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Kinetics of random sequential adsorption (RSA) of spheres on flat, two-dimensional surfaces is governed by a power law with exponent $-1/2$. The study has shown that for RSA of nearly spherically symmetric particles this exponent is $-1/3$,…

Materials Science · Physics 2014-03-14 Michał Cieśla , Jakub Barbasz

Non-local measurements are performed on a multi terminal device to $in-situ$ determine the spin diffusion length and in combination with resistivity measurements also the spin relaxation time in Al films. By varying the thickness of Al we…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 N. Poli , M. Urech , V. Korenivski , D. B. Haviland

Spin properties of organic molecules have attracted great interest for their potential applications in spintronic devices and quantum computing. Fe-tetraphenyl porphyrin (FeTPP) is of particular interest for its robust magnetic properties…

Mesoscale and Nanoscale Physics · Physics 2022-10-19 Mingjun Zhong , Qimeng Wu , Liang Ma , Jie Li , Yifan Wang , Yansong Wang , Xin Li , Yajie Zhang , Jingtao Lü , Yongfeng Wang

We developed a technique to determine suitable spin models for small embedded clusters of arbitrary geometry by combining the spin-cluster expansion with the relativistic disordered local moment scheme. We present results for uncovered and…

Mesoscale and Nanoscale Physics · Physics 2019-04-09 András Lászlóffy , László Udvardi , László Szunyogh

Quantum indistinguishability plays a crucial role in many low-energy physical phenomena, from quantum fluids to molecular spectroscopy. It is, however, typically ignored in most high temperature processes, particularly for ionic…

Chemical Physics · Physics 2018-09-20 Matthew P. A. Fisher , Leo Radzihovsky

The dynamic behavior of a partially wetting polymer droplet driven over a nanostructured interface is studied using molecular dynamics simulations. We consider the bead-spring model to represent a polymeric liquid that partially wets a…

Soft Condensed Matter · Physics 2020-06-17 Anish Thomas , Nikolai V. Priezjev

Molecular nanomagnets are among the first examples of spin systems of finite size and have been test-beds for addressing a range of elusive but important phenomena in quantum dynamics. In fact, for short-enough timescales the spin…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 M. L. Baker , T. Guidi , S. Carretta , J. Ollivier , H. Mutka , H. U. Güdel , G. A. Timco , E. J. L. McInnes , G. Amoretti , R. E. P. Winpenny , P. Santini

Spin squeezing (SS) is a recognized resource for realizing measurement precision beyond the standard quantum limit $\propto 1/\sqrt{N}$. The rudimentary one-axis twisting (OAT) interaction can facilitate SS and has been realized in diverse…

Quantum Gases · Physics 2019-10-16 Feng Chen , Jun-Jie Chen , Ling-Na Wu , Yong-Chun Liu , Li You

A computer code is written that simulates the relaxation back to thermal equilibrium of an ensemble of particles after a pi/2 pulse. Beginning with Bloch's equations the exponential relaxation behavior is discussed and the transition into a…

Medical Physics · Physics 2007-05-23 John L. Haller

We utilize simulations of spin-polarized electron scattering by a chain of localized quantum spins to show that energy and linear momentum conservation laws impose strong constraints on the properties of magnetic excitations induced by spin…

Mesoscale and Nanoscale Physics · Physics 2020-11-11 Alexander Mitrofanov , Sergei Urazhdin

We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, using a cyclic spin system as reference. We consider three variants of antiferromagnetic molecular ring, i.e. Cr$_8$, Cr$_7$Zn and Cr$_7$Ni,…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 S. Carretta , P. Santini , G. Amoretti , M. Affronte , A. Ghirri , I. Sheikin , S. Piligkos , G. Timco , R. E. P. Winpenny

Spin relaxation and decoherence is at the heart of spintronics and spin-based quantum information science. Currently, theoretical approaches that can accurately predict spin relaxation of general solids including necessary scattering…

Materials Science · Physics 2021-12-01 Junqing Xu , Adela Habib , Ravishankar Sundararaman , Yuan Ping

We study the impact of Hund's-rule coupling on orbital excitations, as e.g. measured in inelastic resonant x-ray scattering. We find that the interpretation in terms of spin-orbit separation, which has been derived for one-dimensional…

Strongly Correlated Electrons · Physics 2018-08-15 Jonas Heverhagen , Maria Daghofer

This review describes the physics of spins in quantum dots containing one or two electrons, from an experimentalist's viewpoint. Various methods for extracting spin properties from experiment are presented, restricted exclusively to…

Mesoscale and Nanoscale Physics · Physics 2011-11-09 R. Hanson , L. P. Kouwenhoven , J. R. Petta , S. Tarucha , L. M. K. Vandersypen

In a low-temperature study with a scanning tunneling microscope (STM), the irreducible lateral motion of a CO molecule adsorbed on a Si(001) surface showed a hyperlinear dependence on the tunneling current. This dependence implies that the…

The new generation of proposed light-emitting molecules for OLEDs has raised a considerable research interest due to its exceptional feature-a negative singlet-triplet (ST) gap violating the Hund's multiplicity rule in the excited S1 and T1…

The alkali hyperoxide KO$_2$ is a molecular analog of strongly-correlated systems, comprising of orbitally degenerate magnetic O$_2^-$ ions. Using first-principles electronic structure calculations, we set up an effective spin-orbital model…

Strongly Correlated Electrons · Physics 2008-01-28 I. V. Solovyev

1H nuclear magnetic resonance (NMR) measurements in [YPc2]0, an organic compound formed by radicals stacking along chains, are presented. The temperature dependence of the macroscopic susceptibility, of the NMR shift and of the spin-lattice…

Strongly Correlated Electrons · Physics 2015-05-20 F. Branzoli , P. Carretta , M. Filibian , S. Klyatskaya , M. Ruben

Molecular vibrations are increasingly seen as a key factor for spin dynamics in single-ion magnets and molecular spin qubits. Herein we show how an inexpensive combination of molecular dynamics calculations and a crystal field analysis can…

Mesoscale and Nanoscale Physics · Physics 2018-08-10 Lorena E. Rosaleny , Kirill Zinovjev , Iñaki Tuñón , Alejandro Gaita-Ariño

Recently, the possibility of an all electrical scheme of preparation and readout for a single spin state in a single quantum dot attached to spin biased leads has been shown [F. Chi et al., Phys. Rev. B 81, 075310 (2010)]. However, spin…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Piotr Trocha