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Time-resolved photoemission experiments can reveal fascinating quantum dynamics of correlated electrons. However, the thermalization of the electronic system is typically so fast that very short probe pulses are necessary to resolve the…

Strongly Correlated Electrons · Physics 2009-09-02 Martin Eckstein , Marcus Kollar

We describe the temporal evolution of the time-resolved photoemission response of the spinless Falicov-Kimball model driven out of equilibrium by strong applied fields. The model is one of the few possessing a metal-insulator transition and…

Strongly Correlated Electrons · Physics 2010-04-23 B. Moritz , T. P. Devereaux , J. K. Freericks

We derive exact operator average expressions for the first two spectral moments of nonequilibrium Green's functions for the Falicov-Kimball model and the Hubbard model in the presence of a spatially uniform, time-dependent electric field.…

Strongly Correlated Electrons · Physics 2009-11-11 V. M. Turkowski , J. K. Freericks

In this work we examine the time-resolved, instantaneous current response for the spinless Falicov-Kimball model at half-filling, on both sides of the Mott-Hubbard metal-insulator transition, driven by a strong electric field pump pulse.…

Strongly Correlated Electrons · Physics 2015-05-18 B. Moritz , T. P. Devereaux , J. K. Freericks

We present a linear-response formalism for a system of correlated electrons out of equilibrium, as relevant for the probe optical absorption in pump-probe experiments. We consider the time dependent optical conductivity $\sigma(\omega,t)$…

Strongly Correlated Electrons · Physics 2017-04-04 Zala Lenarčič , Denis Golež , Janez Bonča , Peter Prelovšek

In the last two decades, non-equilibrium spectroscopies have evolved from avant-garde studies to crucial tools for expanding our understanding of the physics of strongly correlated materials. The possibility of obtaining simultaneously…

The theory for time-resolved photoemission spectroscopy as applied to pump-probe experiments is developed and solved for the generic case of a strongly correlated material. The formal development incorporates all of the nonequilibrium…

Strongly Correlated Electrons · Physics 2009-07-09 J. K. Freericks , H. R. Krishnamurthy , Th. Pruschke

We present a review of our recent work in extending the successful dynamical mean-field theory from the equilibrium case to nonequilibrium cases. In particular, we focus on the problem of turning on a spatially uniform, but possibly time…

Strongly Correlated Electrons · Physics 2008-08-14 V. Turkowski , J. K. Freericks

We present a generalized dynamical mean-field approach for the nonequilibrium physics of a strongly correlated system in the presence of a time-dependent external field. The Keldysh Green's function formalism is used to study the…

Strongly Correlated Electrons · Physics 2007-05-23 P. Schmidt , H. Monien

A Response Function Theory and Scattering Theory applicable to the study of physical properties of systems driven arbitrarily away from equilibrium, specialized for dealing with ultrafast processes and in conditions of space resolution…

Statistical Mechanics · Physics 2012-10-31 Clóves G. Rodrigues , Áurea R. Vasconcellos , José Galvão Ramos , Roberto Luzzi

Time-resolved photoemission spectroscopy is the key technique to probe the real-time non-equilibrium dynamics of electronic states. Theoretical predictions of the time dependent spectral function for realistic systems is however, a…

Computational Physics · Physics 2024-05-24 Cian Reeves , Vojtech Vlcek

In time-resolved photoemission experiments, more than one electron can be emitted from the solid by a single ultra-short pulse. We theoretically demonstrate how correlations between the momenta of outgoing electrons relate to time-dependent…

Strongly Correlated Electrons · Physics 2019-06-26 Christopher Stahl , Martin Eckstein

The power spectral density of an observable quantifies the amount of fluctuations at a given frequency and can reveal the influence of different timescales on the observable's dynamics. Here, we show that the spectral density in a…

Statistical Mechanics · Physics 2023-06-02 Andreas Dechant

Causality implies that by measuring an absorption spectrum, the time-dependent linear response function can be retrieved. Recent experiments suggest a link between the shape of spectral lines observed in absorption spectroscopy with the…

We show that, in optical pump-probe experiments on bulk samples, the statistical distribution of the intensity of ultrashort light pulses after the interaction with a nonequilibrium complex material can be used to measure the time-dependent…

Strongly Correlated Electrons · Physics 2017-11-08 Francesco Randi , Martina Esposito , Francesca Giusti , Fulvio Parmigiani , Oleg Misochko , Daniele Fausti , Martin Eckstein

We study the electron-energy loss spectra of strongly correlated electronic systems doped away from half-filling using dynamical mean-field theory ($d=\infty$). The formalism can be used to study the loss spectra in the optical (${\bf…

Strongly Correlated Electrons · Physics 2009-10-31 Luis Craco , Mukul S. Laad

The linear response of non-equilibrium systems with Markovian dynamics satisfies a generalized fluctuation-dissipation relation derived from time symmetry and antisymmetry properties of the fluctuations. The relation involves the sum of two…

Statistical Mechanics · Physics 2011-01-07 Juan Ruben Gomez-Solano , Artyom Petrosyan , Sergio Ciliberto , Christian Maes

Time-resolved photoemission spectroscopy provides a unique and direct way to explore the real-time nonequilibrium dynamics of electrons and holes. The formal theory of the spectral function evolution requires inclusion of electronic…

Materials Science · Physics 2025-05-09 Thomas Blommel , Enrico Perfetto , Gianluca Stefanucci , Vojtěch Vlček

Using the Kadanoff-Baym-Keldysh formalism, we employ nonequilibrium dynamical mean-field theory to exactly solve for the nonlinear response of an electron-mediated charge-density-wave-ordered material. We examine both the dc current and the…

Strongly Correlated Electrons · Physics 2016-01-20 O. P. Matveev , A. M. Shvaika , T. P. Devereaux , J. K. Freericks

We propose a description of nonequilibrium systems via a simple protocol that combines exchange-correlation potentials from density functional theory with self-energies of many-body perturbation theory. The approach, aimed to avoid double…

Strongly Correlated Electrons · Physics 2016-06-15 M. Hopjan , D. Karlsson , S. Ydman , C. Verdozzi , C. -O. Almbladh
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