Stolov , A. M. Tkachuk

The nuclear spin-lattice relaxation rate ($1/T_{1}$) has been measured in the single crystals of hole doped two-leg ladder compounds Sr$_{14-x}$Ca$_{x}$Cu$_{24}$O$_{41}$ and in the undoped parent material La$_6$Ca$_8$Cu$_{24}$O$_{41}$.…

Strongly Correlated Electrons · Physics 2009-10-31 S. Fujiyama , M. Takigawa , N. Motoyama , H. Eisaki , S. Uchida

^{139}La NMR measurements of La_{2/3}Ca_{1/3}MnO_3 performed in the paramagnetic state and high magnetic fields are reported. Analysis of the high temperature spectrum measured establishes that the spectrum it is a standard powder pattern…

Strongly Correlated Electrons · Physics 2009-10-31 K. E. Sakaie , C. P. Slichter , P. Lin , M. Jaime , M. B. Salamon

We explore the quantum dynamics of nuclear spin relaxation in cold collisions of $^1\Sigma^+$ molecules with structureless atoms in an external magnetic field. To this end, we develop a rigorous coupled-channel methodology, which accounts…

Chemical Physics · Physics 2023-06-29 Rebekah Hermsmeier , Xiaodong Xing , Timur V. Tscherbul

Strong hyperfine coupling in a 0.2% Holmium doped LiYF_4 single crystal induces staircaselike hysteresis loops of the magnetization at very low temperatures. The field sweep rate dependence of hysteresis loops allows the study of two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. Giraud , W. Wernsdorfer , A. M. Tkachuk , D. Mailly , B. Barbara

The spin-lattice relaxation rate $T_{1}^{-1}$ and NMR spectra of $^1$H in single crystal molecular magnets of Fe8 have been measured down to 15 mK. The relaxation rate $T_1^{-1}$ shows a strong temperature dependence down to 400 mK. The…

Condensed Matter · Physics 2009-11-07 Miki Ueda , Satoru Maegawa , Susumu Kitagawa

We report on the spin waves and crystal field excitations in single crystal LiFePO$_4$ by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we…

Strongly Correlated Electrons · Physics 2017-03-15 Yuen Yiu , Manh Duc Le , Rasmus Toft-Peterson , Georg Ehlers , Robert McQueeney , David Vaknin

The magnetic interactions between the spin of an unpaired electron and the surrounding nuclear spins can be exploited to gain structural information, to reduce nuclear relaxation times as well as to create nuclear hyperpolarization via…

$^{19}$F NMR measurements in SmFeAsO$_{1-x}$F$_x$, for $0.15\leq x\leq 0.2$, are presented. The nuclear spin-lattice relaxation rate $1/T_1$ increases upon cooling with a trend analogous to the one already observed in…

Superconductivity · Physics 2010-03-22 G. Prando , P. Carretta , A. Rigamonti , S. Sanna , A. Palenzona , M. Putti , M. Tropeano

We report $\beta$-detected nuclear magnetic resonance ($\beta$-NMR) measurements of implanted $^{8}$Li$^{+}$ in a synthetic single crystal of $\alpha$-SiO$_2$ (quartz). At 6.55 Tesla, the spectrum is comprised of a large amplitude broad…

The problem of the nuclear spin-lattice relaxation in La$_2$CuO$_4$ is revisited in connection with the recent measurements of the NQR relaxation rate for temperatures up to $ 900\mbox{K} $ [T.\ Imai {\em et al.}, Phys.\ Rev.\ Lett., in…

Condensed Matter · Physics 2009-10-22 A. Sokol , E. Gagliano , S. Bacci

Spin relaxation between the two lowest-lying spin-states has been studied in the S=4 single molecule magnet Ni$_4$ under steady state conditions of low amplitude and continuous microwave irradiation. The relaxation rate was determined as a…

Mesoscale and Nanoscale Physics · Physics 2008-07-22 G. de Loubens , D. A. Garanin , C. C. Beedle , D. N. Hendrickson , A. D. Kent

When degenerate states are separated by large energy barriers, the approach to thermal equilibrium can be slow enough that physical properties are defined by the thermalization process rather than the equilibrium. The exploration of…

Cross-correlation between magnetism and dielectric is expected to offer novel emergent phenomena. Here, magnetic excitations in the organic donor-acceptor spin-chain system, TTF-BA, with a ferroelectric ground state is investigated by…

Materials Science · Physics 2020-12-09 K. Sunami , Y. Sakai , R. Takehara , H. Adachi , K. Miyagawa , S. Horiuchi , K. Kanoda
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