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Related papers: Raman scattering in current carrying molecular jun…

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Non-equilibrium Green's functions (NEGF) formalism combined with extended Huckel (EHT) and charging model are used to study electrical conduction through single-molecule junctions. Analyzed molecular complex is composed of asymmetric…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Kamil Walczak , Sergey Edward Lyshevski

The nonequilibrium Green's function (NEGF) method is often used to predict transport in atomistically resolved nanodevices and yields an immense numerical load when inelastic scattering on phonons is included. To ease this load, this work…

Computational Physics · Physics 2020-07-22 Daniel A. Lemus , James Charles , Tillmann Kubis

The transport and gain properties of quantum cascade (QC) structures are investigated using a nonequilibrium Green's function (NGF) theory which includes quantum effects beyond a Boltzmann transport description. In the NGF theory, we…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 S. -C. Lee , A. Wacker

We propose a scheme for calculation of linear optical response of current-carrying molecular junctions for the case when electronic tunneling through the junction is much faster than characteristic time of external laser field. We discuss…

Mesoscale and Nanoscale Physics · Physics 2008-04-07 Michael Galperin , Sergei Tretiak

Light scattering limits the penetration depth of non-invasive Raman spectroscopy in biological media. While safe levels of irradiation may be adequate to analyze superficial tissue, scattering of the pump beam reduces the Raman signal to…

We study the effects of chemical bonding on Raman scattering from benzenethiol chemisorbed on silver clusters using time-dependent density functional theory (TDDFT). Raman scattering cross sections are computed using a formalism that…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Semion K. Saikin , Roberto Olivares-Amaya , Dmitrij Rappoport , Michael Stopa , Alán Aspuru-Guzik

Computationally inexpensive approximations describing electron-phonon scattering in molecular-scale conductors are derived from the non-equilibrium Green's function method. The accuracy is demonstrated with a first principles calculation on…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Magnus Paulsson , Thomas Frederiksen , Mads Brandbyge

Emphasizing the contribution of Professor Roger A Cowley, FRS to the Theory of Raman Scattering from crystals, the development of the Theory of Raman cattering since 1928 has been briefly discussed. Some experimental studies of Strontium…

Materials Science · Physics 2007-05-23 Jyoti Dhar Sharma

We consider optical spectroscopy of molecular junctions from the quantum transport perspective when radiation field is quantized and optical response of the system is simulated as photon flux. Using exact expressions for photon and…

Mesoscale and Nanoscale Physics · Physics 2016-05-09 Yi Gao , Michael Galperin

We used Raman light scattering to study the current-stabilized nonequilibrium semimetallic and metallic phases in Ca$_2$RuO$_4$. By determining the local temperature through careful analysis of the Stokes and anti-Stokes intensities, we…

Strongly Correlated Electrons · Physics 2019-08-08 K. Fürsich , J. Bertinshaw , P. Butler , M. Krautloher , M. Minola , B. Keimer

The influence of molecular vibration on the Seebeck coefficient is studied within a simple model. Results of a scattering theory approach are compared to those of a full self-consistent non-equilibrium Green's function scheme. We show, for…

Mesoscale and Nanoscale Physics · Physics 2008-06-18 Michael Galperin , Abraham Nitzan , Mark A. Ratner

We investigate the effects of phonon scattering on the electronic current noise through nanojunctions using the non-equilibrium Green's functions formalism extended to include the counting field. In the case of weak electron-phonon coupling…

Mesoscale and Nanoscale Physics · Physics 2009-09-28 Federica Haupt , Tomas Novotny , Wolfgang Belzig

We review the recent developments in electronic Raman scattering measurements of charge nematic fluctuations in iron-based superconductors. A simple theoretical framework of a $d$-wave Pomeranchuk transition is proposed in order to capture…

Superconductivity · Physics 2016-02-17 Yann Gallais , Indranil Paul

In open-shell atoms and ions, processes such as photoionization, combination (Raman) scattering, electron scattering and recombination, are often mediated by many-electron compound resonances. We show that their interference (neglected in…

Atomic Physics · Physics 2015-05-14 V. V. Flambaum , M. G. Kozlov , G. F. Gribakin

Within a generic model we analyze the Stokes linewidth in surface enhanced Raman scattering (SERS) from molecules embedded as bridges in molecular junctions. We identify four main contributions to the off-resonant Stokes signal and show…

Mesoscale and Nanoscale Physics · Physics 2016-06-30 Yi Gao , Michael Galperin , Abraham Nitzan

We use the symmetry constrained low energy effective Hamiltonian of iron based superconductors to study the Raman scattering in the normal state of underdoped iron-based superconductors. The incoming and scattered Raman photons couple…

Strongly Correlated Electrons · Physics 2015-07-01 M. Khodas , A. Levchenko

Surface enhanced Raman spectra from molecules (bipyridyl ethylene) adsorbed on gold dumbells are observed to become increasingly asymmetric (Fano-like) at higher incident light intensity. The electronic temperature (inferred from the…

Mesoscale and Nanoscale Physics · Physics 2016-01-12 S. Dey , M. Banik , E. Hulkko , K. Rodriguez , V. A. Apkarian , M. Galperin , A. Nitzan

A set of theoretical results on infrared absorption and inelastic (Raman) scattering of light in semiconductor quantum dots is reviewed. When it is possible, qualitative comparisons with recent experimental results are presented.

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Augusto Gonzalez , Alain Delgado

Inelastic light scattering is an intensively used tool in the study of electronic properties of solids. Triggered by the discovery of high temperature superconductivity in the cuprates and by new developments in instrumentation, light…

Strongly Correlated Electrons · Physics 2009-11-11 T. P. Devereaux , R. Hackl

A theory of electronic Raman scattering in nearly antiferromagnetic Fermi liquids is constructed using the phenomenological electron-electron interaction introduced by Millis, Monien, and Pines. The role of "hot spots" and their resulting…

Strongly Correlated Electrons · Physics 2009-10-30 T. P. Devereaux , A. P. Kampf