English
Related papers

Related papers: Spontaneous Unknotting of a Polymer Confined in a …

200 papers

Motivated by recent nanofluidics experiments, we use Brownian dynamics and Monte Carlo simulations to study the conformation, organization and dynamics of two polymer chains confined to a single box-like cavity. The polymers are modeled as…

Soft Condensed Matter · Physics 2021-05-19 James M. Polson , Desiree A. Rehel

When a flexible polymer is sucked into a localized small hole, the chain can initially respond only locally and the sequential nonequilibrium processes follow in line with the propagation of the tensile force along the chain backbone. We…

Soft Condensed Matter · Physics 2009-11-13 Takahiro Sakaue

We study the formation of knots on a macroscopic ball-chain, which is shaken on a horizontal plate at 12 times the acceleration of gravity. We find that above a certain critical length, the knotting probability is independent of chain…

Statistical Mechanics · Physics 2007-05-23 J. Hickford , R. Jones , S. Courrech du Pont , J. Eggers

We present an analytical and computational study characterizing the structural and dynamical properties of an active filament confined in cylindrical channels. We first outline the effects of the interplay between confinement and polar…

Soft Condensed Matter · Physics 2024-10-09 José Martín-Roca , Emanuele Locatelli , Valentino Bianco , Paolo Malgaretti , Chantal Valeriani

We present a theoretical analysis of a simple model of the depinning of an anchored semiflexible polymer from a fixed planar substrate in (1+1) dimensions. We consider a polymer with a discrete sequence of pinning sites along its contour.…

Soft Condensed Matter · Physics 2009-11-07 Panayotis Benetatos , Erwin Frey

We study the translocation of polymers across varying-section channels. Using systematic approximations, we derive a simplified model that reduces the problem of polymer translocation through varying-section channels to that of a point-like…

Soft Condensed Matter · Physics 2017-07-13 Valentino Bianco , Paolo Malgaretti

While the dynamics of polymer chains in equilibrium media is well understood by now, the polymer dynamics in active non-equilibrium environments can be very different. Here we study the dynamics of polymers in a viscous medium containing…

Soft Condensed Matter · Physics 2017-06-23 Jaeoh Shin , Andrey G. Cherstvy , Won Kyu Kim , Vasily Zaburdaev

Semi-flexible polymers in crowded environments exhibit complex dynamics that play a crucial role in various biological and material design processes. Based on the classic reptation theory, it is generally believed that semiflexible polymers…

Soft Condensed Matter · Physics 2023-05-05 Ahmad Reza Motezakker , Andrés Córdoba , Tomas Rosén , Fredrik Lundell , L. Daniel Söderberg

The dynamics of loop formation by linear polymer chains has been a topic of several theoretical/experimental studies. Formation of loops and their opening are key processes in many important biological processes. Loop formation in flexible…

Soft Condensed Matter · Physics 2015-05-14 K. P. Santo , K. L. Sebastian

The freely rotating chain is one of the classic discrete models of a polymer in dilute solution. It consists of a broken line of N straight segments of fixed length such that the angle between adjacent segments is constant and the N-1…

Probability · Mathematics 2017-11-15 Philip Kilanowski , Peter March , Marko Samara

The dynamics of flexible polymer molecules are often assumed to be governed by hydrodynamics of the solvent. However there is considerable evidence that internal dissipation of a polymer contributes as well. Here we investigate the dynamics…

Soft Condensed Matter · Physics 2013-05-29 J. M. Deutsch

We investigate the Rouse dynamics of a flexible ring polymer with a prime knot. Within a Monte Carlo approach, we locate the knot, follow its diffusion, and observe the fluctuations of its length. We characterise a topological time scale,…

Statistical Mechanics · Physics 2007-05-23 Enzo Orlandini , Attilio L. Stella , Carlo Vanderzande , Francesco Zonta

We study the structural and dynamical behaviors of a diblock copolymer chain in a bath of active Brownian particles (ABPs) by extensive Brownian dynamics simulation in a two-dimensional model system. Specifically, the A block of chain is…

Soft Condensed Matter · Physics 2019-05-22 Yi-qi Xia , Zhuang-lin Shen , Wen-de Tian , Kang Chen , Yu-qiang Ma

Using molecular dynamics simulations we examine the dynamics of a family of model polymers with varying chain length and torsional potential barriers. We focus on features of the dynamics of polymers that are seen experimentally but absent…

Soft Condensed Matter · Physics 2019-06-11 Daniel Fragiadakis , C. Michael Roland

We consider the unwinding of two lattice polymer strands of length N that are initially wound around each other in a double-helical conformation and evolve through Rouse dynamics. The problem relates to quickly bringing a double-stranded…

Soft Condensed Matter · Physics 2010-10-25 M. Baiesi , G. T. Barkema , E. Carlon , D. Panja

Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

Soft Condensed Matter · Physics 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder

The persistence length of macromolecules is one of their basic characteristics, describing their intrinsic local stiffness. However, it is difficult to extract this length from physical properties of the polymers, different recipes may give…

Soft Condensed Matter · Physics 2013-03-12 Hsiao-Ping Hsu , Wolfgang Paul , Kurt Binder

Semiflexible polymers are widely used as a paradigm for understanding structural phases in biomolecules including folding of proteins. Here, we compare bead-spring and bead-stick variants of coarse-grained semiflexible polymer models that…

Soft Condensed Matter · Physics 2024-02-16 Wolfhard Janke , Suman Majumder , Martin Marenz , Subhajit Paul

We compare Monte Carlo simulations of knotted and unknotted polymers whose ends are connected to two parallel walls. The force $f$ exerted on the polymer is measured as a function of the separation $R$ between the walls. For unknotted…

Statistical Mechanics · Physics 2009-11-07 Oded Farago , Yacov Kantor , Mehran Kardar

The mechanical properties of polymer knots under stretching in a bad or good solvent are investigated by applying a given force $F$ to a point of the knot while keeping another point fixed. The Monte Carlo sampling of the polymer…

Soft Condensed Matter · Physics 2015-12-15 Yani Zhao , Franco Ferrari