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We report Kondo resonances in the conduction of single-molecule transistors based on transition metal coordination complexes. We find Kondo temperatures in excess of 50 K, comparable to those in purely metallic systems. The observed gate…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 L. H. Yu , Z. K. Keane , J. W. Ciszek , L. Cheng , J. M. Tour , T. Baruah , M. R. Pederson , D. Natelson

Over-screened Kondo effect is feasible in carbon nanotube quantum dot junction hosting a spin $\tfrac{1}{2}$ atom with single $s$-wave valence electron (e.g Au). The idea is to use the two valleys as two symmetry protected flavor quantum…

Strongly Correlated Electrons · Physics 2014-08-22 Igor Kuzmenko , Tetyana Kuzmenko , Yshai Avishai

The low temperature properties of single level molecular quantum dots including both, electron-electron and electron-vibration interactions, are theoretically investigated. The calculated differential conductance in the Kondo regime…

Strongly Correlated Electrons · Physics 2016-04-20 P. Roura-Bas , L. Tosi , A. A. Aligia

We study the interplay between Coulomb blockade and the Kondo effect in quantum dots. We use a self-consistent scheme which describes mesoscopic devices in terms of a collective phase variable (slave rotor) and quasiparticle degrees of…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 S. Florens , P. San Jose , F. Guinea , A. Georges

We report manipulation of a Kondo resonance originated from the spin-electron interactions between a two-dimensional molecular assembly of TBrPP-Co molecules and a Cu(111) surface at 4.6 K using a low temperature scanning tunneling…

Materials Science · Physics 2015-06-25 Violeta Iancu , Aparna Deshpande , Saw-Wai Hla*

We investigate the Kondo effect in a quantum dot with almost degenerate spin-singlet and triplet states for an even number of electrons. We show that the Kondo temperature as a function of the energy difference between the states Delta…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Mikio Eto , Yuli V. Nazarov

We use a combination of first principles many-body methods and the numerical renormalization-group technique to study the Kondo regime of cobalt-porphyrin compounds adsorbed on a Cu(111) surface. We find the Kondo temperature to be highly…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Luis G. G. V. Dias da Silva , Murilo L. Tiago , Sergio E. Ulloa , Fernando A. Reboredo , Elbio Dagotto

We have fabricated single electron tunneling structures by forming nanogap metallic electrodes directly upon single self-assembled InAs quantum dots (QDs). The fabricated samples exhibited clear Coulomb blockade effects. Furthermore, a…

Mesoscale and Nanoscale Physics · Physics 2008-08-20 K. Shibata , K. Hirakawa

The Kondo effect arises due to the interaction between a localized spin and the electrons of a surrounding host. Studies of individual magnetic impurities by scanning tunneling spectroscopy have renewed interest in Kondo physics; however, a…

Strongly Correlated Electrons · Physics 2013-08-22 Yong-hui Zhang , Steffen Kahle , Tobias Herden , Christophe Stroh , Marcel Mayor , Uta Schlickum , Markus Ternes , Peter Wahl , Klaus Kern

Molecular electronics offers unique scientific and technological possibilities, resulting from both the nanometre scale of the devices and their reproducible chemical complexity. Two fundamental yet different effects, with no classical…

Mesoscale and Nanoscale Physics · Physics 2017-05-12 Andrew K. Mitchell , Kim G. L. Pedersen , Per Hedegaard , Jens Paaske

A system of two exchange-coupled Kondo impurities in a magnetic field gives rise to a rich phase space hosting a multitude of correlated phenomena. Magnetic atoms on surfaces probed through scanning tunnelling microscopy provide an…

Mesoscale and Nanoscale Physics · Physics 2016-01-05 A. Spinelli , M. Gerrits , R. Toskovic , B. Bryant , M. Ternes , A. F. Otte

We study the dependence of the Kondo temperature on the gate voltage in a strongly blockaded quantum dot with a small single-particle level spacing. We show that the dependence cannot be fitted to that of the Anderson impurity model with…

Mesoscale and Nanoscale Physics · Physics 2012-06-15 Seungjoo Nah , Michael Pustilnik

The electronic structure of a prototype Kondo system, a cobalt impurity in a copper host is calculated with accurate taking into account of correlation effects on the Co atom. Using the recently developed continuous-time QMC technique, it…

Strongly Correlated Electrons · Physics 2015-05-13 E. Gorelov , T. O. Wehling , A. N. Rubtsov , M. I. Katsnelson , A. I. Lichtenstein

We develop a general method to evaluate the Kondo temperature in a multilevel quantum dot that is weakly coupled to conducting leads. Our theory reveals that the Kondo temperature is strongly enhanced when the intradot energy-level spacing…

Strongly Correlated Electrons · Physics 2015-05-20 Ion Garate , Ian Affleck

Local density of states and quasiparticle interference phenomena of Co/Sb(111) were investigated by scanning tunneling spectroscopy. A sharp peak observed near the Fermi energy is interpreted as a fingerprint of the conventional Kondo…

Mesoscale and Nanoscale Physics · Physics 2013-07-25 Limin She , Yinghui Yu , Gengyu Cao

The Kondo effect observed in recent STM experiments on transport through CoPc and TBrPP-Co molecules adsorbed on Au(111) and Cu(111) surfaces, respectively, is discussed within the framework of a simple model (Phys. Rev. Lett. {\bf 97},…

Strongly Correlated Electrons · Physics 2009-11-13 J. M. Aguiar-Hualde , G. Chiappe , E. Louis , E. V. Anda

A low-temperature scanning tunneling microscope was employed to study the differential conductance in an atomic junction formed by an adsorbed Co atom on a Cu(100) surface and a copper-covered tip. A zero-bias anomaly (ZBA) reveals spin…

Mesoscale and Nanoscale Physics · Physics 2018-03-07 Deung-Jang Choi , Paula Abufager , Laurent Limot , Nicolas Lorente

Recently, Coulomb blockade physics was observed at room temperature in a carbon nanotube single-electron transistor (H. W. Ch. Postma, et. al., Science 293, 76 (2001)). In this work, we suggest that these devices may be promising for…

Strongly Correlated Electrons · Physics 2007-05-23 Eugene H. Kim , German Sierra , C. Kallin

The effects of finite temperature in transport through nanoscopic systems exhibiting uniaxial magnetic anisotropy D, such as molecular magnets, adatoms, or quantum dots side-coupled to a large spin are analyzed in the Kondo regime. The…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Maciej Misiorny , Ireneusz Weymann , Józef Barnaś

We study two tunnel-coupled quantum dots each with a spin 1/2 and attached to leads in the Coulomb blockade regime. We study the interplay between Kondo correlations and the singlet-triplet exchange splitting $K$ between the two spins. We…

Strongly Correlated Electrons · Physics 2009-11-07 Vitaly N. Golovach , Daniel Loss