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Using density-functional theory, we predict that the oxidation of the Ru(0001) surface proceeds via the accumulation of sub-surface oxygen in two-dimensional islands between the first and second substrate layer. This leads locally to a…

The structure property of non-ideal Si/GaAs heterostructures that were integrated with the ultra-thin oxide (UO) tunneling interfacial layer has been systematically investigated. Si nanomembranes (NMs) were oxidized in different time…

In the present work the effect of surface roughness on oxidation behavior during the early stages of high temperature exposure of Ni-base superalloy IN 625 is described. The surface roughness was described using standard contact…

Materials Science · Physics 2020-11-19 Wojciech J. Nowak

During the last decade, an increasing importance has been given to the feedback of mechanical stresses on the chemical diffusion and, further, on corrosion. Many works point the active role of stresses on the material ageing especially on…

Materials Science · Physics 2013-01-10 Virgil Optasanu , Laura Raceanu , Tony Montesin

The possible importance of oxide formation for the catalytic activity of transition metals in heterogenous oxidation catalysis has evoked a lively discussion over the recent years. On the more noble transition metals (like Pd, Pt or Ag) the…

Materials Science · Physics 2009-11-13 Jutta Rogal , Karsten Reuter , Matthias Scheffler

We study the chemical nature of the bonding of an oxide layer to the parent metal. In order to disentangle chemical effects from strain/misfit, Ti(10$\bar{1}$0)/TiO$_{2}$(100) interface has been chosen. We use the density functional…

Materials Science · Physics 2012-12-10 Linggang Zhu , Graeme J. Ackland

The adsorption of atomic oxygen and its inclusion into subsurface sites on Ag(210) and Ag(410) surfaces have been investigated using density functional theory. We find that--in the absence of adatoms on the first metal layer--subsurface…

Condensed Matter · Physics 2009-11-10 A. Kokalj , N. Bonini , A. Dal Corso , S. de Gironcoli , S. Baroni

In this paper we use molecular dynamics (MD) to answer a classical question: how does the surface tension on a liquid/gas interface appear? After defining surface tension from the first principles and performing several consistency checks,…

Soft Condensed Matter · Physics 2013-10-24 Alex Lukyanov , Alexei Likhtman

Large scale first-principles calculations based on density functional theory (DFT) employing two different methods (atomic orbitals and plane wave basis sets) were used to study the energetics, geometry, the electronic charge redistribution…

Materials Science · Physics 2010-05-27 Vitaly Alexandrov , Sergei Piskunov , Yuri F. Zhukovskii , Eugene A. Kotomin , Joachim Maier

The stress-mediated diffusion of nonequilibrium point defects from the surface to the bulk of the semiconductor is investigated by computer simulation. It is supposed that point defects are generated in the surface region by ion…

Materials Science · Physics 2007-05-23 O. I. Velichko

2D materials present an interesting platform for device designs. However, oxidation can drastically change the system's properties, which need to be accounted for. Through {\it ab initio} calculations, we investigated freestanding and…

Materials Science · Physics 2023-11-21 R. L. H. Freire , F. Crasto de Lima , A. Fazzio

We investigate the dissociation of O2 on Pb(111) surface using first-principles calculations. It is found that in a practical high-vacuum environment, the adsorption of molecular O2 takes place on clean Pb surfaces only at low temperatures…

Chemical Physics · Physics 2015-05-14 Yu Yang , Jia Li , Zhirong Liu , Gang Zhou , Jian Wu , Wenhui Duan , Peng Jiang , Jin-Feng Jia , Qi-Kun Xue , Bing-Lin Gu , S. B. Zhang

Heterogeneous nucleation and subsequent growth of surface water occur on the natural substrate when the water vapor concentration reached the point of super-saturation. This study focuses on the parameterization of super-saturation on the…

Atmospheric and Oceanic Physics · Physics 2019-05-21 Limin Feng , Yang Yu , Huan Xie , Yujiao Zhu , Huiwang Gao , Xiaohong Yao

We report on a combined scanning tunneling microscopy and density functional theory calculation study of the SrTiO3(110)-(4 x 1) surface. It is found that antiphase domains are formed along the [1-10]-oriented stripes on the surface. The…

Strongly Correlated Electrons · Physics 2018-04-16 Zhiming Wang , Fengmiao Li , Sheng Meng , Jiandi Zhang , E. W. Plummer , Ulrike Diebold , Jiandong Guo

We use \textit{ab initio} molecular dynamics simulations to investigate the properties of the dry surface of pure silica and sodium silicate glasses. The surface layers are defined based on the atomic distributions along the direction…

Materials Science · Physics 2021-05-12 Zhen Zhang , Walter Kob , Simona Ispas

The synthesis of materials with well-controlled composition and structure improves our understanding of their intrinsic electrical transport properties. Recent developments in atomically controlled growth have been shown to be crucial in…

X-ray reflectivity measurements on the free surface of liquid Sn are presented. They exhibit the high-angle peak, indicative of surface-induced layering, also found for other pure liquid metals (Hg, Ga and In). However, a low-angle peak,…

The influence of surface oxygen vacancies on the oxygen evolution reaction on bismuth vanadate is studied using hybrid density functional theory. Our findings reveal the thermodynamic instability of the neutral unionized defect (${\rm…

Materials Science · Physics 2023-06-19 Nicklas Österbacka , Hassan Ouhbi , Francesco Ambrosio , Julia Wiktor

The influence of the external pressure and surface energy on the wetting transition at nanotextured interfaces is studied using molecular dynamics and continuum simulations. The surface roughness of the composite interface is introduced via…

Soft Condensed Matter · Physics 2018-07-12 Bishal Bhattarai , Nikolai V. Priezjev

Two-dimensional manganese oxide layers have been grown on Pd(100) and have been characterized by scanning tunnelling microscopy (STM), low-energy electron diffraction (LEED) and X-ray photoelectron spectroscopy (XPS). The complex surface…

Materials Science · Physics 2009-11-13 F. Li , G. Parteder , F. Allegretti , C. Franchini , R. Podloucky , S. Surnev , F. P. Netzer
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