Related papers: Four-Wave Mixing in Ultracold Atoms using Intermed…
Rydberg alkaline earth atoms are promising tools for quantum simulation and metrology. When one of the two valence electrons is promoted to long-lived circular states, the second valence electron can be optically manipulated without…
Long-range metastable molecules consisting of two cesium atoms in high Rydberg states have been observed in an ultracold gas. A sequential three-photon two-color photoassociation scheme was employed to form these molecules in states which…
The ac Stark effect was used to induce resonant energy transfer between translationally cold Rydberg atoms. The Rb Rydberg atoms were obtained by laser excitation of cold atoms from a magneto-optical trap. Using two-photon microwave…
We report on the realization of high resolution electron microscopy of Rydberg-excited ultracold atomic samples. The implementation of an ultraviolet laser system allows us to excite the atom, with a single-photon transition, to Rydberg…
Nearly degenerate four-wave mixing (NDFWM) within a closed degenerate two-level atomic transition is theoretically and experimentally examined. Using the model presented by A. Lezama et al [Phys. Rev. A 61, 013801 (2000)] the NDFWM spectra…
We report the creation of ultralong-range Sr$_2$ molecules comprising one ground-state $5s^2$ $^1S_0$ atom and one atom in a $5sns$ $^3S_1$ Rydberg state for $n$ ranging from 29 to 36. Molecules are created in a trapped ultracold atomic gas…
We report on a laser system at a wavelength of 495 nm which is suitable for the excitations of low lying Rydberg states of rubidium atoms. The system is based on frequency doubling of a seeded diode laser in a periodically poled waveguide…
Rydberg helium atoms traveling in pulsed supersonic beams have been coupled to microwave fields in a superconducting coplanar waveguide (CPW) resonator. The atoms were initially prepared in the 1s55s $^3$S$_1$ Rydberg level by two-color…
We experimentally investigate trap-loss spectra of the cesium 6S1/2(F=4)-71P3/2 Rydberg state by combining the cesium atomic magneto-optical trap with the narrow-linewidth, continuously-tunable 318.6 nm ultraviolet laser. That is, the atoms…
Rydberg molecules, often exemplified by long-range "trilobite" molecules, are a subject of much recent interest at high principal quantum number $n$. States that use the same bonding mechanism can exist at much lower $n$ and less-extreme…
We explore the electronic structure of ultralong-range pentaatomic Rydberg molecules from a merger of a Rydberg atom and two ground state heteronuclear diatomic molecules. Our focus is on the interaction of Rb($23s$) and Rb($n=20$, $l\ge…
We demonstrate the ability to excite atoms at well-defined, programmable locations in a magneto-optical trap, either to the continuum (ionisation), or to a Rydberg state. To this end, excitation laser light is shaped into arbitrary…
Within a dense environment ($\rho \approx 10^{14}\,$atoms/cm$^3$) at ultracold temperatures ($T < 1\,\mu{}\text{K}$), a single atom excited to a Rydberg state acts as a reaction center for surrounding neutral atoms. At these temperatures…
We demonstrate a non-equilibrium phase transition in a dilute thermal atomic gas. The phase transition, between states of low and high Rydberg occupancy, is induced by resonant dipole-dipole interactions between Rydberg atoms. The gas can…
Although Rydberg atoms have shown promise for use in novel types of radio frequency receivers, they have generally not been considered phase sensitive without the use of closed-loop interferometry or auxiliary radio frequency fields. Here,…
We propose a scheme for state-insensitive trapping of neutral atoms by using light with two independent wavelengths. In particular, we describe the use of trapping and control lasers to minimize the variance of the potential experienced by…
Radio-frequency (rf) fields in the MHz range are used to induce resonant energy transfer between cold Rydberg atoms in spatially separated volumes. After laser preparation of the Rydberg atoms, dipole-dipole coupling excites the 49s atoms…
We report the measurement of ultrafast relaxation dynamics of excited states of carbon dioxide molecule using time-resolved pump-probe photoelectron spectroscopy. Neutral ground state carbon dioxide is excited to $nd\sigma_g$ Henning sharp…
We examine spectral signatures of Rydberg atoms driven with near-resonant dual-tone radio-frequency (RF) fields in the regime of strong driving. We experimentally demonstrate and theoretically model a variety of nonlinear and multiphoton…
We propose and demonstrate the laser cooling and trapping of Rydberg-dressed Sr atoms. By off-resonantly coupling the excited state of a narrow (7 kHz) cooling transition to a high-lying Rydberg state, we transfer Rydberg properties such as…