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In an experiment on three-photon laser excitation $5S_{1/2} \to 5P_{3/2} \to 6S_{1/2} \to 37P_{3/2}$ of a single $^{87}$Rb Rydberg atom in an optical dipole trap, we have observed for the first time three-photon Rabi oscillations between…

We demonstrate a non-equilibrium phase transition in a dilute thermal atomic gas. The phase transition, between states of low and high Rydberg occupancy, is induced by resonant dipole-dipole interactions between Rydberg atoms. The gas can…

Atomic Physics · Physics 2016-11-04 Christopher Carr , Ralf Ritter , Christopher Wade , Charles S Adams , Kevin J Weatherill

Electric field sensors based on Rydberg atoms offer unique capabilities, relative to traditional sensors, for detecting radio-frequency signals. In this work, we demonstrate simultaneous demodulation and detection of five rf tones spanning…

Atomic Physics · Physics 2023-01-11 David H. Meyer , Joshua C. Hill , Paul D. Kunz , Kevin C. Cox

We investigate the impact of an electric field on the structure of ultralong-range polar diatomic Rydberg molecules. Both the s-wave and p-wave interactions of the Rydberg electron and the neutral ground state atom are taken into account.…

Atomic Physics · Physics 2015-06-15 Markus Kurz , Peter Schmelcher

We report on time-resolved pulsed four-wave mixing (FWM) signals in a thermal Rubidium vapor involving a Rydberg state. We observe FWM signals with dephasing times up to 7 ns, strongly dependent on the excitation bandwidth to the Rydberg…

Atomic Physics · Physics 2016-02-17 Yi-Hsin Chen , Fabian Ripka , Robert Löw , Tilman Pfau

A candidate for converting quantum information from microwave to optical frequencies is the use of a single atom that interacts with a superconducting microwave resonator on one hand and an optical cavity on the other. The large electric…

Quantum Physics · Physics 2017-07-26 Bryan T. Gard , Kurt Jacobs , R. McDermott , M. Saffman

Divalent atoms provide excellent means for advancing control in Rydberg atom-based quantum simulation and computing, due to the second optically active valence electron available. Particularly promising in this context are circular Rydberg…

A highly excited Rydberg atom via electromagnetically induced transparency with two color cascading lasers has extreme sensitivity to electric fields of microwave ranging from 100 MHz to over 1 THz. It can be used as susceptible atom-based…

Atomic Physics · Physics 2021-11-15 M. H. Cai , Z. S. Xu , S. H. You , H. P. Liu

The dissociation dynamics of the $\tilde{A}$-state of ammonia have been studied using a resonant multiphoton ionisation probe in a photoelectron spectroscopy experiment. The use of a resonant intermediate in the multiphoton ionisation…

We study Rydberg atoms modulated by strong radio-frequency (RF) fields with a frequency of 70 MHz. The Rydberg atoms are prepared in a room temperature cesium cell, and their level structure is probed using electromagnetically induced…

Atomic Physics · Physics 2017-07-31 Yuechun Jiao , Zhiwei Yang , Jingkui Li , Georg Raithel , Jianming Zhao , Suotang Jia

Rydberg atom-based electric field sensing can provide all-optical readout of radio frequency fields in a dielectric environment. However, because a single set of optical fields is typically used to prepare the Rydberg state and read out its…

Dipole-dipole interactions lead to frequency shifts that are expected to limit the performance of next-generation atomic clocks. In this work, we compute dipolar frequency shifts accounting for the intrinsic atomic multilevel structure in…

Quantum Gases · Physics 2021-07-07 A. Cidrim , A. Piñeiro Orioli , C. Sanner , R. B. Hutson , J. Ye , R. Bachelard , A. M. Rey

Atoms interact with each other through the electromagnetic field, creating collective states that can radiate faster or slower than a single atom, i.e. super- and sub-radiance. The generation and control of such states by engineering the…

We formulate the theory for a diatomic molecule in a spatially degenerate electronic state interacting with a non-resonant laser field and investigate its rovibrational structure in the presence of the field. We report on \textit{ab initio}…

The advent of digital neutral-atom quantum computers relies on the development of fast and robust protocols for high-fidelity quantum operations. In this work, we introduce a novel scheme for entangling gates using four atomic levels per…

Quantum Physics · Physics 2025-07-22 Giuliano Giudici , Stefano Veroni , Giacomo Giudice , Hannes Pichler , Johannes Zeiher

Applicability of Rydberg atoms to quantum computers is examined from experimental point of view. In many theoretical proposals appeared recently, excitation of atoms into highly excited Rydberg states was considered as a way to achieve…

Quantum Physics · Physics 2007-05-23 Igor I. Ryabtsev , Denis B. Tretyakov , Ilya I. Beterov

The theory is presented for resonance interaction between two atoms in an excited configuration: one atom, the "receptor" of information (i.e. energy), adsorbed on a phospholipid surface and the other atom, the "emitter" of information…

Quantum Physics · Physics 2013-05-20 Mathias Boström , Clas Persson , Dan Huang , Barry W. Ninham , Bo E. Sernelius

We present an experimental and theoretical study of phase-dependent interference effects in multi-photon excitation under bichromatic radio-frequency (rf) field. Using an intense rf pulse, we study the interference between the three-photon…

Quantum Physics · Physics 2011-03-14 Pankaj K. Jha , Hebin Li , Vladimir A. Sautenkov , Yuri V. Rostovtsev , Marlan O. Scully

Coupling by the resonant dipole-dipole energy transfer between cold cesium Rydberg atoms is investigated using time-resolved narrow-band de-excitation spectroscopy. This technique combines the advantage of efficient Rydberg excitation with…

Atomic Physics · Physics 2009-11-11 Marcel Mudrich , Nassim Zahzam , Thibault Vogt , Daniel Comparat , Pierre Pillet

In this work, we demonstrate the generation of sidebands in electromagnetically induced transparency (EIT) signal due to frequency modulation of Rydberg states in $^{87}\text{Rb}$ thermal vapor. An oscillating radio-frequency (RF) electric…

Atomic Physics · Physics 2023-09-14 Nabendu S. Mishra
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